Tricyclic Benzoylpyrazole Derivatives

Abstract

Tricyclic benzoylpyrazole derivatives of the formula I ##STR1## where: X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7, NR.sup.8 or a bond; Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated 5- or 6-membered heterocycle; R.sup.1, R.sup.2, R.sup.6, R.sup.7 are hydrogen, alkyl, haloalkyl, alkoxy or haloalkoxy; R.sup.3 is halogen, alkyl, haloalkyl, alkoxy or haloalkoxy; R.sup.4 is hydrogen, nitro, halogen, cyano, alkyl, haloalkyl, alkoxy, haloalkoxy, alkylthio, haloalkylthio, alkylsulfinyl, haloalkylsulfinyl, alkylsulfonyl, haloalkylsulfonyl, unsubstituted or substituted aminosulfonyl or unsubstituted or substituted sulfonylamino; R.sup.5 is hydrogen, alkyl or halogen; l is 0, 1 or 2; R.sup.8 is hydrogen, alkyl, haloalkyl, alkylcarbonyl, formyl, alkoxycarbonyl, haloalkoxycarbonyl, alkylsulfonyl or haloalkylsulfonyl; R.sup.9 is substituted pyrazol-4-ylcarbonyl or substituted 5-oxopyrazolin-4-ylmethylidene; and their agriculturally useful salts; processes and intermediates for preparing the tricyclic benzoylpyrazole derivatives; compositions comprising them and the use of these derivatives or of the compositions comprising them for controlling undesirable plants are described.

Description

[0001] The present invention relates to novel tricyclic benzoylpyrazole derivatives of the formula I ##STR2## where: [0002] X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7, NR.sup.8 or a bond; [0003] Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated 5- or 6-membered heterocycle which contains one to three identical or different heteroatoms selected from the following group: oxygen, sulfur or nitrogen; [0004] R.sup.1, R.sup.2, R.sup.6, R.sup.7 are hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0005] R.sup.3 is halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0006] R.sup.4 is hydrogen, nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl) amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; [0007] R.sup.5 is hydrogen, C.sub.1-C.sub.6-alkyl or halogen; [0008] R.sup.8 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkylcarbonyl, formyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.1-C.sub.6-haloalkoxycarbonyl, C.sub.1-C.sub.6-alkylsulfonyl or C.sub.1-C.sub.6-haloalkylsulfonyl; [0009] l is 0, 1 or 2; [0010] R.sup.9 is a radical IIa or IIb ##STR3## where [0011] R.sup.10 is hydroxyl, mercapto, halogen, OR.sup.13, SR.sup.13, SO.sub.2R.sup.14, NR.sup.15R.sup.16 or N-bonded heterocyclyl, where the heterocyclyl radical may be partially or fully halogenated and/or may carry one to three of the following radicals: [0012] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; [0013] R.sup.11 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.3-C.sub.6-cycloalkyl, hydroxyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0014] R.sup.12 is hydrogen, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, hydroxyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-haloalkylthio; [0015] R.sup.13 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-alkynyl, C.sub.3-C.sub.6-haloalkynyl, C.sub.3-C.sub.6-cycloalkyl, C.sub.1-C.sub.20-alkylcarbonyl, C.sub.2-C.sub.20-alkenylcarbonyl, C.sub.2-C.sub.6-alkynylcarbonyl, C.sub.3-C.sub.6-cycloalkylcarbonyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.3-C.sub.6-alkenyloxycarbonyl, C.sub.3-C.sub.6-alkynyloxycarbonyl, C.sub.1-C.sub.6-alkylthiocarbonyl, C.sub.1-C.sub.6-alkylaminocarbonyl, C.sub.3-C.sub.6-alkenylaminocarbonyl, C.sub.3-C.sub.6-alkynylaminocarbonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkyl) aminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.1-C.sub.6-alkoxy)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl, di(C.sub.1-C.sub.6-alkyl)aminothiocarbonyl, C.sub.1-C.sub.6-alkylcarbonyl-C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-alkoxyimino-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl or N,N-di(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl, where the abovementioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three of the following groups: [0016] cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, di(C.sub.1-C.sub.4-alkyl)amino, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxycarbonyl, di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, C.sub.1-C.sub.4-alkylaminocarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; [0017] is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl, heterocyclyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl-C.sub.1-C.sub.6-alkyl, heterocyclylcarbonyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl, heterocyclylcarbonyl, phenoxycarbonyl, phenyloxythiocarbonyl, heterocyclyloxycarbonyl, heterocyclyloxythiocarbonyl, phenylaminocarbonyl, N--(C.sub.1-C.sub.6-alkyl)-N-(phenyl)aminocarbonyl, heterocyclylaminocarbonyl, N--(C.sub.1-C.sub.6-alkyl)-N-(heterocyclyl)aminocarbonyl, phenyl-C.sub.2-C.sub.6-alkenylcarbonyl or heterocyclyl-C.sub.2-C.sub.6-alkenylcarbonyl, where the phenyl and the heterocyclyl radical of the 18 lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: [0018] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-haloalkoxy, heterocyclyl or N-bonded heterocyclyl, where the two lastmentioned substitutents for their part may be partially or fully halogenated and/or may carry one to three of the following radicals: [0019] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; [0020] R.sup.14 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-alkynyl, C.sub.3-C.sub.6-haloalkynyl, C.sub.3-C.sub.6-cycloalkyl, C.sub.1-C.sub.6-alkoxy, di(C.sub.1-C.sub.6-alkyl)amino or di(C.sub.1-C.sub.6-haloalkyl)amino, where the above-mentioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three of the following groups: [0021] cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, di(C.sub.1-C.sub.4-alkyl)amino, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxycarbonyl, di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, C.sub.1-C.sub.4-alkylaminocarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; [0022] is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl, heterocyclyl-C.sub.1-C.sub.6-alkyl, phenoxy, heterocyclyloxy, where the phenyl and the heterocyclyl radical of the lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: [0023] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; [0024] R.sup.15 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-alkynyl, C.sub.3-C.sub.6-haloalkynyl, C.sub.3-C.sub.6-cycloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.3-C.sub.6-alkenyloxy, C.sub.3-C.sub.6-alkynyloxy, di(C.sub.1-C.sub.6-alkyl)amino or C.sub.1-C.sub.6-alkylcarbonylamino, where the abovementioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three radicals of the following group: [0025] cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, di(C.sub.1-C.sub.4-alkyl)amino, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxycarbonyl, di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, C.sub.1-C.sub.4-alkylaminocarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; [0026] is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl or heterocyclyl-C.sub.1-C.sub.6-alkyl, where the phenyl or heterocyclyl radical of the four lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: [0027] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; [0028] R.sup.16 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-alkynyl or C.sub.1-C.sub.6-alkylcarbonyl; and their agriculturally useful salts.

[0029] Moreover, the invention relates to processes and intermediates for preparing compounds of the formula I, to compositions comprising them, and to the use of these derivatives or of the compositions comprising them for controlling harmful plants.

[0030] WO 97/19087 and EP-A 860 441 disclose tricyclic compounds which are characterized in that the respective benzoyl unit that they contain is fused via positions 3 and 4 with a bicycle. However, the herbicidal properties of the prior-art compounds and their compatibility with crop plants are not entirely satisfactory. It is an object of the present invention to provide novel, biologically, in particular herbicidally, active compounds having improved properties.

[0031] We have found that this object is achieved by the tricyclic benzoylpyrazole derivatives of the formula I and their herbicidal action.

[0032] Furthermore, we have found processes and intermediates for synthesizing the compounds of the formula I. Likewise, we have found herbicidal compositions which comprise the compounds I and have very good herbicidal action. Moreover, we have found processes for preparing these compositions and methods for controlling undesirable vegetation using the compounds I.

[0033] Depending on the substitution pattern, the compounds of the formula I can contain one or more chiral centers, in which case they are present as enantiomers or diastereomer mixtures. The invention provides both the pure enantiomers or diastereomers and their mixtures.

[0034] The compounds of the formula I can also be present in the form of their agriculturally useful salts, the type of salt generally being immaterial. Generally suitable are the salts of those cations or the acid addition salts of those acids whose cations and anions, respectively, do not negatively affect the herbicidal action of the compounds I.

[0035] Suitable cations are, in particular, ions of the alkali metals, preferably lithium, sodium and potassium, of the alkaline earth metals, preferably calcium and magnesium, and of the transition metals, preferably manganese, copper, zinc and iron, and also ammonium, where, if desired, one to four hydrogen atoms may be replaced by C.sub.1-C.sub.4-alkyl, hydroxy-C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkyl, hydroxy-C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkyl, phenyl or benzyl, preferably ammonium, dimethylammonium, diisopropylammonium, tetramethylammonium, tetrabutylammonium, 2-(2-hydroxyeth-1-oxy)eth-1-ylammonium, di(2-hydroxyeth-1-yl)ammonium, trimethylbenzylammonium, furthermore phosphonium ions, sulfonium ions, preferably tri(C.sub.1-C.sub.4-alkyl)sulfonium, and sulfoxonium ions, preferably tri(C.sub.1-C.sub.4-alkyl)sulfoxonium.

[0036] Anions of useful acid addition salts are primarily chloride, bromide, fluoride, hydrogen sulfate, sulfate, dihydrogen phosphate, hydrogen phosphate, nitrate, hydrogen carbonate, carbonate, hexafluorosilicate, hexafluorophosphate, benzoate and the anions of C.sub.1-C.sub.4-alkanoic acids, preferably formate, acetate, propionate and butyrate.

[0037] In the case of R.sup.10=hydroxyl or mercapto, IIa also represents the tautomeric forms IIa' and IIa'' ##STR4##

[0038] Likewise, in the case of R.sup.10=hydroxyl or mercapto, IIb also represents the tautomeric forms IIb' and IIb'' ##STR5##

[0039] The organic molecular moieties mentioned for the substitutents R.sup.1-R.sup.17 or as radicals on phenyl and heterocyclyl radicals are collective terms for individual enumerations of the individual group members. All hydrocarbon chains, i.e. all alkyl, haloalkyl, hydroxyalkyl, alkoxy, haloalkoxy, alkylthio, haloalkylthio, alkylsulfinyl, haloalkylsulfinyl, alkylsulfonyl, haloalkylsulfonyl, N-alkylaminosulfonyl, N,N-dialkylaminosulfonyl, N-alkylamino, N,N-dialkylamino, N-haloalkylamino, N,N-dihaloalkylamino, N-alkylsulfonylamino, N-haloalkylsulfonylamino, N-alkyl-N-alkylsulfonylamino, N-alkyl-N-haloalkylsulfonylamino, alkylcarbonyl, alkoxycarbonyl, haloalkoxycarbonyl, alkylthiocarbonyl, alkylcarbonyloxy, alkylaminocarbonyl, dialkylaminocarbonyl, dialkylaminothiocarbonyl, alkoxyalkyl, hydroxyalkoxyalkyl, alkylcarbonylalkyl, alkoxyiminoalkyl, N-(alkylamino)iminoalkyl, N-(dialkylamino)iminoalkyl, phenylalkenylcarbonyl, heterocyclylalkenylcarbonyl, N-alkoxy-N-alkylaminocarbonyl, N-alkyl-N-phenylaminocarbonyl, N-alkyl-N-heterocyclylaminocarbonyl, phenylalkyl, heterocyclylalkyl, phenylcarbonylalkyl, heterocyclylcarbonylalkyl, dialkylaminoalkoxycarbonyl, alkoxyalkoxycarbonyl, alkenylcarbonyl, alkenyloxycarbonyl, alkenylaminocarbonyl, N-alkenyl-N-alkylaminocarbonyl, N-alkenyl-N-alkoxyaminocarbonyl, alkynylcarbonyl, alkynyloxycarbonyl, alkynylaminocarbonyl, N-alkynyl-N-alkylaminocarbonyl, N-alkynyl-N-alkoxyaminocarbonyl, alkenyl, alkynyl, haloalkenyl, haloalkynyl, alkenyloxy and alkynyloxy moieties, may be straight-chain or branched. Unless indicated otherwise, halogenated substitutents preferably carry one to five identical or different halogen atoms. The term halogen denotes in each case fluorine, chlorine, bromine or iodine.

