U.S. patent number 3,790,787 [Application Number 05/240,947] was granted by the patent office on 1974-02-05 for method and device for producing by charge-transfer a beam of neutral particles or of ions having multiple charges.
This patent grant is currently assigned to Commissariat A L'Energie Atomique. Invention is credited to Richard Geller.
United States Patent |
3,790,787 |
Geller |
February 5, 1974 |
METHOD AND DEVICE FOR PRODUCING BY CHARGE-TRANSFER A BEAM OF
NEUTRAL PARTICLES OR OF IONS HAVING MULTIPLE CHARGES
Abstract
A method and device for the production of a beam of neutral
particles or of heavy ions charged a plurality of times in which
electric charges are neutralized or transferred between the charged
particles of an incident beam and a substance traversed by the
beam. A substantially homogeneous stream of powder consisting of
grains having a diameter of the order of 100 A is caused to pass
through the incident beam of charged particles in order to form a
target which is traversed by said beam, the rate of circulation
being such that each charged particle should meet either one grain
or at least a plurality of atoms of one grain.
Inventors: |
Geller; Richard (Grenoble,
FR) |
Assignee: |
Commissariat A L'Energie
Atomique (Paris, FR)
|
Family
ID: |
22908592 |
Appl.
No.: |
05/240,947 |
Filed: |
April 4, 1972 |
Current U.S.
Class: |
250/251;
976/DIG.437; 313/359.1 |
Current CPC
Class: |
H01J
27/02 (20130101); G21K 1/14 (20130101) |
Current International
Class: |
G21K
1/00 (20060101); G21K 1/14 (20060101); H01J
27/02 (20060101); H01j 035/00 () |
Field of
Search: |
;250/41.3,84
;313/63 |
References Cited
[Referenced By]
U.S. Patent Documents
Primary Examiner: Lindquist; William F.
Claims
1. A method of production of a beam of neutral particles or of
heavy ions charged a plurality of times in which electric charges
are neutralized or transferred between the charged particles of an
incident beam and a substance traversed by the beam, the steps of
passing a substantially homogeneous stream of powder consisting of
grains having a diameter of the order of 100 A through the incident
beam of charged particles, forming a target of the powder which is
traversed by said beam, the thickness of the target being
equivalent to the mean free path of charge transfer and adjusting
the rate of circulation of the powder whereby each charged particle
meets either one grain or at least a plurality of atoms of one
2. A device for the production of a beam of neutral particles or
heavy ions charged a plurality of times by neutralization of
charged particles of an incident beam or addition of charges to
said particles, wherein said device comprises a tube, means for
passing a charged particle beam through said tube, and means for
circulating transversely to the beam passing through said tube a
substantially homogeneous flow of powder consisting of grains
having a diameter of the order of 100 A and forming a target, the
thickness of the target being equivalent to the mean free path of
charge transfer, the flow rate of powder being such that each
charged particle
3. A device according to claim 2, wherein said target forming means
includes a vertical duct opening into said tube through which the
beam passes and a supply which releases an adjustable flow of
powder at the
4. A device according to claim 2, wherein said means for forming
said target includes means for giving an electric charge to the
grains of powder and means for creating an electric field for
accelerating the
5. A device according to claim 4, wherein said device includes
means for producing an electric field within a localized zone
outside the beam and the grains which have passed through the beam
entering said zone, said
6. A device according to claim 4 including irradiation means
producing
7. A device according to claim 2, wherein said device includes a
laser in which the beam radiation pressure accelerates the grains
of said powder.
8. A device according to claim 2, the powder being selected from
the group consisting of chromium oxide grains having a grain
diameter on the order of 40 A and of slightly substoichiometric
titanium oxide grains having a particle diameter on the order of 80
A.
Description
This invention relates to a method of production of a beam of
uncharged particles which consists in neutralizing the ions of an
incident beam of charged particles by transfer of electric charges
between said ions and the atoms of a substance which is traversed
by the beam; the invention is also directed to a device for
carrying out said method.
When a beam of I.sup.+ ions passes through a target formed of a
substance having a density N.sub.0 and a thickness 1, the
charge-transfer collisions between the I.sup.+ ions and the atoms A
of the substance neutralize the ions and give rise to neutral or
uncharged particles in accordance with the reaction:
I.sup.+ + A -- I + A.sup.+ (1)
the charge-transfer yield, and therefore the proportion of
uncharged particles in the output beam, is of maximum value if the
density N.sub.0 and the thickness 1 comply with the condition :
N.sub.0 1 = 1/.delta..sub.+.sub.o ( 2)
In formula (2), .delta..sub.+.sub.o designates the electron-capture
charge transfer cross-section : the above condition amounts to
saying that the mean free path of charge transfer is equivalent to
the thickness of the target.
