U.S. patent number 3,894,403 [Application Number 05/368,351] was granted by the patent office on 1975-07-15 for vibration-free refrigeration transfer.
This patent grant is currently assigned to Air Products and Chemicals, Inc.. Invention is credited to Ralph C. Longsworth.
United States Patent |
3,894,403 |
Longsworth |
July 15, 1975 |
Vibration-free refrigeration transfer
Abstract
An apparatus for transferring refrigeration to an object to be
cooled without mechanical contact of the refrigerator and object so
that vibrational loads are not transferred to the object. The
apparatus is characterized in that a fluid transfer medium is
caused to circulate in a confined path adjacent the refrigeration
source and the object to effect cooling of the object. An apparatus
such as disclosed is ideally suited for cooling samples for
Mossbauer Spectroscopy.
Inventors: |
Longsworth; Ralph C.
(Allentown, PA) |
Assignee: |
Air Products and Chemicals,
Inc. (Allentown, PA)
|
Family
ID: |
23450863 |
Appl.
No.: |
05/368,351 |
Filed: |
June 8, 1973 |
Current U.S.
Class: |
62/51.1; 505/892;
505/897 |
Current CPC
Class: |
F25D
19/006 (20130101); H01F 6/04 (20130101); Y10S
505/892 (20130101); Y10S 505/897 (20130101) |
Current International
Class: |
F25D
19/00 (20060101); F17C 13/00 (20060101); F17c
007/02 () |
Field of
Search: |
;62/514,45,55 |
References Cited
[Referenced By]
U.S. Patent Documents
Other References
Chow et al., The Use of a Helium Refrigerator for Mossbauer
Studies, 9/2/68, Nuclear Instruments and Methods 66 (1968),
177-180..
|
Primary Examiner: Perlin; Meyer
Assistant Examiner: Capossela; Ronald C.
Attorney, Agent or Firm: Simmons; James C. Noyerman;
Barry
Claims
I claim:
1. Apparatus for transferring refrigeration from a cold
refrigeration source to an object to be cooled comprising in
combination:
a source of cryogenic refrigeration;
means for confining and circulating a fluid transfer medium in
contact with the source of refrigeration; said means including a
structural member affixed to the source of refrigeration thereby
producing an elongated confined flow path for the fluid transfer
medium; and
a support means for holding an object to be cooled in contact with
the circulating fluid transfer medium, the support means being
mounted in spaced relation to the refrigeration source to prevent
forces induced by motion of the refrigeration source from being
transmitted directly to the object support means.
2. An apparatus according to claim 1 wherein the refrigeration
source and object support means are disposed within a vacuum jacket
and the fluid transfer medium is maintained at a pressure of one
atmosphere.
3. An apparatus according to claim 1 wherein the means for
confining and circulating the fluid transfer medium includes a
first heat exchanger in contact with the refrigeration source, the
heat exchanger having a plurality of elongated generally parallel
fluid passages therein for inducing convective circulation of the
fluid transfer medium.
4. An apparatus according to claim 3 including a second heat
exchanger positioned coaxially to the first heat exchanger in
contact with the refrigeration source thereby extending the length
of the circulation path of the fluid transfer medium.
5. An apparatus according to claim 4 wherein a chimney is
interposed between said first and second heat exchangers to further
enhance convective circulation of the fluid transfer medium.
6. An apparatus according to claim 1 including a flexible
bellows-shaped sleeve between the refrigeration source and the
object support means operable as part of the means for confining
the fluid transfer medium, thus preventing transfer of forces
induced by motion of the refrigeration source to the object support
means.
7. An apparatus according to claim 6 wherein the fluid transfer
medium is maintained at a pressure of one atmosphere.
8. An apparatus according to claim 6 wherein the fluid transfer
medium is helium.
9. A superconducting magnet cooling apparatus comprising in
combination:
an elongated cryogenic refrigerator with a cold end disposed
adjacent the superconducting magnet;
means for confining and circulating a fluid transfer medium in
contact with the refrigerator cold end, said means including a heat
exchanger affixed to the refrigerator cold end whereby the heat
exchanger causes the fluid transfer medium to circulate in an
elongated confined flow path; and
a superconducting magnet support, said support positioning the
superconducting magnet in contact with the circulating fluid
transfer medium, the support mounted to prevent forces induced by
motion of the refrigerator from being transmitted directly to the
superconducting magnet.