[0040] Examples of other meanings are: [0041] C.sub.1-C.sub.4-alkyl and the alkyl moieties of hydroxy-C.sub.1-C.sub.4-alkyl: for example methyl, ethyl, propyl, 1-methylethyl, butyl, 1-methylpropyl, 2-methylpropyl or 1,1-dimethylethyl; [0042] C.sub.1-C.sub.6-alkyl, and the alkyl moieties of C.sub.1-C.sub.6-alkylcarbonyl-C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-alkoxyimino-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl, N-(di-C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkoxy)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.1-C.sub.6-alkyl)-N-phenylaminocarbonyl, N--(C.sub.1-C.sub.6-alkyl)-N-heterocyclylaminocarbonyl, phenyl-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl) amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, heterocyclyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl-C.sub.1-C.sub.6-alkyl, heterocyclylcarbonyl-C.sub.1-C.sub.6-alkyl: C.sub.1-C.sub.4-alkyl as mentioned above, and also, for example, pentyl, 1-methylbutyl, 2-methylbutyl, 3-methylbutyl, 2,2-dimethylpropyl, 1-ethylpropyl, hexyl, 1,1-dimethylpropyl, 1,2-dimethylpropyl, 1-methylpentyl, 2-methylpentyl, 3-methylpentyl, 4-methylpentyl, 1,1-dimethylbutyl, 1,2-dimethylbutyl, 1,3-dimethylbutyl, 2,2-dimethylbutyl, 2,3-dimethylbutyl, 3,3-dimethylbutyl, 1-ethylbutyl, 2-ethylbutyl, 1,1,2-trimethylpropyl, 1-ethyl-1-methylpropyl or 1-ethyl-3-methylpropyl; [0043] C.sub.1-C.sub.4-haloalkyl: a C.sub.1-C.sub.4-alkyl radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, chloromethyl, dichloromethyl, trichloromethyl, fluoromethyl, difluoromethyl, trifluoromethyl, chlorofluoromethyl, dichlorofluoromethyl, chlorodifluoromethyl, 2-fluoroethyl, 2-chloroethyl, 2-bromoethyl, 2-iodoethyl, 2,2-difluoroethyl, 2,2,2-trifluoroethyl, 2-chloro-2-fluoroethyl, 2-chloro-2,2-difluoroethyl, 2,2-dichloro-2-fluoroethyl, 2,2,2-trichloroethyl, pentafluoroethyl, 2-fluoropropyl, 3-fluoropropyl, 2,2-difluoropropyl, 2,3-difluoropropyl, 2-chloropropyl, 3-chloropropyl, 2,3-dichloropropyl, 2-bromopropyl, 3-bromopropyl, 3,3,3-trifluoropropyl, 3,3,3-trichloropropyl, 2,2,3,3,3-pentafluoropropyl, heptafluoropropyl, 1-(fluoromethyl)-2-fluoroethyl, 1-(chloromethyl)-2-chloroethyl, 1-(bromomethyl)-2-bromoethyl, 4-fluorobutyl, 4-chlorobutyl, 4-bromobutyl or nonafluorobutyl; [0044] C.sub.1-C.sub.6-haloalkyl, and the haloalkyl moieties of N--C.sub.1-C.sub.6-haloalkylamino and N,N-(di-C.sub.1-C.sub.6-haloalkyl)amino: C.sub.1-C.sub.4-haloalkyl as mentioned above, and also, for example, 5-fluoropentyl, 5-chloropentyl, 5-bromopentyl, 5-iodopentyl, undecafluoropentyl, 6-fluorohexyl, 6-chlorohexyl, 6-bromohexyl, 6-iodohexyl or dodecafluorohexyl; [0045] C.sub.1-C.sub.4-alkoxy: for example methoxy, ethoxy, propoxy, 1-methylethoxy, butoxy, 1-methylpropoxy, 2-methylpropoxy or 1,1-dimethylethoxy; [0046] C.sub.1-C.sub.6-alkoxy, and the alkoxy moieties of C.sub.1-C.sub.6-alkoxyimino-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkoxy)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl and N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl: C.sub.1-C.sub.4-alkoxy as mentioned above, and also, for example, pentoxy, 1-methylbutoxy, 2-methylbutoxy, 3-methylbutoxy, 1,1-dimethylpropoxy, 1,2-dimethylpropoxy, 2,2-dimethylpropoxy, 1-ethylpropoxy, hexoxy, 1-methylpentoxy, 2-methylpentoxy, 3-methylpentoxy, 4-methylpentoxy, 1,1-dimethylbutoxy, 1,2-dimethylbutoxy, 1,3-dimethylbutoxy, 2,2-dimethylbutoxy, 2,3-dimethylbutoxy, 3,3-dimethylbutoxy, 1-ethylbutoxy, 2-ethylbutoxy, 1,1,2-trimethylpropoxy, 1,2,2-trimethylpropoxy, 1-ethyl-1-methylpropoxy or 1-ethyl-2-methylpropoxy; [0047] C.sub.1-C.sub.4-haloalkoxy: a C.sub.1-C.sub.4-alkoxy radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, fluoromethoxy, difluoromethoxy, trifluoromethoxy, chlorodifluoromethoxy, bromodifluoromethoxy, 2-fluoroethoxy, 2-chloroethoxy, 2-bromoethoxy, 2-iodoethoxy, 2,2-difluoroethoxy, 2,2,2-trifluoroethoxy, 2-chloro-2-fluoroethoxy, 2-chloro-2,2-difluoroethoxy, 2,2-dichloro-2-fluoroethoxy, 2,2,2-trichloroethoxy, pentafluoroethoxy, 2-fluoropropoxy, 3-fluoropropoxy, 2-chloropropoxy, 3-chloropropoxy, 2-bromopropoxy, 3-bromopropoxy, 2,2-difluoropropoxy, 2,3-difluoropropoxy, 2,3-dichloropropoxy, 3,3,3-trifluoropropoxy, 3,3,3-trichloropropoxy, 2,2,3,3,3-pentafluoropropoxy, heptafluoropropoxy, 1-(fluoromethyl)-2-fluoroethoxy, 1-(chloromethyl)-2-chloroethoxy, 1-(bromomethyl)-2-bromoethoxy, 4-fluorobutoxy, 4-chlorobutoxy, 4-bromobutoxy or nonafluorobutoxy; [0048] C.sub.1-C.sub.6-haloalkoxy: C.sub.1-C.sub.4-haloalkoxy as mentioned above, and also, for example, 5-fluoropentoxy, 5-chloropentoxy, 5-bromopentoxy, 5-iodopentoxy, undecafluoropentoxy, 6-fluorohexoxy, 6-chlorohexoxy, 6-bromohexoxy, 6-iodohexoxy or dodecafluorohexoxy; [0049] C.sub.1-C.sub.4-alkylthio: for example methylthio, ethylthio, propylthio, 1-methylethylthio, butylthio, 1-methylpropylthio, 2-methylpropylthio or 1,1-dimethylethylthio; [0050] C.sub.1-C.sub.6-alkylthio, and the alkylthio moieties of C.sub.1-C.sub.6-alkylthiocarbonyl: C.sub.1-C.sub.4-alkylthio as mentioned above and also, for example, pentylthio, 1-methylbutylthio, 2-methylbutylthio, 3-methylbutylthio, 2,2-dimethylpropylthio, 1-ethylpropylthio, hexylthio, 1,1-dimethylpropylthio, 1,2-dimethylpropylthio, 1-methylpentylthio, 2-methylpentylthio, 3-methylpentylthio, 4-methylpentylthio, 1,1-dimethylbutylthio, 1,2-dimethylbutylthio, 1,3-dimethylbutylthio, 2,2-dimethylbutylthio, 2,3-dimethylbutylthio, 3,3-dimethylbutylthio, 1-ethylbutylthio, 2-ethylbutylthio, 1,1,2-trimethylpropylthio, 1,2,2-trimethylpropylthio, 1-ethyl-1-methylpropylthio or 1-ethyl-2-methylpropylthio; [0051] C.sub.1-C.sub.6-haloalkylthio: a C.sub.1-C.sub.6-alkylthio radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, fluoromethylthio, difluoromethylthio, trifluoromethylthio, chlorodifluoromethylthio, bromodifluoromethylthio, 2-fluoroethylthio, 2-chloroethylthio, 2-bromoethylthio, 2-iodoethylthio, 2,2-difluoroethylthio, 2,2,2-trifluoroethylthio, 2,2,2-trichloroethylthio, 2-chloro-2-fluoroethylthio, 2-chloro-2,2-difluoroethylthio, 2,2-dichloro-2-fluoroethylthio, pentafluoroethylthio, 2-fluoropropylthio, 3-fluoropropylthio, 2-chloropropylthio, 3-chloropropylthio, 2-bromopropylthio, 3-bromopropylthio, 2,2-difluoropropylthio, 2,3-difluoropropylthio, 2,3-dichloropropylthio, 3,3,3-trifluoropropylthio, 3,3,3-trichloropropylthio, 2,2,3,3,3-pentafluoropropylthio, heptafluoropropylthio, 1-(fluoromethyl)-2-fluoroethylthio, 1-(chloromethyl)-2-chloroethylthio, 1-(bromomethyl)-2-bromoethylthio, 4-fluorobutylthio, 4-chlorobutylthio, 4-bromobutylthio, nonafluorobutylthio, 5-fluoropentylthio, 5-chloropentylthio, 5-bromopentylthio, 5-iodopentylthio, undecafluoropentylthio, 6-fluorohexylthio, 6-chlorohexylthio, 6-bromohexylthio, 6-iodohexylthio or dodecafluorohexylthio; [0052] C.sub.1-C.sub.6-alkylsulfinyl (C.sub.1-C.sub.6-alkyl-S(.dbd.O)--): for example methylsulfinyl, ethylsulfinyl, propylsulfinyl, 1-methylethylsulfinyl, butylsulfinyl, 1-methylpropylsulfinyl, 2-methylpropylsulfinyl, 1,1-dimethylethylsulfinyl, pentylsulfinyl, 1-methylbutylsulfinyl, 2-methylbutylsulfinyl, 3-methylbutylsulfinyl, 2,2-dimethylpropylsulfinyl, 1-ethylpropylsulfinyl, 1,1-dimethylpropylsulfinyl, 1,2-dimethylpropylsulfinyl, hexylsulfinyl, 1-methylpentylsulfinyl, 2-methylpentylsulfinyl, 3-methylpentylsulfinyl, 4-methylpentylsulfinyl, 1,1-dimethylbutylsulfinyl, 1,2-dimethylbutylsulfinyl, 1,3-dimethylbutylsulfinyl, 2,2-dimethylbutylsulfinyl, 2,3-dimethylbutylsulfinyl, 3,3-dimethylbutylsulfinyl, 1-ethylbutylsulfinyl, 2-ethylbutylsulfinyl, 1,1,2-trimethylpropylsulfinyl, 1,2,2-trimethylpropylsulfinyl, 1-ethyl-1-methylpropylsulfinyl or 1-ethyl-2-methylpropylsulfinyl; [0053] C.sub.1-C.sub.6-haloalkylsulfinyl: a C.sub.1-C.sub.6-alkylsulfinyl radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, fluoromethylsulfinyl, difluoromethylsulfinyl, trifluoromethylsulfinyl, chlorodifluoromethylsulfinyl, bromodifluoromethylsulfinyl, 2-fluoroethylsulfinyl, 2-chloroethylsulfinyl, 2-bromoethylsulfinyl, 2-iodoethylsulfinyl, 2,2-difluoroethylsulfinyl, 2,2,2-trifluoroethylsulfinyl, 2,2,2-trichloroethylsulfinyl, 2-chloro-2-fluoroethylsulfinyl, 2-chloro-2,2-difluoroethylsulfinyl, 2,2-dichloro-2-fluoroethylsulfinyl, pentafluoroethylsulfinyl, 2-fluoropropylsulfinyl, 3-fluoropropylsulfinyl, 2-chloropropylsulfinyl, 3-chloropropylsulfinyl, 2-bromopropylsulfinyl, 3-bromopropylsulfinyl, 2,2-difluoropropylsulfinyl, 2,3-difluoropropylsulfinyl, 2,3-dichloropropylsulfinyl, 3,3,3-trifluoropropylsulfinyl, 3,3,3-trichloropropylsulfinyl, 2,2,3,3,3-pentafluoropropylsulfinyl, heptafluoropropylsulfinyl, 1-(fluoromethyl)-2-fluoroethylsulfinyl, 1-(chloromethyl)-2-chloroethylsulfinyl, 1-(bromomethyl)-2-bromoethylsulfinyl, 4-fluorobutylsulfinyl, 4-chlorobutylsulfinyl, 4-bromobutylsulfinyl, nonafluorobutylsulfinyl, 5-fluoropentylsulfinyl, 5-chloropentylsulfinyl, 5-bromopentylsulfinyl, 5-iodopentylsulfinyl, undecafluoropentylsulfinyl, 6-fluorohexylsulfinyl, 6-chlorohexylsulfinyl, 6-bromohexylsulfinyl, 6-iodohexylsulfinyl or dodecafluorohexylsulfinyl; [0054] C.sub.1-C.sub.6-alkylsulfonyl (C.sub.1-C.sub.6-alkyl-S(.dbd.O).sub.2--), and the alkylsulfonyl radicals of N--(C.sub.1-C.sub.6-alkylsulfonyl)amino and N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino: for example methylsulfonyl, ethylsulfonyl, propylsulfonyl, 1-methylethylsulfonyl, butylsulfonyl, 1-methylpropylsulfonyl, 2-methylpropylsulfonyl, 1,1-dimethylethylsulfonyl, pentylsulfonyl, 1-methylbutylsulfonyl, 2-methylbutylsulfonyl, 3-methylbutylsulfonyl, 1,1-dimethylpropylsulfonyl, 1,2-dimethylpropylsulfonyl, 2,2-dimethylpropylsulfonyl, 1-ethylpropylsulfonyl, hexylsulfonyl, 1-methylpentylsulfonyl, 2-methylpentylsulfonyl, 3-methylpentylsulfonyl, 4-methylpentylsulfonyl, 1,1-dimethylbutylsulfonyl, 1,2-dimethylbutylsulfonyl, 1,3-dimethylbutylsulfonyl, 2,2-dimethylbutylsulfonyl, 2,3-dimethylbutylsulfonyl, 3,3-dimethylbutylsulfonyl, 1-ethylbutylsulfonyl, 2-ethylbutylsulfonyl, 1,1,2-trimethylpropylsulfonyl, 1,2,2-trimethylpropylsulfonyl, 1-ethyl-1-methylpropylsulfonyl or 1-ethyl-2-methylpropylsulfonyl; [0055] C.sub.1-C.sub.6-haloalkylsulfonyl, and the haloalkylsulfonyl radicals of N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino and N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino: a C.sub.1-C.sub.6-alkylsulfonyl radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, fluoromethylsulfonyl, difluoromethylsulfonyl, trifluoromethylsulfonyl, chlorodifluoromethylsulfonyl, bromodifluoromethylsulfonyl, 2-fluoroethylsulfonyl, 2-chloroethylsulfonyl, 2-bromoethylsulfonyl, 2-iodoethylsulfonyl, 2,2-difluoroethylsulfonyl, 2,2,2-trifluoroethylsulfonyl, 2-chloro-2-fluoroethylsulfonyl, 2-chloro-2,2-difluoroethylsulfonyl, 2,2-dichloro-2-fluoroethylsulfonyl, 2,2,2-trichloroethylsulfonyl, pentafluoroethylsulfonyl, 2-fluoropropylsulfonyl, 3-fluoropropylsulfonyl, 2-chloropropylsulfonyl, 3-chloropropylsulfonyl, 2-bromopropylsulfonyl, 3-bromopropylsulfonyl, 2,2-difluoropropylsulfonyl, 2,3-difluoropropylsulfonyl, 2,3-dichloropropylsulfonyl, 3,3,3-trifluoropropylsulfonyl, 3,3,3-trichloropropylsulfonyl, 2,2,3,3,3-pentafluoropropylsulfonyl, heptafluoropropylsulfonyl, 1-(fluoromethyl)-2-fluoroethylsulfonyl, 1-(chloromethyl)-2-chloroethylsulfonyl, 1-(bromomethyl)-2-bromoethylsulfonyl, 4-fluorobutylsulfonyl, 4-chlorobutylsulfonyl, 4-bromobutylsulfonyl, nonafluorobutylsulfonyl, 5-fluoropentylsulfonyl, 5-chloropentylsulfonyl, 5-bromopentylsulfonyl, 5-iodopentylsulfonyl, 6-fluorohexylsulfonyl, 6-bromohexylsulfonyl, 6-iodohexylsulfonyl or dodecafluorohexylsulfonyl; [0056] C.sub.1-C.sub.6-alkylamino, and the alkylamino radicals of N--(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl: for example methylamino, ethylamino, propylamino, 1-methylethylamino, butylamino, 1-methylpropylamino, 2-methylpropylamino, 1,1-dimethylethylamino, pentylamino, 1-methylbutylamino, 2-methylbutylamino, 3-methylbutylamino, 2,2-dimethylpropylamino, 1-ethylpropylamino, hexylamino, 1,1-dimethylpropylamino, 1,2-dimethylpropylamino, 1-methylpentylamino, 2-methylpentylamino, 3-methylpentylamino, 4-methylpentylamino, 1,1-dimethylbutylamino, 1,2-dimethylbutylamino, 1,3-dimethylbutylamino, 2,2-dimethylbutylamino, 2,3-dimethylbutylamino, 3,3-dimethylbutylamino, 1-ethylbutylamino, 2-ethylbutylamino, 1,1,2-trimethylpropylamino, 1,2,2-trimethylpropylamino, 1-ethyl-1-methylpropylamino or 1-ethyl-2-methylpropylamino; [0057] (C.sub.1-C.sub.6-alkylamino)sulfonyl: for example methylaminosulfonyl, ethylaminosulfonyl, propylaminosulfonyl, 1-methylethylaminosulfonyl, butylaminosulfonyl, 1-methylpropylaminosulfonyl, 2-methylpropylaminosulfonyl, 1,1-dimethylethylaminosulfonyl, pentylaminosulfonyl, 1-methylbutylaminosulfonyl, 2-methylbutylaminosulfonyl, 3-methylbutylaminosulfonyl, 2,2-dimethylpropylaminosulfonyl, 1-ethylpropylaminosulfonyl, hexylaminosulfonyl, 1,1-dimethylpropylaminosulfonyl, 1,2-dimethylpropylaminosulfonyl, 1-methylpentylaminosulfonyl, 2-methylpentylaminosulfonyl, 3-methylpentylaminosulfonyl, 4-methylpentylaminosulfonyl, 1,1-dimethylbutylaminosulfonyl, 1,2-dimethylbutylaminosulfonyl, 1,3-dimethylbutylaminosulfonyl, 2,2-dimethylbutylaminosulfonyl, 2,3-dimethylbutylaminosulfonyl, 3,3-dimethylbutylaminosulfonyl, 1-ethylbutylaminosulfonyl, 2-ethylbutylaminosulfonyl, 1,1,2-trimethylpropylaminosulfonyl, 1,2,2-trimethylpropylaminosulfonyl, 1-ethyl-1-methylpropylaminosulfonyl or 1-ethyl-2-methylpropylaminosulfonyl; [0058] di(C.sub.1-C.sub.6-alkyl)aminosulfonyl: for example N,N-dimethylaminosulfonyl, N,N-diethylaminosulfonyl, N,N-di(1-methylethyl)aminosulfonyl, N,N-dipropylaminosulfonyl, N,N-dibutylaminosulfonyl, N,N-di(1-methylpropyl)aminosulfonyl, N,N-di(2-methylpropyl)aminosulfonyl, N,N-di(1,1-dimethylethyl)aminosulfonyl, N-ethyl-N-methylaminosulfonyl, N-methyl-N-propylaminosulfonyl, N-methyl-N-(1-methylethyl)aminosulfonyl, N-butyl-N-methylaminosulfonyl, N-methyl-N-(1-methylpropyl)aminosulfonyl, N-methyl-N-(2-methylpropyl)aminosulfonyl, N-(1,1-dimethylethyl)-N-methylaminosulfonyl, N-ethyl-N-propylaminosulfonyl, N-ethyl-N-(1-methylethyl)aminosulfonyl, N-butyl-N-ethylaminosulfonyl, N-ethyl-N-(1-methylpropyl)aminosulfonyl, N-ethyl-N-(2-methylpropyl)aminosulfonyl, N-ethyl-N-(1,1-dimethylethyl)aminosulfonyl, N-(1-methylethyl)-N-propylaminosulfonyl, N-butyl-N-propylaminosulfonyl, N-(1-methylpropyl)-N-propylaminosulfonyl, N-(2-methylpropyl)-N-propylaminosulfonyl, N-(1,1-dimethylethyl)-N-propylaminosulfonyl, N-butyl-N-(1-methylethyl)aminosulfonyl, N-(1-methylethyl)-N-(1-methylpropyl)aminosulfonyl, N-(1-methylethyl)-N-(2-methylpropyl)aminosulfonyl, N-(1,1-dimethylethyl)-N-(1-methylethyl)aminosulfonyl, N-butyl-N-(1-methylpropyl)aminosulfonyl, N-butyl-N-(2-methylpropyl)aminosulfonyl, N-butyl-N-(1,1-dimethylethyl)aminosulfonyl, N-(1-methylpropyl)-N-(2-methylpropyl)aminosulfonyl, N-(1,1-dimethylethyl)-N-(1-methylpropyl)aminosulfonyl, N-(1,1-dimethylethyl)-N-(2-methylpropyl)aminosulfonyl,