Consideration has been given in the past to a number of different
expedients for satisfying condition (2) at least in an approximate
manner. A first expedient consists in making use of a very thin
diaphragm which is interposed on the path of the beam of ions to be
neutralized. However, a simple calculation shows that the diaphragm
which satisfies condition (2) has a degree of thinness such that it
proves extremely difficult to fabricate and is fragile to such a
degree that it is pierced instantaneously if it is subjected to an
intense beam of particles. By way of example, should it be desired
to convert protons having 5 keV energy (for which
.delta..sub.+.sub.o = 10.sup.-.sup.15 cm.sup.2) to uncharged
particles H.sup.0 having practically the same energy, it is
necessary to have a target consisting of a sheet for which N.sub.0
.sup.. 1 is of the order of 10.sup.15. If the diaphragm is
fabricated from carbon-12, the ideal thickness for said diaphragm
is of the order of 1 A., with a mass per unit area of approximately
0.02 .mu.g/cm.sup.2. In point of fact, the fabrication of
diaphragms having a thickness of less than 100 A is not practicable
in the present state of knowledge.
A diaphragm 100 A in thickness (corresponding to N.sub.0 1 =
10.sup.17) would still be acceptable from the point of view of
neutralization. However, an intense beam of particles which passes
through a diaphragm of this thickness would leave a sufficient
proportion of its energy to destroy the diaphragm practically
instantaneously. The only solution which remains is to adopt
diaphragms having even greater thicknesses which have the
disadvantage of attenuating the beam to a very substantial extent
and to diffuse this latter.
Another solution which also forms part of the prior art consists in
making use of a condensable gas curtain instead of a solid
diaphragm and this curtain circulates transversely to the beam at
supersonic velocity. The gas curtain is discharged at supersonic
velocity from an ejector which must be so designed that the curtain
maintains accurate localization in space (to permit adjustment of
the thickness 1 and of the density N.sub.0) and condenses on a cold
wall. A description of this design concept is given in the
communication by R. Geller and F. Prevot (C.R. Acad. Sc. Paris 38,
page 1578, 1954) to which reference may usefully be made. This
method represents a substantial advance over the previous method.
Carbon dioxide gas, water vapors and magnesium are employed in
particular to form the condensable gas curtain. But this solution
is subject to major difficulties of a technological order when the
particle production rate increases : it is in fact necessary to
increase the flow rate of the gas which constitutes the curtain
progressively as the rate of production of the ions of the incident
beam increases since the gas flow rate at supersonic velocity must
represent a production rate of particles of the same order as that
of the beam in order that each incident ion should find at least
one neutral or uncharged atom with which it can carry out a charge
transfer. In order to achieve neutralization of a beam representing
a charge of several tens of amperes, namely a flux of the order of
10.sup.20 particles per second, and if it is desired to increase
the pressure on each side of the curtain from 1 torr to 10.sup.7
torr over a distance of less than 1 m, the cold condensation wall
must be capable of ensuring a pumping output of the order of 1,000
million liters per second at 10.sup.-.sup.7 torr, which would
represent the equivalent of a large plant within a very small
available volume.
Similar complications would be encountered if, instead of
neutralizing an ion beam, it was desired to convert by
charge-transfer a beam of weakly charged heavy ions into strongly
charged heavy ions. It will be recalled by way of reference that
the charge transfer process applies both to the capture of an
electron (neutralization) and to the loss of one or a number of
electrons when the ion passes through a curtain of material. Since
the probabilities of electron captures or losses are essentially a
function of the energy of the incident ion, in order to strip the
electrons from a weakly charged heavy ion, it is only necessary to
accelerate this latter to a velocity which is higher than that of
its orbital electrons and then to pass said ion through the curtain
of material.
By way of example, there have been obtained nitrogen ion beams of
low intensity but strongly charged by passing through a thin
diaphragm nitrogen ions of 15 MeV energy and charged once. The
composition of the emergent beam was :
ions charged three times : 0.4% " " four " : 6 % namely an average
charge " " five " : 45.6 % of 5.5 " " six " : 40 % " " seven " :
7.5 %
The aim of this invention is to provide a method and a device for
producing by charge-transfer a beam of neutral particles or of
heavy ions charged a plurality of times and capable of receiving
intense particle beams while remaining within a technologically
feasible range. To this end, the invention proposes a method which
is primarily characterized in that a substantially homogeneous
stream of powder consisting of grains having a diameter of the
order of 100 A forming a target is circulated transversely to the
incident beam of charged particles.
The invention also proposes a device for the production of a beam
of neutral particles by neutralization of the ions of an incident
beam, which makes it possible to carry out the method hereinabove
defined, characterized in that said device comprises means for
circulating transversely to the beam a substantially homogeneous
flow of powder consisting of grains having a diameter of the order
of 100 A and forming a target, the flow rate of powder being such
that either one grain or at least a number of atoms of one grain
each to each charged particle.