Description
BACKGROUND OF THE INVENTION
This invention pertains to the field of refrigeration and, in
particular, transfer of refrigeration from a refrigeration source
to an object to be cooled without transfer of vibrational forces
from the refrigeration source to the object being cooled. Such
vibrationless transfer of refrigeration is required for among other
things, cooling samples to be examined by emission and absorption
spectroscopy. One branch of spectroscopy for which this type of
refrigeration transfer is absolutely critical is that which is
known as Mossbauer Spectroscopy. In the late 1950's, one Rudolf
Mossbauer discovered that nuclei that are embedded in solids can
emit and absorb low-energy gamma rays which display the natural
line width and possess the full transition energy. No recoil energy
is transferred to the lattice vibration. This discovery is known as
the Mossbauer effect. In those nuclei with low Debye temperatures,
it becomes necessary for the gamma-ray emitter and absorber to be
cooled to cryogenic temperatures on the order of 10.degree.K
(Kelvin). In order to achieve these temperatures, it had been
necessary to employ a source of liquid helium and/or liquid
nitrogen. For studies following coulomb excitation or nuclear
reactions, the time required for a single run can comprise several
days. In order to achieve a single run, the cost of liquid helium
and the labor involved in maintaining a level of liquid helium are
significant.
More recently, it has been proposed to use a closed-cycle helium
refrigerator to cool the sample for Mossbauer studies. This is set
forth in an article entitled, "The Use of a Helium Refrigerator for
Mossbauer Studies," by Y. W. Chow, E. S. Greenbaum, R. H. Howes, F.
H. H. Hsu, P. H. Swerdlow, and C. S. Wu, which appeared in Nuclear
Instruments and Methods 66 (1968) at Pages 177-180 published by the
North-Holland Publishing Company. In this article the authors
described a helium refrigerator mechanically coupled to the
specimen holder to be cooled by a closed-cycle helium refrigerator.
The article sets forth a bellows arrangement to minimize transfer
of the vibrations associated with the closed-cycle helium
refrigerator from being transferred to the sample holder.
The foregoing article and most of the prior art devices that are
used commercially require a mechanical contact between the
refrigerator and the sample being cooled, such contact is usually
achieved by flexible braided copper straps to further minimize
transfer of vibration from the refrigerator to the sample being
cooled.
It is apparent that if the mechanical coupling has a large enough
cross section to be a good heat conductor then it will also
transmit vibration thus a compromise is always required between the
desire to have a large cross section for good heat transfer and a
small cross section to minimize transmitted vibration.
SUMMARY OF THE INVENTION
In order to overcome the above-described problems and to provide a
more effective vibration-free transfer of refrigeration from a
mechanical refrigeration source to a sample to be cooled, it has
been discovered that if a quantity of a fluid transfer medium is
circulated in a confined path adjacent the refrigeration source
(e.g. cold end of the closed-cycle helium refrigerator) the
circulating fluid transfer medium can be brought in contact with
the sample holder, and the sample can thus be effectively cooled.
In the foregoing apparatus, the sample holder can be mounted
independently of the refrigerator, thus avoiding any mechanical
contact between the source of refrigeration and the sample
undergoing cooling.
Therefore, it is the primary object of this invention to provide an
improved apparatus for transferring of refrigeration.
It is another object of this invention to provide an apparatus for
transfer of refrigeration between a refrigeration source and a
sample to be cooled without mechanical contact of the refrigerator
and the sample.
It is still another object of this invention to provide an
apparatus for transfer of refrigeration from a closed-cycle helium
refrigerator to a sample holder.
It is a further object of this invention to provide a minimized
vibration environment for cooling a sample holder in Mossbauer
Spectroscopy.
BRIEF DESCRIPTION OF THE DRAWING
FIG. 1 is an elevational view partially in section of an apparatus
according to the present invention.
FIG. 2 is an enlarged section taken along line 2--2 of FIG. 1.
FIG. 3 is a fractional portion of the apparatus of FIG. 1 enlarged
for clarity and illustrating another embodiment of the present
invention.
FIG. 4 is an elevational view partially in section showing another
embodiment of the present invention.
FIG. 5 is an elevational view partially in section showing a device
according to the present invention suitable for cooling a
superconducting magnet.
DESCRIPTION OF THE PREFERRED EMBODIMENT
The invention in its broadest aspects will be described as applied
to a sample holder for Mossbauer Spectroscopy. The sample holder
portion of the Mossbauer Spectroscopy technique is shown in FIGS. 1
and 2 and includes a closed-cycle helium refrigerator shown
generally as 10. The refrigerator 10 is of the two-stage type
comprising a first stage 12 and a second stage 14. Such a
refrigerator is capable of producing temperatures of 10.degree.K at
the lower end of the second stage (cold end of the refrigerator)
and extension stud 16. Stud 16 is generally of a high conductivity
material such as copper. A refrigerator such as 10 is disclosed in
detail in U.S. Pat. No. 3,620,029, which Patent specification is
incorporated herein by reference. The present applicant is also the
patentee of the aforementioned U.S. Pat. No. 3,620,029.