N-methyl-N-pentylaminosulfonyl, N-methyl-N-(1-methylbutyl)aminosulfonyl, N-methyl-N-(2-methylbutyl)aminosulfonyl, N-methyl-N-(3-methylbutyl)aminosulfonyl, N-methyl-N-(2,2-dimethylpropyl)aminosulfonyl, N-methyl-N-(1-ethylpropyl)aminosulfonyl, N-methyl-N-hexylaminosulfonyl, N-methyl-N-(1,1-dimethylpropyl)aminosulfonyl, N-methyl-N-(1,2-dimethylpropyl)aminosulfonyl, N-methyl-N-(1-methylpentyl)aminosulfonyl, N-methyl-N-(2-methylpentyl)aminosulfonyl, N-methyl-N-(3-methylpentyl)aminosulfonyl, N-methyl-N-(4-methylpentyl)aminosulfonyl, N-methyl-N-(1,1-dimethylbutyl)aminosulfonyl, N-methyl-N-(1,2-dimethylbutyl)aminosulfonyl, N-methyl-N-(1,3-dimethylbutyl)aminosulfonyl, N-methyl-N-(2,2-dimethylbutyl)aminosulfonyl, N-methyl-N-(2,3-dimethylbutyl)aminosulfonyl, N-methyl-N-(3,3-dimethylbutyl)aminosulfonyl, N-methyl-N-(1-ethylbutyl)aminosulfonyl, N-methyl-N-(2-ethylbutyl)aminosulfonyl, N-methyl-N-(1,1,2-trimethylpropyl)aminosulfonyl, N-methyl-N-(1,2,2-trimethylpropyl)aminosulfonyl, N-methyl-N-(1-ethyl-1-methylpropyl)aminosulfonyl, N-methyl-N-(1-ethyl-2-methylpropyl)aminosulfonyl, N-ethyl-N-pentylaminosulfonyl, N-ethyl-N-(1-methylbutyl)aminosulfonyl, N-ethyl-N-(2-methylbutyl)aminosulfonyl, N-ethyl-N-(3-methylbutyl)aminosulfonyl, N-ethyl-N-(2,2-dimethylpropyl)aminosulfonyl, N-ethyl-N-(1-ethylpropyl)aminosulfonyl, N-ethyl-N-hexylaminosulfonyl, N-ethyl-N-(1,1-dimethylpropyl)aminosulfonyl, N-ethyl-N-(1,2-dimethylpropyl)aminosulfonyl, N-ethyl-N-(1-methylpentyl)aminosulfonyl, N-ethyl-N-(2-methylpentyl)aminosulfonyl, N-ethyl-N-(3-methylpentyl)aminosulfonyl, N-ethyl-N-(4-methylpentyl)aminosulfonyl, N-ethyl-N-(1,1-dimethylbutyl)aminosulfonyl, N-ethyl-N-(1,2-dimethylbutyl)aminosulfonyl, N-ethyl-N-(1,3-dimethylbutyl)aminosulfonyl, N-ethyl-N-(2,2-dimethylbutyl)aminosulfonyl, N-ethyl-N-(2,3-dimethylbutyl)aminosulfonyl, N-ethyl-N-(3,3-dimethylbutyl)aminosulfonyl, N-ethyl-N-(1-ethylbutyl)aminosulfonyl, N-ethyl-N-(2-ethylbutyl)aminosulfonyl, N-ethyl-N-(1,1,2-trimethylpropyl)aminosulfonyl, N-ethyl-N-(1,2,2-trimethylpropyl)aminosulfonyl, N-ethyl-N-(1-ethyl-1-methylpropyl)aminosulfonyl, N-ethyl-N-(1-ethyl-2-methylpropyl)aminosulfonyl, N-propyl-N-pentylaminosulfonyl, N-butyl-N-pentylaminosulfonyl, N,N-dipentylaminosulfonyl, N-propyl-N-hexylaminosulfonyl, N-butyl-N-hexylaminosulfonyl, N-pentyl-N-hexylaminosulfonyl or N,N-dihexylaminosulfonyl;