In accordance with a particular mode of application of the
invention, said means comprise a duct adapted to open into a tube
through which the beam passes, a supply which releases an
adjustable flow of powder at the upper extremity of the duct and
means for creating a vacuum within the tube and the duct.
In accordance with another mode of application, said means for
constituting the target comprise an installation for delivering an
electric charge to the grains of powder and means whereby an
electric field for accelerating the grains towards the beam is
produced within a separate zone with respect to the zone through
which the beam passes.
Within the foregoing definitions, the term "charged particles" must
be interpreted as applying essentially to molecular or atomic ions
which can be accompanied by electrons.
The maximum grain diameter of 100 A corresponding substantially to
the minimum thickness which can possibly be given to a solid
diaphragm is the size which is found in various divided states,
some of which do not in any case exist in the dry state and must
accordingly be rejected. More precisely, there is found in
particular in the grain-size range extending from 20 to 200 A
metallic micelles, various aerosols, dust particles of smokes
constituted by a dispersion in the colloidal state in a gas as well
as charged clusters. The charged clusters, which are agglomerates
of neutral molecules which are formed around ions produced by
ionizing agents, are provided in comparison with the other
substances contemplated above with the property of being charged :
this property offers additional possibilities in the field of
acceleration and collection but, on the other hand, entails the
application of a costly and complex technology.
The powder which is employed must further comply with a certain
number of conditions : the constituent material of said powder must
not permit outgassing or dissociation by producing gases under the
action of the incident particle beam. The grains must not give rise
to particles of larger size by flocculation or coalescence at the
end of a very short half-life. Among the particles whose use can be
contemplated for converting an incident ion beam (nuclei of
deuterium or tritium, for example) into a beam of neutral
particles, it is possible in particular to mention chromium oxide
in the form of powder having a grain size on the order of 40 A and
slightly sub-stoichiometric titanium oxide having a grain size on
the order of 80 A.
Once the powder has been chosen, three parameters are available for
modifying the action of the target of powder on the beam of
particles. These are the rate of passage of the grains, the
thickness 1 of the target and the density N.sub.0 of the target.
The choice will consist of a compromise between requirements which
are to some extent contradictory : on the one hand, it is clearly
necessary to ensure that the flow rate of grains is such that at
least one grain should meet each incident charged particle. In
practice, it will be found necessary to have a much higher ratio in
order to come close to the optimum value so far as the other
conditions are concerned. The ratio N.sub.0 .sup.. 1 must be chosen
so as to comply substantially with condition (2) hereinabove.
Finally, the target must be such that it does not diffuse the
incident beam to an excessive extent. The thickness and the density
of the target as well as the sizes of the unitary grains must
accordingly be chosen in such a manner as to take into account the
energy of the incident particles.
By way of example, if it is assumed that the grains have a diameter
of on the order of 80 A and consist of a substance having a
molecular mass of 50, it is possible to impart a velocity of 1.4
.times. 10.sup.3 cm/sec to the grains by allowing these latter to
fall into empty space over a vertical distance of 10 m. If 100
atoms are permitted for each incident charge particle, a result of
N.sub.0.1 = 5 .times. 10.sup.16 is achieved, that is to say a value
which is scarcely higher than that provided by a solid diaphragm of
very short duration. It is hardly possible for material reasons to
increase the height of drop but, if charged grains are employed, it
is only necessary to have a potential difference of 10 kV in order
to impart a velocity of the order of 10.sup.5 cm/sec to said
grains.
A theoretical study which need not be given here permits a
determination of the angular diffusion of the incident particles.
It is observed that in the case of ions having an energy of more
than 1 KeV and grains having a maximum thickness of 100 A, the
angular diffusion is limited to a few degrees. On the other hand,
electrons are deviated to a much greater extent but this result
represents an advantage rather than a disadvantage in the majority
of applications, in particular in the case of the particle beams
employed in thermonuclear physics in which it is desired to obtain
neutral particles unaccompanied by electrons and produced at the
same time as ions by many accelerating structures.
It is apparent that the invention provides a method and a device
which replaces a static diaphragm having a thickness 1 which is
incapable of withstanding an intense ion beam by a target
constituted by flowing powder, the grians of which are continuously
renewed. Provided that the powder which is selected does not
undergo intense outgassing under the action of incident ion beam,
there is no restrictive condition similar to that which is
attendant upon the use of a condensable gas target.
A clearer understanding of the invention will be gained from the
following description of a particular device for carrying out the
invention which is given by way of non-limitative example,
reference being made to the accompanying drawings, wherein :
Fig. 1 is a sectional diagram of the device ;
Fig. 2 is a view in elevation showing the device of FIG. 1.