The refrigerator 10 is mounted in a support ring 18, which is in
turn fixed to a rigid support such as the floor of the laboratory
building by support member 20. The device also includes a sample
holder designated generally as 22, which sample holder is held by
support 24 which support 24 is in turn fixed to the optical bench
by support members 26. The refrigerator 10 stages 12 and 14 are
inserted inside sample support 22. In order to provide a closed
system, a flexible vibration isolating sleeve 28, such as a very
thin-walled, corrugated rubber sleeve, is affixed to the
refrigerator 10 and sample holder 22 with hose clamps as shown in
FIG. 1.
The sample holder 22 includes an outer vacuum shroud 30 with a
suitable vacuum outlet 32 for evacuating the cavity defined by the
vacuum shroud and the inner system components as will hereinafter
be more fully described. Disposed within the vacuum shroud and
surrounding the first stage 12 of the refrigerator is a stainless
steel inner vacuum jacket sleeve 34. Affixed to the lower end of
sleeve 34 is a radiation shield support adaptor 36. Disposed below
the support adaptor 36 and affixed thereto as by a threaded
connection is a second stage radiation shield 38. The radiation
shield 38 can be a solid copper cylinder or can be with an
aluminized plastic overwrap such as is commonly employed in
cryogenic devices. Disposed within radiation shield 38 and affixed
in fluidtight relation to sleeve 34 is an inner vacuum jacket
extension 40 which surrounds the second stage 14 of the
refrigerator 12. Affixed to the bottom of jacket 40 is a specimen
holder adaptor 42, which in turn supports the sample holder 44. The
specimen holder adaptor 42 includes a series of vertical passages
43, the function of which will be more fully explained
hereinafter.
Disposed around the first stage 12 of the refrigerator is a first
stage heat exchanger 46 and disposed around the copper stud 16 is a
second stage heat exchanger 48. The heat exchangers are shown in
cross section in FIG. 2 and can in one embodiment be manufactured
from a sheet of copper, which is wrapped in cylindrical fashion
with a plurality of vertical spacers 49, thereby defining a series
of vertical flow passages through the heat exchangers 46 and 48.
The heat exchangers 46 and 48, while different in size, are
identical in structure. The heat exchangers provide for convective
circulation of the fluid transfer medium through the vertical
passages as will hereinafter be more fully explained.
The system is completed with an instrument feed through 50 for
measuring temperature and the like. There is also provided a
fitting 52 for introducing the fluid transfer medium into the area
between the refrigerator stages 12, 14 and sleeves 34 and 40.
Fitting 52 includes a pressure relief valve for maintaining one
atmosphere pressure of fluid transfer medium in the nonevacuated
spaces. There is also inlet conduit 54 and outlet conduit 56 for
introducing and removing helium from the refrigerator 10. The inlet
and outlet conduits are connected to a compressor (not shown) by
flexible conduits (not shown) so that the compressor can be
isolated from the refrigerator thereby minimizing any vibration
forces produced by the compressor from being transferred to the
refrigerator 10 and hence to sample holder 44.
The device is assembled as shown with the flexible sleeve 28 fitted
in fluid-tight relationship between the refrigerator 10 and the
sample holder 22. A fluid transfer medium, preferably helium, is
introduced through fitting 52 and fills the space between the
refrigerator 10 (stages 12 and 14) and the sample holder internal
sleeves 34, 40, and 42. The fluid transfer medium port 52 is
connected to a source of fluid transfer medium that will maintain
one atmosphere pressure and the refrigerator is energized, thereby
producing refrigeration at the lower end of first stage 12 and
second stage 14. The refrigeration causes the fluid transfer medium
to circulate in a vertical manner through the heat exchangers 46
and 48 by convective phenomenon. At the lower end of second stage
14, the passages 43 is specimen holder 42 lengthen the circulation
path of the fluid transfer medium, thereby achieving good exchange
of refrigeration between the second stage 14 of refrigerator 10 and
the specimen holder 44. Since there are no mechanical connections
between the heat exchangers and the sample holder, there is no
vibrational loading directly communicated between the refrigerator
and the sample holder. Furthermore, the flexible vibration
isolating sleeve 28 prevents transfer of vibration or other motion
induced forces from other parts of the refrigerator to the sample
holder 22. The vibration isolating sleeve 28 can be of a very thin
flexible material as long as the system operates at one atmosphere,
thereby having equalized pressure inside of the cavity filled by
the fluid transfer medium and outside as determined by ambient
pressure. As long as there is no differential pressure, the
flexible isolating sleeve will isolate vibration and prevent
transfer of vibration forces to the sample holder 44.
It is apparent that with the device, as illustrated in FIG. 1, the
design criteria of maximum transfer of refrigeration per minimum
volume of fluid transfer medium can be achieved by the convective
circulation. The driving force for circulation is the difference in
density between the warm and cold gas and the length of the
confined circulation path as determined by the length of the heat
exchanger 48 in relation to the extreme cold end of the
refrigeration source. The circulation is somewhat enhanced by the
passages 43 and specimen holder 42, however, there is shown in FIG.