[0059] di(C.sub.1-C.sub.4-alkyl)amino, and the dialkylamino radicals of di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl and N-(di-C.sub.1-C.sub.4-alkylamino)imino-C.sub.1-C.sub.6-alkyl: for example N,N-dimethylamino, N,N-diethylamino, N,N-dipropylamino, N,N-di(1-methylethyl)amino, N,N-dibutylamino, N,N-di(1-methylpropyl)amino, N,N-di(2-methylpropyl)amino, N,N-di(1,1-dimethylethyl)amino, N-ethyl-N-methylamino, N-methyl-N-propylamino, N-methyl-N-(1-methylethyl)amino, N-butyl-N-methylamino, N-methyl-N-(1-methylpropyl)amino, N-methyl-N-(2-methylpropyl)amino, N-(1,1-dimethylethyl)-N-methylamino, N-ethyl-N-propylamino, N-ethyl-N-(1-methylethyl)amino, N-butyl-N-ethylamino, N-ethyl-N-(1-methylpropyl)amino, N-ethyl-N-(2-methylpropyl)amino, N-ethyl-N-(1,1-dimethylethyl)amino, N-(1-methylethyl)-N-propylamino, N-butyl-N-propylamino, N-(1-methylpropyl)-N-propylamino, N-(2-methylpropyl)-N-propylamino, N-(1,1-dimethylethyl)-N-propylamino, N-butyl-N-(1-methylethyl)amino, N-(1-methylethyl)-N-(1-methylpropyl)amino, N-(1-methylethyl)-N-(2-methylpropyl)amino, N-(1,1-dimethylethyl)-N-(1-methylethyl)amino, N-butyl-N-(1-methylpropyl)amino, N-butyl-N-(2-methylpropyl)amino, N-butyl-N-(1,1-dimethylethyl)amino, N-(1-methylpropyl)-N-(2-methylpropyl)amino, N-(1,1-dimethylethyl)-N-(1-methylpropyl)amino or N-(1,1-dimethylethyl)-N-(2-methylpropyl)amino; [0060] di(C.sub.1-C.sub.6-alkyl)amino, and the dialkylamino radicals of di(C.sub.1-C.sub.6-alkyl)aminoimino-C.sub.1-C.sub.6-alkyl: di(C.sub.1-C.sub.4-alkyl)amino as mentioned above, and also N,N-dipentylamino, N,N-dihexylamino, N-methyl-N-pentylamino, N-ethyl-N-pentylamino, N-methyl-N-hexylamino or N-ethyl-N-hexylamino; [0061] C.sub.1-C.sub.4-alkylcarbonyl: for example methylcarbonyl, ethylcarbonyl, propylcarbonyl, 1-methylethylcarbonyl, butylcarbonyl, 1-methylpropylcarbonyl, 2-methylpropylcarbonyl or 1,1-dimethylethylcarbonyl; [0062] C.sub.1-C.sub.6-alkylcarbonyl, and the alkylcarbonyl radicals of C.sub.1-C.sub.6-alkylcarbonyl-C.sub.1-C.sub.6-alkyl: C.sub.1-C.sub.4-alkylcarbonyl as mentioned above, and also, for example, pentylcarbonyl, 1-methylbutylcarbonyl, 2-methylbutylcarbonyl, 3-methylbutylcarbonyl, 2,2-dimethylpropylcarbonyl, 1-ethylpropylcarbonyl, hexylcarbonyl, 1,1-dimethylpropylcarbonyl, 1,2-dimethylpropylcarbonyl, 1-methylpentylcarbonyl, 2-methylpentylcarbonyl, 3-methylpentylcarbonyl, 4-methylpentylcarbonyl, 1,1-dimethylbutylcarbonyl, 1,2-dimethylbutylcarbonyl, 1,3-dimethylbutylcarbonyl, 2,2-dimethylbutylcarbonyl, 2,3-dimethylbutylcarbonyl, 3,3-dimethylbutylcarbonyl, 1-ethylbutylcarbonyl, 2-ethylbutylcarbonyl, 1,1,2-trimethylpropylcarbonyl, 1,2,2-trimethylpropylcarbonyl, 1-ethyl-1-methylpropylcarbonyl or 1-ethyl-2-methylpropylcarbonyl; [0063] C.sub.1-C.sub.20-alkylcarbonyl: C.sub.1-C.sub.6-alkylcarbonyl as mentioned above, and also heptylcarbonyl, octylcarbonyl, pentadecylcarbonyl or heptadecylcarbonyl; [0064] C.sub.1-C.sub.4-alkoxycarbonyl, and the alkoxycarbonyl moieties of di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl: for example methoxycarbonyl, ethoxycarbonyl, propoxycarbonyl, 1-methylethoxycarbonyl, butoxycarbonyl, 1-methylpropoxycarbonyl, 2-methylpropoxycarbonyl or 1,1-dimethylethoxycarbonyl; [0065] (C.sub.1-C.sub.6-alkoxy)carbonyl: (C.sub.1-C.sub.4-alkoxy)carbonyl as mentioned above, and also, for example, pentoxycarbonyl, 1-methylbutoxycarbonyl, 2-methylbutoxycarbonyl, 3-methylbutoxycarbonyl, 2,2-dimethylpropoxycarbonyl, 1-ethylpropoxycarbonyl, hexoxycarbonyl, 1,1-dimethylpropoxycarbonyl, 1,2-dimethylpropoxycarbonyl, 1-methylpentoxycarbonyl, 2-methylpentoxycarbonyl, 3-methylpentoxycarbonyl, 4-methylpentoxycarbonyl, 1,1-dimethylbutoxycarbonyl, 1,2-dimethylbutoxycarbonyl, 1,3-dimethylbutoxycarbonyl, 2,2-dimethylbutoxycarbonyl, 2,3-dimethylbutoxycarbonyl, 3,3-dimethylbutoxycarbonyl, 1-ethylbutoxycarbonyl, 2-ethylbutoxycarbonyl, 1,1,2-trimethylpropoxycarbonyl, 1,2,2-trimethylpropoxycarbonyl, 1-ethyl-1-methyl-propoxycarbonyl or 1-ethyl-2-methyl-propoxycarbonyl; [0066] C.sub.1-C.sub.6-haloalkoxycarbonyl: a C.sub.1-C.sub.6-alkoxycarbonyl radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, fluoromethoxycarbonyl, difluoromethoxycarbonyl, trifluoromethoxycarbonyl, chlorodifluoromethoxycarbonyl, bromodifluoromethoxycarbonyl, 2-fluoroethoxycarbonyl, 2-chloroethoxycarbonyl, 2-bromoethoxycarbonyl, 2-iodoethoxycarbonyl, 2,2-difluoroethoxycarbonyl, 2,2,2-trifluoroethoxycarbonyl, 2-chloro-2-fluoroethoxycarbonyl, 2-chloro-2,2-difluoroethoxycarbonyl, 2,2-dichloro-2-fluoroethoxycarbonyl, 2,2,2-trichloroethoxycarbonyl, pentafluoroethoxycarbonyl, 2-fluoropropoxycarbonyl, 3-fluoropropoxycarbonyl, 2-chloropropoxycarbonyl, 3-chloropropoxycarbonyl, 2-bromopropoxycarbonyl, 3-bromopropoxycarbonyl, 2,2-difluoropropoxycarbonyl, 2,3-difluoropropoxycarbonyl, 2,3-dichloropropoxycarbonyl, 3,3,3-trifluoropropoxycarbonyl, 3,3,3-trichloropropoxycarbonyl, 2,2,3,3,3-pentafluoropropoxycarbonyl, heptafluoropropoxycarbonyl, 1-(fluoromethyl)-2-fluoroethoxycarbonyl, 1-(chloromethyl)-2-chloroethoxycarbonyl, 1-(bromomethyl)-2-bromoethoxycarbonyl, 4-fluorobutoxycarbonyl, 4-chlorobutoxycarbonyl, 4-bromobutoxycarbonyl, nonafluorobutoxycarbonyl, 5-fluoropentoxycarbonyl, 5-chloropentoxycarbonyl, 5-bromopentoxycarbonyl, 5-iodopentoxycarbonyl, 6-fluorohexoxycarbonyl, 6-bromohexoxycarbonyl, 6-iodohexoxycarbonyl or dodecafluorohexoxycarbonyl; [0067] (C.sub.1-C.sub.4-alkyl)carbonyloxy: acetyloxy, ethylcarbonyloxy, propylcarbonyloxy, 1-methylethylcarbonyloxy, butylcarbonyloxy, 1-methylpropylcarbonyloxy, 2-methylpropylcarbonyloxy or 1,1-dimethylethylcarbonyloxy; [0068] (C.sub.1-C.sub.4-alkylamino)carbonyl: for example methylaminocarbonyl, ethylaminocarbonyl, propylaminocarbonyl, 1-methylethylaminocarbonyl, butylaminocarbonyl, 1-methylpropylaminocarbonyl, 2-methylpropylaminocarbonyl or 1,1-dimethylethylaminocarbonyl; [0069] (C.sub.1-C.sub.6-alkylamino)carbonyl: (C.sub.1-C.sub.4-alkylamino)carbonyl as mentioned above, and also, for example, pentylaminocarbonyl, 1-methylbutylaminocarbonyl, 2-methylbutylaminocarbonyl, 3-methylbutylaminocarbonyl, 2,2-dimethylpropylaminocarbonyl, 1-ethylpropylaminocarbonyl, hexylaminocarbonyl, 1,1-dimethylpropylaminocarbonyl, 1,2-dimethylpropylaminocarbonyl, 1-methylpentylaminocarbonyl, 2-methylpentylaminocarbonyl, 3-methylpentylaminocarbonyl, 4-methylpentylaminocarbonyl, 1,1-dimethylbutylaminocarbonyl, 1,2-dimethylbutylaminocarbonyl, 1,3-dimethylbutylaminocarbonyl, 2,2-dimethylbutylaminocarbonyl, 2,3-dimethylbutylaminocarbonyl, 3,3-dimethylbutylaminocarbonyl, 1-ethylbutylaminocarbonyl, 2-ethylbutylaminocarbonyl, 1,1,2-trimethylpropylaminocarbonyl, 1,2,2-trimethylpropylaminocarbonyl, 1-ethyl-1-methylpropylaminocarbonyl or 1-ethyl-2-methylpropylaminocarbonyl; [0070] di(C.sub.1-C.sub.4-alkyl)aminocarbonyl: for example N,N-dimethylaminocarbonyl, N,N-diethylaminocarbonyl, N,N-di(1-methylethyl)aminocarbonyl, N,N-dipropylaminocarbonyl, N,N-dibutylaminocarbonyl, N,N-di(1-methylpropyl)aminocarbonyl, N,N-di(2-methylpropyl)aminocarbonyl, N,N-di(1,1-dimethylethyl)aminocarbonyl, N-ethyl-N-methylaminocarbonyl, N-methyl-N-propylaminocarbonyl, N-methyl-N-(1-methylethyl)aminocarbonyl, N-butyl-N-methylaminocarbonyl, N-methyl-N-(1-methylpropyl)aminocarbonyl, N-methyl-N-(2-methylpropyl)aminocarbonyl, N-(1,1-dimethylethyl)-N-methylaminocarbonyl, N-ethyl-N-propylaminocarbonyl, N-ethyl-N-(1-methylethyl)aminocarbonyl, N-butyl-N-ethylaminocarbonyl, N-ethyl-N-(1-methylpropyl)aminocarbonyl, N-ethyl-N-(2-methylpropyl)aminocarbonyl, N-ethyl-N-(1,1-dimethylethyl)aminocarbonyl, N-(1-methylethyl)-N-propylaminocarbonyl, N-butyl-N-propylaminocarbonyl, N-(1-methylpropyl)-N-propylaminocarbonyl, N-(2-methylpropyl)-N-propylaminocarbonyl, N-(1,1-dimethylethyl)-N-propylaminocarbonyl, N-butyl-N-(1-methylethyl)aminocarbonyl, N-(1-methylethyl)-N-(1-methylpropyl)aminocarbonyl, N-(1-methylethyl)-N-(2-methylpropyl)aminocarbonyl, N-(1,1-dimethylethyl)-N-(1-methylethyl)aminocarbonyl, N-butyl-N-(1-methylpropyl)aminocarbonyl, N-butyl-N-(2-methylpropyl)aminocarbonyl, N-butyl-N-(1,1-dimethylethyl)aminocarbonyl, N-(1-methylpropyl)-N-(2-methylpropyl)aminocarbonyl, N-(1,1-dimethylethyl)-N-(1-methylpropyl)aminocarbonyl or N-(1,1-dimethylethyl)-N-(2-methylpropyl)aminocarbonyl; [0071] di(C.sub.1-C.sub.6-alkyl)aminocarbonyl: di(C.sub.1-C.sub.4-alkyl)aminocarbonyl as mentioned above, and also, for example, N-methyl-N-pentylaminocarbonyl, N-methyl-N-(1-methylbutyl)aminocarbonyl, N-Methyl-N-(2-methylbutyl)aminocarbonyl, N-methyl-N-(3-methylbutyl)aminocarbonyl, N-methyl-N-(2,2-dimethylpropyl)aminocarbonyl, N-methyl-N-(1-ethylpropyl)aminocarbonyl, N-methyl-N-hexylaminocarbonyl, N-methyl-N-(1,1-dimethylpropyl)aminocarbonyl, N-methyl-N-(1,2-dimethylpropyl)aminocarbonyl, N-methyl-N-(1-methylpentyl)aminocarbonyl, N-methyl-N-(2-methylpentyl)aminocarbonyl, N-methyl-N-(3-methylpentyl)aminocarbonyl, N-methyl-N-(4-methylpentyl)aminocarbonyl, N-methyl-N-(1,1-dimethylbutyl)aminocarbonyl, N-methyl-N-(1,2-dimethylbutyl)aminocarbonyl, N-methyl-N-(1,3-dimethylbutyl)aminocarbonyl, N-methyl-N-(2,2-dimethylbutyl)aminocarbonyl, N-methyl-N-(2,3-dimethylbutyl)aminocarbonyl, N-methyl-N-(3,3-dimethylbutyl)aminocarbonyl, N-methyl-N-(1-ethylbutyl)aminocarbonyl, N-methyl-N-(2-ethylbutyl)aminocarbonyl, N-methyl-N-(1,1,2-trimethylpropyl)aminocarbonyl, N-methyl-N-(1,2,2-trimethylpropyl)aminocarbonyl, N-methyl-N-(1-ethyl-1-methylpropyl)aminocarbonyl, N-methyl-N-(1-ethyl-2-methylpropyl)aminocarbonyl, N-ethyl-N-pentylaminocarbonyl, N-ethyl-N-(1-methylbutyl)aminocarbonyl, N-ethyl-N-(2-methylbutyl)aminocarbonyl, N-ethyl-N-(3-methylbutyl)aminocarbonyl, N-ethyl-N-(2,2-dimethylpropyl)aminocarbonyl, N-ethyl-N-(1-ethylpropyl)aminocarbonyl, N-ethyl-N-hexylaminocarbonyl, N-ethyl-N-(1,1-dimethylpropyl)aminocarbonyl, N-ethyl-N-(1,2-dimethylpropyl)aminocarbonyl, N-ethyl-N-(1-methylpentyl)aminocarbonyl, N-ethyl-N-(2-methylpentyl)aminocarbonyl, N-ethyl-N-(3-methylpentyl)aminocarbonyl, N-ethyl-N-(4-methylpentyl)aminocarbonyl, N-ethyl-N-(1,1-dimethylbutyl)aminocarbonyl, N-ethyl-N-(1,2-dimethylbutyl)aminocarbonyl, N-ethyl-N-(1,3-dimethylbutyl)aminocarbonyl, N-ethyl-N-(2,2-dimethylbutyl)aminocarbonyl, N-ethyl-N-(2,3-dimethylbutyl)aminocarbonyl, N-ethyl-N-(3,3-dimethylbutyl)aminocarbonyl, N-ethyl-N-(1-ethylbutyl)aminocarbonyl, N-ethyl-N-(2-ethylbutyl)aminocarbonyl, N-ethyl-N-(1,1,2-trimethylpropyl)aminocarbonyl, N-ethyl-N-(1,2,2-trimethylpropyl)aminocarbonyl, N-ethyl-N-(1-ethyl-1-methylpropyl)aminocarbonyl, N-ethyl-N-(1-ethyl-2-methylpropyl)aminocarbonyl, N-propyl-N-pentylaminocarbonyl, N-butyl-N-pentylaminocarbonyl, N,N-dipentylaminocarbonyl, N-propyl-N-hexylaminocarbonyl, N-butyl-N-hexylaminocarbonyl, N-pentyl-N-hexylaminocarbonyl or N,N-dihexylaminocarbonyl; [0072] di(C.sub.1-C.sub.6-alkyl)aminothiocarbonyl: for example N,N-dimethylaminothiocarbonyl, N,N-diethylaminothiocarbonyl, N,N-di(1-methylethyl)aminothiocarbonyl, N,N-dipropylaminothiocarbonyl, N,N-dibutylaminothiocarbonyl, N,N-di(1-methylpropyl)aminothiocarbonyl, N,N-di(2-methylpropyl)aminothiocarbonyl, N,N-di(1,1-dimethylethyl)aminothiocarbonyl, N-ethyl-N-methylaminothiocarbonyl, N-methyl-N-propylaminothiocarbonyl, N-methyl-N-(1-methylethyl)aminothiocarbonyl, N-butyl-N-methylaminothiocarbonyl, N-methyl-N-(1-methylpropyl)aminothiocarbonyl, N-methyl-N-(2-methylpropyl)aminothiocarbonyl, N-(1,1-dimethylethyl)-N-methylaminothiocarbonyl, N-ethyl-N-propylaminothiocarbonyl, N-ethyl-N-(1-methylethyl)aminothiocarbonyl, N-butyl-N-ethylaminothiocarbonyl, N-ethyl-N-(1-methylpropyl)aminothiocarbonyl, N-ethyl-N-(2-methylpropyl)aminothiocarbonyl, N-ethyl-N-(1,1-dimethylethyl)aminothiocarbonyl, N-(1-methylethyl)-N-propylaminothiocarbonyl, N-butyl-N-propylaminothiocarbonyl, N-(1-methylpropyl)-N-propylaminothiocarbonyl, N-(2-methylpropyl)-N-propylaminothiocarbonyl, N-(1,1-dimethylethyl)-N-propylaminothiocarbonyl, N-butyl-N-(1-methylethyl)aminothiocarbonyl, N-(1-methylethyl)-N-(1-methylpropyl)aminothiocarbonyl, N-(1-methylethyl)-N-(2-methylpropyl)aminothiocarbonyl, N-(1,1-dimethylethyl)-N-(1-methylethyl)aminothiocarbonyl, N-butyl-N-(1-methylpropyl)aminothiocarbonyl, N-butyl-N-(2-methylpropyl)aminothiocarbonyl, N-butyl-N-(1,1-dimethylethyl)aminothiocarbonyl, N-(1-methylpropyl)-N-(2-methylpropyl)aminothiocarbonyl, N-(1,1-dimethylethyl)-N-(1-methylpropyl)aminothiocarbonyl, N-(1,1-dimethylethyl)-N-(2-methylpropyl)aminothiocarbonyl, N-methyl-N-pentylaminothiocarbonyl, N-methyl-N-(1-methylbutyl)aminothiocarbonyl, N-methyl-N-(2-methylbutyl)aminothiocarbonyl, N-methyl-N-(3-methylbutyl)aminothiocarbonyl, N-methyl-N-(2,2-dimethylpropyl)aminothiocarbonyl, N-methyl-N-(1-ethylpropyl)aminothiocarbonyl, N-methyl-N-hexylaminothiocarbonyl, N-methyl-N-(1,1-dimethylpropyl)aminothiocarbonyl, N-methyl-N-(1,2-dimethylpropyl)aminothiocarbonyl, N-methyl-N-(1-methylpentyl)aminothiocarbonyl, N-methyl-N-(2-methylpentyl)aminothiocarbonyl, N-methyl-N-(3-methylpentyl)aminothiocarbonyl, N-methyl-N-(4-methylpentyl)aminothiocarbonyl, N-methyl-N-(1,1-dimethylbutyl)aminothiocarbonyl, N-methyl-N-(1,2-dimethylbutyl)aminothiocarbonyl, N-methyl-N-(1,3-dimethylbutyl)aminothiocarbonyl, N-methyl-N-(2,2-dimethylbutyl)aminothiocarbonyl, N-methyl-N-(2,3-dimethylbutyl)aminothiocarbonyl, N-methyl-N-(3,3-dimethylbutyl)aminothiocarbonyl, N-methyl-N-(1-ethylbutyl)aminothiocarbonyl, N-methyl-N-(2-ethylbutyl)aminothiocarbonyl, N-methyl-N-ethyl-N-(1,1,2-trimethylpropyl)aminothiocarbonyl, N-methyl-N-(1,2,2-trimethylpropyl)aminothiocarbonyl,