The device which is illustrated diagrammatically in FIG. 1 and from
the exterior in FIG. 2 comprises a reservoir 10 for receiving the
powder. A filling opening 12 fitted with a leak-tight valve 14
serves to introduce the powder therein. The reservoir 10 is
connected by means of an adjustable leakage cock 16 to a pumping
installation for creating a vacuum therein. The leakage cock 16
permits progressive evacuation of the system which is compatible
with the capacity of the pumping installation. This installation
can consist solely of a primary pump 18 (shown in FIG. 2). There is
also shown in the diagram of FIG. 1 a duct 20 for introducing an
inert rinsing gas into the reservoir.
The dimensions of the reservoir 10 are such that this latter
ensures a certain degree of self-contained operation and prevents
over-frequent opening of the system, the result of which would be
to release the vacuum. As a rule, this reservoir will be provided
with moisture absorbent, with resistors for heating the walls and
with calibrated screens for filtering the powder which escapes
therefrom.
The powder 22 which rests on the bottom of the reservoir 10 flows
towards a supply tank 24 through a duct 25 fitted with a
flow-regulating valve 27, said tank being placed at a lower level
and fitted with a slow-agitation device for maintaining the powder
in the form of a homogeneous suspension. The tank 24 which is
illustrated has a cylindrical shape and is fitted with a rotary
stirrer 26 which ensures controlled agitation. Instead of a rotary
stirrer, it would be possible to make use of other known types such
as those which operate by translational motion ; the transmission
can be effected without passing through the wall, for example by
electromagnetic means. The stirrer can also be replaced by a sound
generator: the major condition to be satisfied consists in
preventing any deposit or sedimentation of the powder and in
maintaining a substantially homogeneous concentration within the
entire tank 24.
The tank 24 communicates through a duct 28 with a vacuum
installation which can be the same as that of the reservoir 10.
Baffles 30 (shown in FIG. 1) must usually be provided within the
tank in order to prevent the entrainment towards the pumping
installation of the powder grains which are maintained in
suspension by means of the stirrer.
The tank 24 supplies by means of a variable-flow valve 32 a
vertical duct 34 for the acceleration of the powder grains. The
length of this duct is determined as a function of the velocity to
be imparted to the grains in that portion of their trajectory in
which they constitute the target. The duct 34 has its opening in a
charge-transfer cell 35 traversed by the tube through which the
incident ion beam 36 passes. A branch pipe 38 is taken off the duct
34 and connected to a pumping installation which serves to produce
a vacuum therein. So far as concerns the transfer cell through
which the ion beam passes, said cell is connected at 40 to a
pumping installation which can be common with that of the
powder-recovery chamber 42.
The chamber 42 in which the powder collects under the action of
gravity, is connected by means of the duct 44 to a vacuum-producing
installation which comprises not only a primary pump (not shown),
but also a secondary vacuum pump 46 (ion pump, for example). The
powder which collects at the bottom of the chamber can be withdrawn
through a duct 48 and regenerated in order to permit re-use or else
is finally removed, depending on requirements.
The charge-transfer cell 35 which is illustrated diagrammatically
in FIGS. 1 and 2 corresponds to the case of an incident beam 36
made up of ions and electrons such as the beams produced by an
accelerator of the "Pleiade" type, a description of which may be
found in the article by T. Consoli entitled "H.F. Fields and Plasma
Accelerators" (B.I.S.T. No. 102, March, 1966, pages 35 to 48), to
which reference may usefully be made. With this type of beam, it is
necessary to ensure that the transfer cell 35 in which the incident
ions (hydrogen or deuterium nuclei) yield their charge to the
powder is placed in an intense magnetic field produced by coils 49.
In this case, the beam 50 which is delivered from the cell is
essentially composed of neutral particles derived from the incident
ions, a high proportion of the electrons having been diffused by
the powder and retained by the collimator 52.
The powder is brought up to speed solely under the action of
gravity within the vertical pipe 34 which is illustrated in FIGS. 1
and 2. Other solutions can be employed, especially when it is
sought to attain a high velocity. In the case of batch operation,
the action of periodic jets of fluid or of impulses produced by a
piston may be added to the action of gravity. A further solution
consists in charging the powder grains (for example by causing
these latter to pass through a low-energy electron cloud which
yields negative charges to said grains or by subjecting these
latter to electron bombardment which causes the appearance of
positive charges). It is also possible to make use of charged
clusters. In this case, the grains can be accelerated by an
electric field at the outlet of the tank 24. The collection of the
powder can also be obtained by means of a localized electric field
in the chamber 42.
Finally, the grains of substance can be accelerated by employing
the radiation pressure of a laser beam disposed above the powder
jet.
It is readily apparent that the invention is not limited to the
embodiment hereinabove described and illustrated by way of example
and accordingly extends to alternative forms of either all or part
of the arrangements described which remain within the definition of
equivalent means.
* * * * *