3 a further means of enhancing the circulation. As shown in FIG. 3,
a generally cylindrical chimney 100 is interposed between the heat
exchanger 48 and the specimen holder 42, thereby defining a long
flow path through the heat exchanger down to the sample holder 44
and around through passages 43 back up to the upper end of heat
exchanger 48. Such a chimney is preferably made from a
nonconductive material such as bakelite or other plastic material.
The chimney does not mechanically link the refrigerator 10 to the
sample holder 44 so no vibrational loads are transmitted to the
sample holder 44, thus making the device ideally suited for
Mossbauer effect studies.
It is also possible to achieve various temperature levels and
temperature control by using a different transfer fluid in
conjunction with the refrigerator 12 and the sample holder 22 as
shown. For example, at high temperature levels (e.g. 20.degree.K)
more effective refrigeration transfer can be achieved when the
fluid transfer medium is hydrogen and is condensed to a liquid and
then evaporated. A mixture of transfer fluids will achieve a
different range of temperatures so that this condensing mode can be
adequately effected.
There is shown in FIG. 4 yet another embodiment of the present
invention wherein the overall length of the refrigeration system is
shortened. This is achieved by, in essence, folding over the two
stages of the circulating fluid transfer system to effect the
shortened version of the system. In the embodiment of FIG. 4, there
is shown a refrigerator 10' having a first and second stage 12' and
14' respectively as with the embodiment of FIG. 1.
In the embodiment of FIG. 4, the refrigerator is disposed inside of
a fluid housing 70. The housing 70 is isolated from the
refrigerator as in FIG. 1 by a thin, flexible sleeve 28'. The first
stage 12' has two heat exchangers 58, 60 with a chimney device 62
therebetween. The chimney device is affixed to heat exchanger 58
but does not contact heat exchanger 60. The second stage 14' has
heat exchangers 64, 66, and chimney 68 constructed in an identical
manner. The second stage 14' heat exchangers 64, 66 are disposed
within sleeve 72, which sleeve is made to be recessed inside sleeve
70 as shown. Disposed on the end of sleeve 72 is a cold end cap 74,
which is cooled by the second stage 14' cold end of the
refrigerator. As with the embodiment of FIG. 1, the fluid transfer
medium, e.g. helium, is introduced through a suitable port 52 to
fill the space between the refrigerator stages 12', 14' and
corresponding shells 70, 72. The heat exchanger and chimney
combinations, in co-operation with the cooling effect of the
refrigerator, causes convective circulation in both stages of the
fluid transfer medium, thus affecting refrigeration without the
mechanical coupling of the refrigerator to the cold end plate
74.
There is shown in FIG. 5 yet another embodiment of a refrigeration
system wherein the refrigeration system is applied to cooling a
superconducting magnet, which magnet structure includes an outer
vacuum shell 80, a first heat shield 82 which is referred to as a
75.degree.K shield, a second heat shield 84 referred to as a
20.degree.K shield, a liquid helium dewar 86 containing liquid
helium, a magnet cavity 88, magnet 90, helium fill tube 92 and
electrical feed through 94. The refrigerator 10' is identical to
that shown in the embodiment of FIG. 4 having first stage 12' and
second stage 14' with heat exchangers as shown. The first stage 12'
serves to maintain heat shield 82 at temperature of about
75.degree.K and second stage 14' serves to maintain shield 84 at a
temperature of about 20.degree.K thereby minimizing heat leaking
into the liquid helium in dewar 86. With the above-described setup,
it would be possible to provide a Joule-Thompson type cryostat in
conjunction with the refrigerator to maintain the level of liquid
helium in the dewar 86 by taking the vaporized helium in the space
above the liquid level and recondensing it to liquid. Such
cryostats are well known to a worker skilled in the art and their
inclusion would be readily achieved by a skilled artisan.
While the heat exchangers have been described as preferably being
constructed from a sheet copper with spaces brazed thereon, it is
possible to use many types of heat exchangers including folded
copper sheet, a plurality of tubes or the like that will provide
the same elongated closed flow path for circulation of the liquid
transfer medium at the various stages of the refrigerator.
It is also within the purview of this invention to use a
single-stage refrigerator for providing a fixed cryogenic
temperature at the cold end of the refrigerator in an identical
manner using similar structure.
It is also within the purview of the invention to use other fluid
transfer means such as nitrogen, argon, air, hydrogen, halocarbons,
noble gases, methane, and mixtures thereof.
It is still further within the purview of the invention to provide
small mechanical fans or a like forced circulating device at the
extreme ends of the various stages of the refrigerator to further
enhance fluid transfer medium circulation.
Having thus described my invention, the following is desired to be
secured by Letters Patent of the United States.
* * * * *