N-methyl-N-(1-ethyl-1-methylpropyl)aminothiocarbonyl, N-methyl-N-(1-ethyl-2-methylpropyl)aminothiocarbonyl, N-ethyl-N-pentylaminothiocarbonyl, N-ethyl-N-(1-methylbutyl)aminothiocarbonyl, N-ethyl-N-(2-methylbutyl)aminothiocarbonyl, N-ethyl-N-(3-methylbutyl)aminothiocarbonyl, N-ethyl-N-(2,2-dimethylpropyl)aminothiocarbonyl, N-ethyl-N-(1-ethylpropyl)aminothiocarbonyl, N-ethyl-N-hexylaminothiocarbonyl, N-ethyl-N-(1,1-dimethylpropyl)aminothiocarbonyl, N-ethyl-N-(1,2-dimethylpropyl)aminothiocarbonyl, N-ethyl-N-(1-methylpentyl)aminothiocarbonyl, N-ethyl-N-(2-methylpentyl)aminothiocarbonyl, N-ethyl-N-(3-methylpentyl)aminothiocarbonyl, N-ethyl-N-(4-methylpentyl)aminothiocarbonyl, N-ethyl-N-(1,1-dimethylbutyl)aminothiocarbonyl, N-ethyl-N-(1,2-dimethylbutyl)aminothiocarbonyl, N-ethyl-N-(1,3-dimethylbutyl)aminothiocarbonyl, N-ethyl-N-(2,2-dimethylbutyl)aminothiocarbonyl, N-ethyl-N-(2,3-dimethylbutyl)aminothiocarbonyl, N-ethyl-N-(3,3-dimethylbutyl)aminothiocarbonyl, N-ethyl-N-(1-ethylbutyl)aminothiocarbonyl, N-ethyl-N-(2-ethylbutyl)aminothiocarbonyl, N-ethyl-N-(1,1,2-trimethylpropyl)aminothiocarbonyl, N-ethyl-N-(1,2,2-trimethylpropyl)aminothiocarbonyl, N-ethyl-N-(1-ethyl-1-methylpropyl)aminothiocarbonyl, N-ethyl-N-(1-ethyl-2-methylpropyl)aminothiocarbonyl, N-propyl-N-pentylaminothiocarbonyl, N-butyl-N-pentylaminothiocarbonyl, N,N-dipentylaminothiocarbonyl, N-propyl-N-hexylaminothiocarbonyl, N-butyl-N-hexylaminothiocarbonyl, N-pentyl-N-hexylaminothiocarbonyl or N,N-dihexylaminothiocarbonyl;

[0073] C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkyl and the alkoxyalkyl moieties of hydroxy-C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkyl: C.sub.1-C.sub.4-alkyl which is substituted by C.sub.1-C.sub.4-alkoxy as mentioned above, i.e., for example, methoxymethyl, ethoxymethyl, propoxymethyl, (1-methylethoxy)methyl, butoxymethyl, (1-methylpropoxy)methyl, (2-methylpropoxy)methyl, (1,1-dimethylethoxy)methyl, 2-(methoxy)ethyl, 2-(ethoxy)ethyl, 2-(propoxy)ethyl, 2-(1-methylethoxy)ethyl, 2-(butoxy)ethyl, 2-(1-methylpropoxy)ethyl, 2-(2-methylpropoxy)ethyl, 2-(1,1-dimethylethoxy)ethyl, 2-(methoxy)propyl, 2-(ethoxy)propyl, 2-(propoxy)propyl, 2-(1-methylethoxy)propyl, 2-(butoxy)propyl, 2-(1-methylpropoxy)propyl, 2-(2-methylpropoxy)propyl, 2-(1,1-dimethylethoxy)propyl, 3-(methoxy)propyl, 3-(ethoxy)propyl, 3-(propoxy)propyl, 3-(1-methylethoxy)propyl, 3-(butoxy)propyl, 3-(1-methylpropoxy)propyl, 3-(2-methylpropoxy)propyl, 3-(1,1-dimethylethoxy)propyl, 2-(methoxy)butyl, 2-(ethoxy)butyl, 2-(propoxy)butyl, 2-(1-methylethoxy)butyl, 2-(butoxy)butyl, 2-(1-methylpropoxy)butyl, 2-(2-methylpropoxy)butyl, 2-(1,1-dimethylethoxy)butyl, 3-(methoxy)butyl, 3-(ethoxy)butyl, 3-(propoxy)butyl, 3-(1-methylethoxy)butyl, 3-(butoxy)butyl, 3-(1-methylpropoxy)butyl, 3-(2-methylpropoxy)butyl, 3-(1,1-dimethylethoxy)butyl, 4-(methoxy)butyl, 4-(ethoxy)butyl, 4-(propoxy)butyl, 4-(1-methylethoxy)butyl, 4-(butoxy)butyl, 4-(1-methylpropoxy)butyl, 4-(2-methylpropoxy)butyl or 4-(1,1-dimethylethoxy)butyl; [0074] C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxy as alkoxyalkoxy moieties of C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxycarbonyl: C.sub.1-C.sub.4-alkoxy which is substituted by C.sub.1-C.sub.4-alkoxy as mentioned above, i.e., for example, methoxymethoxy, ethoxymethoxy, propoxymethoxy, (1-methylethoxy)methoxy, butoxymethoxy, (1-methylpropoxy)methoxy, (2-methylpropoxy)methoxy, (1,1-dimethylethoxy)methoxy, 2-(methoxy)ethoxy, 2-(ethoxy)ethoxy, 2-(propoxy)ethoxy, 2-(1-methylethoxy)ethoxy, 2-(butoxy)ethoxy, 2-(1-methylpropoxy)ethoxy, 2-(2-methylpropoxy)ethoxy, 2-(1,1-dimethylethoxy)ethoxy, 2-(methoxy)propoxy, 2-(ethoxy)propoxy, 2-(propoxy)propoxy, 2-(1-methylethoxy)propoxy, 2-(butoxy)propoxy, 2-(1-methylpropoxy)propoxy, 2-(2-methylpropoxy)propoxy, 2-(1,1-dimethylethoxy)propoxy, 3-(methoxy)propoxy, 3-(ethoxy)propoxy, 3-(propoxy)propoxy, 3-(1-methylethoxy)propoxy, 3-(butoxy)propoxy, 3-(1-methylpropoxy)propoxy, 3-(2-methylpropoxy)propoxy, 3-(1,1-dimethylethoxy)propoxy, 2-(methoxy)butoxy, 2-(ethoxy)butoxy, 2-(propoxy)butoxy, 2-(1-methylethoxy)butoxy, 2-(butoxy)butoxy, 2-(1-methylpropoxy)butoxy, 2-(2-methylpropoxy)butoxy, 2-(1,1-dimethylethoxy)butoxy, 3-(methoxy)butoxy, 3-(ethoxy)butoxy, 3-(propoxy)butoxy, 3-(1-methylethoxy)butoxy, 3-(butoxy)butoxy, 3-(1-methylpropoxy)butoxy, 3-(2-methylpropoxy)butoxy, 3-(1,1-dimethylethoxy)butoxy, 4-(methoxy)butoxy, 4-(ethoxy)butoxy, 4-(propoxy)butoxy, 4-(1-methylethoxy)butoxy, 4-(butoxy)butoxy, 4-(1-methylpropoxy)butoxy, 4-(2-methylpropoxy)butoxy or 4-(1,1-dimethylethoxy)butoxy; [0075] C.sub.3-C.sub.6-alkenyl, and the alkenyl moieties of C.sub.3-C.sub.6-alkenylcarbonyl, C.sub.3-C.sub.6-alkenyloxy, C.sub.3-C.sub.6-alkenyloxycarbonyl, C.sub.3-C.sub.6-alkenylaminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl: for example prop-2-en-1-yl, but-1-en-4-yl, 1-methylprop-2-en-1-yl, 2-methylprop-2-en-1-yl, 2-buten-1-yl, 1-penten-3-yl, 1-penten-4-yl, 2-penten-4-yl, 1-methylbut-2-en-1-yl, 2-methylbut-2-en-1-yl, 3-methylbut-2-en-1-yl, 1-methylbut-3-en-1-yl, 2-methylbut-3-en-1-yl, 3-methylbut-3-en-1-yl, 1,1-dimethylprop-2-en-1-yl, 1,2-dimethylprop-2-en-1-yl, 1-ethylprop-2-en-1-yl, hex-3-en-1-yl, hex-4-en-1-yl, hex-5-en-1-yl, 1-methylpent-3-en-1-yl, 2-methylpent-3-en-1-yl, 3-methylpent-3-en-1-yl, 4-methylpent-3-en-1-yl, 1-methylpent-4-en-1-yl, 2-methylpent-4-en-1-yl, 3-methylpent-4-en-1-yl, 4-methylpent-4-en-1-yl, 1,1-dimethylbut-2-en-1-yl, 1,1-dimethylbut-3-en-1-yl, 1,2-dimethylbut-2-en-1-yl, 1,2-dimethylbut-3-en-1-yl, 1,3-dimethylbut-2-en-1-yl, 1,3-dimethylbut-3-en-1-yl, 2,2-dimethylbut-3-en-1-yl, 2,3-dimethylbut-2-en-1-yl, 2,3-dimethylbut-3-en-1-yl, 3,3-dimethylbut-2-en-1-yl, 1-ethylbut-2-en-1-yl, 1-ethylbut-3-en-1-yl, 2-ethylbut-2-en-1-yl, 2-ethylbut-3-en-1-yl, 1,1,2-trimethylprop-2-en-1-yl, 1-ethyl-1-methylprop-2-en-1-yl or 1-ethyl-2-methylprop-2-en-1-yl; [0076] C.sub.2-C.sub.6-alkenyl, and the alkenyl moieties of C.sub.2-C.sub.6-alkenylcarbonyl, phenyl-C.sub.2-C.sub.6-alkenylcarbonyl and heterocyclyl-C.sub.2-C.sub.6-alkenylcarbonyl: C.sub.3-C.sub.6-alkenyl as mentioned above, and also ethenyl; [0077] C.sub.2-C.sub.20-alkenyl as alkenyl moiety of C.sub.2-C.sub.20-alkenylcarbonyl: C.sub.2-C.sub.6-alkenyl as mentioned above, and also pentadecenyl or heptadecenyl; [0078] C.sub.3-C.sub.6-haloalkenyl: a C.sub.3-C.sub.6-alkenyl radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, 2-chloroallyl, 3-chloroallyl, 2,3-dichloroallyl, 3,3-dichloroallyl, 2,3,3-trichloroallyl, 2,3-dichlorobut-2-phenyl, 2-bromoallyl, 3-bromoallyl, 2,3-dibromoallyl, 3,3-dibromoallyl, 2,3,3-tribromoallyl or 2,3-dibromobut-2-enyl; [0079] C.sub.3-C.sub.6-alkynyl, and the alkynyl moieties of C.sub.3-C.sub.6-alkynylcarbonyl, C.sub.3-C.sub.6-alkynyloxy, C.sub.3-C.sub.6-alkynyloxycarbonyl, C.sub.3-C.sub.6-alkynylaminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkoxyamino)carbonyl: for example propargyl, but-1-yn-3-yl, but-1-yn-4-yl, but-2-yn-1-yl, pent-1-yn-3-yl, pent-1-yn-4-yl, pent-1-yn-5-yl, pent-2-yn-1-yl, pent-2-yn-4-yl, pent-2-yn-5-yl, 3-methylbut-1-yn-3-yl, 3-methylbut-1-yn-4-yl, hex-1-yn-3-yl, hex-1-yn-4-yl, hex-1-yn-5-yl, hex-1-yn-6-yl, hex-2-yn-1-yl, hex-2-yn-4-yl, hex-2-yn-5-yl, hex-2-yn-6-yl, hex-3-yn-1-yl, hex-3-yn-2-yl, 3-methylpent-1-yn-3-yl, 3-methylpent-1-yn-4-yl, 3-methylpent-1-yn-5-yl, 4-methylpent-2-yn-4-yl or 4-methylpent-2-yn-5-yl; [0080] C.sub.2-C.sub.6-alkynyl, and the alkynyl moieties of C.sub.2-C.sub.6-alkynylcarbonyl: C.sub.3-C.sub.6-alkynyl as mentioned above, and also ethynyl; [0081] C.sub.3-C.sub.6-haloalkynyl: a C.sub.3-C.sub.6-alkynyl radical as mentioned above which is partially or fully substituted by fluorine, chlorine, bromine and/or iodine, i.e., for example, 1,1-difluoroprop-2-yn-1-yl, 3-iodoprop-2-yn-1-yl, 4-fluorobut-2-yn-1-yl, 4-chlorobut-2-yn-1-yl, 1,1-difluorobut-2-yn-1-yl, 4-iodobut-3-yn-1-yl, 5-fluoropent-3-yn-1-yl, 5-iodopent-4-yn-1-yl, 6-fluorohex-4-yn-1-yl or 6-iodohex-5-yn-1-yl; [0082] C.sub.3-C.sub.6-cycloalkyl, and the cycloalkyl moieties of C.sub.3-C.sub.6-cycloalkylcarbonyl: for example cyclopropyl, cyclobutyl, cyclopentyl or cyclohexyl; [0083] heterocyclyl, and the heterocyclyl moieties of heterocyclyloxy, heterocyclylcarbonyl, heterocyclyl-C.sub.1-C.sub.6-alkyl, heterocyclyloxycarbonyl, heterocyclyloxythiocarbonyl, heterocyclyl-C.sub.2-C.sub.6-alkenylcarbonyl, heterocyclylcarbonyl-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkyl)-N-(heterocyclyl)aminocarbonyl, heterocyclylaminocarbonyl: a saturated, partially saturated or unsaturated 5- or 6-membered heterocyclic ring which is attached via carbon and contains one to four identical or different heteroatoms selected from the following group: oxygen, sulfur and nitrogen, i.e., for example, 5-membered rings having, for example, one heteroatom, having two heteroatoms, having three heteroatoms or having four heteroatoms or, for example, 6-membered rings having, for example, one heteroatom, having two heteroatoms, having three heteroatoms or having four heteroatoms, i.e. 5-membered rings having one heteroatom, such as: [0084] tetrahydrofuran-2-yl, tetrahydrofuran-3-yl, tetrahydrothien-2-yl, tetrahydrothien-3-yl, tetrahydropyrrol-2-yl, tetrahydropyrrol-3-yl, 2,3-dihydrofuran-2-yl, 2,3-dihydrofuran-3-yl, 2,5-dihydrofuran-2-yl, 2,5-dihydrofuran-3-yl, 4,5-dihydrofuran-2-yl, 4,5-dihydrofuran-3-yl, 2,3-dihydrothien-2-yl, 2,3-dihydrothien-3-yl, 2,5-dihydrothien-2-yl, 2,5-dihydrothien-3-yl, 4,5-dihydrothien-2-yl, 4,5-dihydrothien-3-yl, 2,3-dihydro-1H-pyrrol-2-yl, 2,3-dihydro-1H-pyrrol-3-yl, 2,5-dihydro-1H-pyrrol-2-yl, 2,5-dihydro-1H-pyrrol-3-yl, 4,5-dihydro-1H-pyrrol-2-yl, 4,5-dihydro-1H-pyrrol-3-yl, 3,4-dihydro-2H-pyrrol-2-yl, 3,4-dihydro-2H-pyrrol-3-yl, 3,4-dihydro-5H-pyrrol-2-yl, 3,4-dihydro-5H-pyrrol-3-yl, 2-furyl, 3-furyl, 2-thienyl, 3-thienyl, pyrrol-2-yl or pyrrol-3-yl; [0085] 5-membered rings having two heteroatoms such as: tetrahydropyrazol-3-yl, tetrahydropyrazol-4-yl, tetrahydroisoxazol-3-yl, tetrahydroisoxazol-4-yl, tetrahydroisoxazol-5-yl, 1,2-oxathiolan-3-yl, 1,2-oxathiolan-4-yl, 1,2-oxathiolan-5-yl, tetrahydroisothiazol-3-yl, tetrahydroisothiazol-4-yl, tetrahydroisothiazol-5-yl, 1,2-dithiolan-3-yl, 1,2-dithiolan-4-yl, tetrahydroimidazol-2-yl, tetrahydroimidazol-4-yl, tetrahydrooxazol-2-yl, tetrahydrooxazol-4-yl, tetrahydrooxazol-5-yl, tetrahydrothiazol-2-yl, tetrahydrothiazol-4-yl, tetrahydrothiazol-5-yl, 1,3-dioxolan-2-yl, 1,3-dioxolan-4-yl, 1,3-oxathiolan-2-yl, 1,3-oxathiolan-4-yl, 1,3-oxathiolan-5-yl, 1,3-dithiolan-2-yl, 1,3-dithiolan-4-yl, 4,5-dihydro-1H-pyrazol-3-yl, 4,5-dihydro-1H-pyrazol-4-yl, 4,5-dihydro-1H-pyrazol-5-yl, 2,5-dihydro-1H-pyrazol-3-yl, 2,5-dihydro-1H-pyrazol-4-yl, 2,5-dihydro-1H-pyrazol-5-yl, 4,5-dihydroisoxazol-3-yl, 4,5-dihydroisoxazol-4-yl, 4,5-dihydroisoxazol-5-yl, 2,5-dihydroisoxazol-3-yl, 2,5-dihydroisoxazol-4-yl, 2,5-dihydroisoxazol-5-yl, 2,3-dihydroisoxazol-3-yl, 2,3-dihydroisoxazol-4-yl, 2,3-dihydroisoxazol-5-yl, 4,5-dihydroisothiazol-3-yl, 4,5-dihydroisothiazol-4-yl, 4,5-dihydroisothiazol-5-yl, 2,5-dihydroisothiazol-3-yl, 2,5-dihydroisothiazol-4-yl, 2,5-dihydroisothiazol-5-yl, 2,3-dihydroisothiazol-3-yl, 2,3-dihydroisothiazol-4-yl, 2,3-dihydroisothiazol-5-yl, .DELTA..sup.3-1,2-dithiol-3-yl, .DELTA..sup.3-1,2-dithiol-4-yl, .DELTA..sup.3-1,2-dithiol-5-yl, 4,5-dihydro-1H-imidazol-2-yl, 4,5-dihydro-1H-imidazol-4-yl, 4,5-dihydro-1H-imidazol-5-yl, 2,5-dihydro-1H-imidazol-2-yl, 2,5-dihydro-1H-imidazol-4-yl, 2,5-dihydro-1H-imidazol-5-yl, 2,3-dihydro-1H-imidazol-2-yl, 2,3-dihydro-1H-imidazol-4-yl, 4,5-dihydrooxazol-2-yl, 4,5-dihydrooxazol-4-yl, 4,5-dihydrooxazol-5-yl, 2,5-dihydrooxazol-2-yl, 2,5-dihydrooxazol-4-yl, 2,5-dihydrooxazol-5-yl, 2,3-dihydrooxazol-2-yl, 2,3-dihydrooxazol-4-yl, 2,3-dihydrooxazol-5-yl, 4,5-dihydrothiazol-2-yl, 4,5-dihydrothiazol-4-yl, 4,5-dihydrothiazol-5-yl, 2,5-dihydrothiazol-2-yl, 2,5-dihydrothiazol-4-yl, 2,5-dihydrothiazol-5-yl, 2,3-dihydrothiazol-2-yl, 2,3-dihydrothiazol-4-yl, 2,3-dihydrothiazol-5-yl, 1,3-dioxol-2-yl, 1,3-dioxol-4-yl, 1,3-dithiol-2-yl, 1,3-dithiol-4-yl, 1,3-oxathiol-2-yl, 1,3-oxathiol-4-yl, 1,3-oxathiol-5-yl, pyrazol-3-yl, pyrazol-4-yl, isoxazol-3-yl, isoxazol-4-yl, isoxazol-5-yl, isothiazol-3-yl, isothiazol-4-yl, isothiazol-5-yl, imidazol-2-yl, imidazol-4-yl, oxazol-2-yl, oxazol-4-yl, oxazol-5-yl, thiazol-2-yl, thiazol-4-yl or thiazol-5-yl; [0086] 5-membered rings having three heteroatoms such as: 1,2,3-.DELTA..sup.2-oxadiazolin-4-yl, 1,2,3-.DELTA..sup.2-oxadiazolin-5-yl, 1,2,4-.DELTA..sup.4-oxadiazolin-3-yl, 1,2,4-.DELTA..sup.4-oxadiazolin-5-yl, 1,2,4-.DELTA..sup.2-oxadiazolin-3-yl, 1,2,4-.DELTA..sup.2-oxadiazolin-5-yl, 1,2,4-.DELTA..sup.3-oxadiazolin-3-yl, 1,2,4-.DELTA..sup.3-oxadiazolin-5-yl, 1,3,4-.DELTA..sup.2-oxadiazolin-2-yl, 1,3,4-.DELTA..sup.2-oxadiazolin-5-yl, 1,3,4-.DELTA..sup.3-oxadiazolin-2-yl, 1,3,4-oxadiazolin-2-yl, 1,2,3-.DELTA..sup.2-thiadiazolin-4-yl, 1,2,3-.DELTA..sup.2-thiadiazolin-5-yl, 1,2,4-.DELTA..sup.4-thiadiazolin-3-yl, 1,2,4-.DELTA..sup.4-thiadiazolin-5-yl, 1,2,4-.DELTA..sup.3-thiadiazolin-3-yl, 1,2,4-.DELTA..sup.3-thiadiazolin-5-yl, 1,2,4-.DELTA..sup.2-thiadiazolin-3-yl, 1,2,4-.DELTA..sup.2-thiadiazolin-5-yl, 1,3,4-.DELTA..sup.2-thiadiazolin-2-yl, 1,3,4-.DELTA..sup.2-thiadiazolin-5-yl, 1,3,4-.DELTA..sup.3-thiadiazolin-2-yl, 1,3,4-thiadiazolin-2-yl, 1,3,2-dioxathiolan-4-yl, 1,2,3-.DELTA..sup.2-triazolin-4-yl, 1,2,3-.DELTA..sup.2-triazolin-5-yl, 1,2,4-.DELTA..sup.2-triazolin-3-yl, 1,2,4-.DELTA..sup.2-triazolin-5-yl, 1,2,4-.DELTA..sup.3-triazolin-3-yl, 1,2,4-.DELTA..sup.3-triazolin-5-yl, 1,2,4-.DELTA..sup.1-triazolin-2-yl, 1,2,4-triazolin-3-yl, 3H-1,2,4-dithiazol-5-yl, 2H-1,3,4-dithiazol-5-yl, 2H-1,3,4-oxathiazol-5-yl, 1,2,3-oxadiazol-4-yl, 1,2,3-oxadiazol-5-yl, 1,2,4-oxadiazol-3-yl, 1,2,4,-oxadiazol-5-yl, 1,3,4-oxadiazol-2-yl, 1,2,3-thiadiazol-4-yl, 1,2,3-thiadiazol-5-yl, 1,2,4-thiadiazol-3-yl, 1,2,4-thiadiazol-5-yl, 1,3,4-thiadiazolyl-2-yl, 1,2,3-triazol-4-yl or 1,2,4-triazol-3-yl; [0087] 5-membered rings having four heteroatoms such as: tetrazol-5-yl; [0088] 6-membered rings having one heteroatom such as: tetrahydropyran-2-yl, tetrahydropyran-3-yl, tetrahydropyran-4-yl, piperidin-2-yl, piperidin-3-yl, piperidin-4-yl, tetrahydrothiopyran-2-yl, tetrahydrothiopyran-3-yl, tetrahydrothiopyran-4-yl, 2H-3,4-dihydropyran-6-yl, 2H-3,4-dihydropyran-5-yl, 2H-3,4-dihydropyran-4-yl, 2H-3,4-dihydropyran-3-yl, 2H-3,4-dihydropyran-2-yl, 2H-3,4-dihydropyran-6-yl, 2H-3,4-dihydrothiopyran-5-yl, 2H-3,4-dihydrothiopyran-4-yl, 2H-3,4-dihydropyran-3-yl, 2H-3,4-dihydropyran-2-yl, 1,2,3,4-tetrahydropyridin-6-yl, 1,2,3,4-tetrahydropyridin-5-yl, 1,2,3,4-tetrahydropyridin-4-yl, 1,2,3,4-tetrahydropyridin-3-yl, 1,2,3,4-tetrahydropyridin-2-yl, 2H-5,6-dihydropyran-2-yl, 2H-5,6-dihydropyran-3-yl, 2H-5,6-dihydropyran-4-yl, 2H-5,6-dihydropyran-5-yl, 2H-5,6-dihydropyran-6-yl, 2H-5,6-dihydrothiopyran-2-yl, 2H-5,6-dihydrothiopyran-3-yl, 2H-5,6-dihydrothiopyran-4-yl, 2H-5,6-dihydrothiopyran-5-yl, 2H-5,6-dihydrothiopyran-6-yl, 1,2,5,6-tetrahydropyridin-2-yl, 1,2,5,6-tetrahydropyridin-3-yl, 1,2,5,6-tetrahydropyridin-4-yl, 1,2,5,6-tetrahydropyridin-5-yl, 1,2,5,6-tetrahydropyridin-6-yl, 2,3,4,5-tetrahydropyridin-2-yl, 2,3,4,5-tetrahydropyridin-3-yl, 2,3,4,5-tetrahydropyridin-4-yl, 2,3,4,5-tetrahydropyridin-5-yl, 2,3,4,5-tetrahydropyridin-6-yl, 4H-pyran-2-yl, 4H-pyran-3-yl, 4H-pyran-4-yl, 4H-thiopyran-2-yl, 4H-thiopyran-3-yl, 4H-thiopyran-4-yl, 1,4-dihydropyridin-2-yl, 1,4-dihydropyridin-3-yl, 1,4-dihydropyridin-4-yl, 2H-pyran-2-yl, 2H-pyran-3-yl, 2H-pyran-4-yl, 2H-pyran-5-yl, 2H-pyran-6-yl, 2H-thiopyran-2-yl, 2H-thiopyran-3-yl, 2H-thiopyran-4-yl, 2H-thiopyran-5-yl, 2H-thiopyran-6-yl, 1,2-dihydropyridin-2-yl, 1,2-dihydropyridin-3-yl, 1,2-dihydropyridin-4-yl, 1,2-dihydropyridin-5-yl, 1,2-dihydropyridin-6-yl, 3,4-dihydropyridin-2-yl, 3,4-dihydropyridin-3-yl, 3,4-dihydropyridin-4-yl, 3,4-dihydropyridin-5-yl, 3,4-dihydropyridin-6-yl, 2,5-dihydropyridin-2-yl, 2,5-dihydropyridin-3-yl, 2,5-dihydropyridin-4-yl, 2,5-dihydropyridin-5-yl, 2,5-dihydropyridin-6-yl, 2,3-dihydropyridin-2-yl, 2,3-dihydropyridin-3-yl, 2,3-dihydropyridin-4-yl, 2,3-dihydropyridin-5-yl, 2,3-dihydropyridin-6-yl, pyridin-2-yl, pyridin-3-yl or pyridin-4-yl; [0089] 6-membered rings having two heteroatoms such as: 1,3-dioxan-2-yl, 1,3-dioxan-4-yl, 1,3-dioxan-5-yl, 1,4-dioxan-2-yl, 1,3-dithian-2-yl,

1,3-dithian-4-yl, 1,3-dithian-5-yl, 1,4-dithian-2-yl, 1,3-oxathian-2-yl, 1,3-oxathian-4-yl, 1,3-oxathian-5-yl, 1,3-oxathian-6-yl, 1,4-oxathian-2-yl, 1,4-oxathian-3-yl, 1,2-dithian-3-yl, 1,2-dithian-4-yl, hexahydropyrimidin-2-yl, hexahydropyrimidin-4-yl, hexahydropyrimidin-5-yl, hexahydropyrazin-2-yl, hexahydropyridazin-3-yl, hexahydropyridazin-4-yl, tetrahydro-1,3-oxazin-2-yl, tetrahydro-1,3-oxazin-4-yl, tetrahydro-1,3-oxazin-5-yl, tetrahydro-1,3-oxazin-6-yl, tetrahydro-1,3-thiazin-2-yl, tetrahydro-1,3-thiazin-4-yl, tetrahydro-1,3-thiazin-5-yl, tetrahydro-1,3-thiazin-6-yl, tetrahydro-1,4-thiazin-2-yl, tetrahydro-1,4-thiazin-3-yl, tetrahydro-1,4-oxazin-2-yl, tetrahydro-1,4-oxazin-3-yl, tetrahydro-1,2-oxazin-3-yl, tetrahydro-1,2-oxazin-4-yl, tetrahydro-1,2-oxazin-5-yl, tetrahydro-1,2-oxazin-6-yl, 2H-5,6-dihydro-1,2-oxazin-3-yl, 2H-5,6-dihydro-1,2-oxazin-4-yl, 2H-5,6-dihydro-1,2-oxazin-5-yl, 2H-5,6-dihydro-1,2-oxazin-6-yl, 2H-5,6-dihydro-1,2-thiazin-3-yl, 2H-5,6-dihydro-1,2-thiazin-4-yl, 2H-5,6-dihydro-1,2-thiazin-5-yl, 2H-5,6-dihydro-1,2-thiazin-6-yl, 4H-5,6-dihydro-1,2-oxazin-3-yl, 4H-5,6-dihydro-1,2-oxazin-4-yl, 4H-5,6-dihydro-1,2-oxazin-5-yl, 4H-5,6-dihydro-1,2-oxazin-6-yl, 4H-5,6-dihydro-1,2-thiazin-3-yl, 4H-5,6-dihydro-1,2-thiazin-4-yl, 4H-5,6-dihydro-1,2-thiazin-5-yl, 4H-5,6-dihydro-1,2-thiazin-6-yl, 2H-3,6-dihydro-1,2-oxazin-3-yl, 2H-3,6-dihydro-1,2-oxazin-4-yl, 2H-3,6-dihydro-1,2-oxazin-5-yl, 2H-3,6-dihydro-1,2-oxazin-6-yl, 2H-3,6-dihydro-1,2-thiazin-3-yl, 2H-3,6-dihydro-1,2-thiazin-4-yl, 2H-3,6-dihydro-1,2-thiazin-5-yl, 2H-3,6-dihydro-1,2-thiazin-6-yl, 2H-3,4-dihydro-1,2-oxazin-3-yl, 2H-3,4-dihydro-1,2-oxazin-4-yl, 2H-3,4-dihydro-1,2-oxazin-5-yl, 2H-3,4-dihydro-1,2-oxazin-6-yl, 2H-3,4-dihydro-1,2-thiazin-3-yl, 2H-3,4-dihydro-1,2-thiazin-4-yl, 2H-3,4-dihydro-1,2-thiazin-5-yl, 2H-3,4-dihydro-1,2-thiazin-6-yl, 2,3,4,5-tetrahydropyridazin-3-yl, 2,3,4,5-tetrahydropyridazin-4-yl, 2,3,4,5-tetrahydropyridazin-5-yl, 2,3,4,5-tetrahydropyridazin-6-yl, 3,4,5,6-tetrahydropyridazin-3-yl, 3,4,5,6-tetrahydropyridazin-4-yl, 1,2,5,6-tetrahydropyridazin-3-yl, 1,2,5,6-tetrahydropyridazin-4-yl, 1,2,5,6-tetrahydropyridazin-5-yl, 1,2,5,6-tetrahydropyridazin-6-yl, 1,2,3,6-tetrahydropyridazin-3-yl, 1,2,3,6-tetrahydropyridazin-4-yl, 4H-5,6-dihydro-1,3-oxazin-2-yl, 4H-5,6-dihydro-1,3-oxazin-4-yl, 4H-5,6-dihydro-1,3-oxazin-5-yl, 4H-5,6-dihydro-1,3-oxazin-6-yl, 4H-5,6-dihydro-1,3-thiazin-2-yl, 4H-5,6-dihydro-1,3-thiazin-4-yl, 4H-5,6-dihydro-1,3-thiazin-5-yl, 4H-5,6-dihydro-1,3-thiazin-6-yl, 3,4,5,6-tetrahydropyrimidin-2-yl, 3,4,5,6-tetrahydropyrimidin-4-yl, 3,4,5,6-tetrahydropyrimidin-5-yl, 3,4,5,6-tetrahydropyrimidin-6-yl, 1,2,3,4-tetrahydropyrazin-2-yl, 1,2,3,4-tetrahydropyrazin-5-yl, 1,2,3,4-tetrahydropyrimidin-2-yl, 1,2,3,4-tetrahydropyrimidin-4-yl, 1,2,3,4-tetrahydropyrimidin-5-yl, 1,2,3,4-tetrahydropyrimidin-6-yl, 2,3-dihydro-1,4-thiazin-2-yl, 2,3-dihydro-1,4-thiazin-3-yl, 2,3-dihydro-1,4-thiazin-5-yl, 2,3-dihydro-1,4-thiazin-6-yl, 2H-1,2-oxazin-3-yl, 2H-1,2-oxazin-4-yl, 2H-1,2-oxazin-5-yl, 2H-1,2-oxazin-6-yl, 2H-1,2-thiazin-3-yl, 2H-1,2-thiazin-4-yl, 2H-1,2-thiazin-5-yl, 2H-1,2-thiazin-6-yl, 4H-1,2-oxazin-3-yl, 4H-1,2-oxazin-4-yl, 4H-1,2-oxazin-5-yl, 4H-1,2-oxazin-6-yl, 4H-1,2-thiazin-3-yl, 4H-1,2-thiazin-4-yl, 4H-1,2-thiazin-5-yl, 4H-1,2-thiazin-6-yl, 6H-1,2-oxazin-3-yl, 6H-1,2-oxazin-4-yl, 6H-1,2-oxazin-5-yl, 6H-1,2-oxazin-6-yl, 6H-1,2-thiazin-3-yl, 6H-1,2-thiazin-4-yl, 6H-1,2-thiazin-5-yl, 6H-1,2-thiazin-6-yl, 2H-1,3-oxazin-2-yl, 2H-1,3-oxazin-4-yl, 2H-1,3-oxazin-5-yl, 2H-1,3-oxazin-6-yl, 2H-1,3-thiazin-2-yl, 2H-1,3-thiazin-4-yl, 2H-1,3-thiazin-5-yl, 2H-1,3-thiazin-6-yl, 4H-1,3-oxazin-2-yl, 4H-1,3-oxazin-4-yl, 4H-1,3-oxazin-5-yl, 4H-1,3-oxazin-6-yl, 4H-1,3-thiazin-2-yl, 4H-1,3-thiazin-4-yl, 4H-1,3-thiazin-5-yl, 4H-1,3-thiazin-6-yl, 6H-1,3-oxazin-2-yl, 6H-1,3-oxazin-4-yl, 6H-1,3-oxazin-5-yl, 6H-1,3-oxazin-6-yl, 6H-1,3-thiazin-2-yl, 6H-1,3-oxazin-4-yl, 6H-1,3-oxazin-5-yl, 6H-1,3-thiazin-6-yl, 2H-1,4-oxazin-2-yl, 2H-1,4-oxazin-3-yl, 2H-1,4-oxazin-5-yl, 2H-1,4-oxazin-6-yl, 2H-1,4-thiazin-2-yl, 2H-1,4-thiazin-3-yl, 2H-1,4-thiazin-5-yl, 2H-1,4-thiazin-6-yl, 4H-1,4-oxazin-2-yl, 4H-1,4-oxazin-3-yl, 4H-1,4-thiazin-2-yl, 4H-1,4-thiazin-3-yl, 1,4-dihydropyridazin-3-yl, 1,4-dihydropyridazin-4-yl, 1,4-dihydropyridazin-5-yl, 1,4-dihydropyridazin-6-yl, 1,4-dihydropyrazin-2-yl, 1,2-dihydropyrazin-2-yl, 1,2-dihydropyrazin-3-yl, 1,2-dihydropyrazin-5-yl, 1,2-dihydropyrazin-6-yl, 1,4-dihydropyrimidin-2-yl, 1,4-dihydropyrimidin-4-yl, 1,4-dihydropyrimidin-5-yl, 1,4-dihydropyrimidin-6-yl, 3,4-dihydropyrimidin-2-yl, 3,4-dihydropyrimidin-4-yl, 3,4-dihydropyrimidin-5-yl or 3,4-dihydropyrimidin-6-yl, pyridazin-3-yl, pyridazin-4-yl, pyrimidin-2-yl, pyrimidin-4-yl, pyrimidin-5-yl or pyrazin-2-yl;

[0090] 6-membered rings having three heteroatoms such as: 1,3,5-triazin-2-yl, 1,2,4-triazin-3-yl, 1,2,4-triazin-5-yl, 1,2,4-triazin-6-yl; [0091] 6-membered rings having four heteroatoms such as: 1,2,4,5-tetrazin-3-yl; [0092] where, if appropriate, the sulfur of the above-mentioned heterocycles may be oxidized to S.dbd.O or S(.dbd.O).sub.2 [0093] and where a bicyclic ring system may be formed with a fused-on phenyl ring or with a C.sub.3-C.sub.6-carbocycle or with a further 5- to 6-membered heterocycle. [0094] N-bonded heterocyclyl: a saturated, partially saturated or unsaturated 5- or 6-membered heterocyclic ring which is attached via nitrogen and contains at least one nitrogen and, if appropriate, one to three identical or different heteroatoms selected from the following group: oxygen, sulfur and nitrogen, i.e., for example, [0095] N-bonded 5-membered rings such as: tetrahydropyrrol-1-yl, 2,3-dihydro-1H-pyrrol-1-yl, 2,5-dihydro-1H-pyrrol-1-yl, pyrrol-1-yl, tetrahydropyrazol-1-yl, tetrahydroisoxazol-2-yl, tetrahydroisothiazol-2-yl, tetrahydroimidazol-1-yl, tetrahydrooxazol-3-yl, tetrahydrothiazol-3-yl, 4,5-dihydro-1H-pyrazol-1-yl, 2,5-dihydro-1H-pyrazol-1-yl, 2,3-dihydro-1H-pyrazol-1-yl, 2,5-dihydroisoxazol-2-yl, 2,3-dihydroisoxazol-2-yl, 2,5-dihydroisothiazol-2-yl, 2,3-dihydroisoxazol-2-yl, 4,5-dihydro-1H-imidazol-1-yl, 2,5-dihydro-1H-imidazol-1-yl, 2,3-dihydro-1H-imidazol-1-yl, 2,3-dihydrooxazol-3-yl, 2,3-dihydrothiazol-3-yl, pyrazol-1-yl, imidazol-1-yl, 1,2,4-.DELTA..sup.4-oxadiazolin-2-yl, 1,2,4-.DELTA..sup.2-oxadiazolin-4-yl, 1,2,4-.DELTA..sup.3-oxadiazolin-2-yl, 1,3,4-.DELTA..sup.2-oxadiazolin-4-yl, 1,2,4-.DELTA..sup.5-thiadiazolin-2-yl, 1,2,4-.DELTA..sup.3-thiadiazolin-2-yl, 1,2,4-.DELTA..sup.2-thiadiazolin-4-yl, 1,3,4-.DELTA..sup.2-thiadiazolin-4-yl, 1,2,3-.DELTA..sup.2-triazolin-1-yl, 1,2,4-.DELTA..sup.2-triazolin-1-yl, 1,2,4-.DELTA..sup.2-triazolin-4-yl, 1,2,4-.DELTA..sup.3-triazolin-1-yl, 1,2,4-.DELTA..sup.1-triazolin-4-yl, 1,2,3-triazol-1-yl, 1,2,4-triazol-1-yl, tetrazol-1-yl; [0096] and also N-bonded 6-membered rings such as: piperidin-1-yl, 1,2,3,4-tetrahydropyridin-1-yl, 1,2,5,6-tetrahydropyridin-1-yl, 1,4-dihydropyridin-1-yl, 1,2-dihydropyridin-1-yl, hexahydropyrimidin-1-yl, hexahydropyrazin-1-yl, hexahydropyridazin-1-yl, tetrahydro-1,3-oxazin-3-yl, tetrahydro-1,3-thiazin-3-yl, tetrahydro-1,4-thiazin-4-yl, tetrahydro-1,4-oxazin-4-yl, tetrahydro-1,2-oxazin-2-yl, 2H-5,6-dihydro-1,2-oxazin-2-yl, 2H-5,6-dihydro-1,2-thiazin-2-yl, 2H-3,6-dihydro-1,2-oxazin-2-yl, 2H-3,6-dihydro-1,2-thiazin-2-yl, 2H-3,4-dihydro-1,2-oxazin-2-yl, 2H-3,4-dihydro-1,2-thiazin-2-yl, 2,3,4,5-tetrahydropyridazin-2-yl, 1,2,5,6-tetrahydropyridazin-1-yl, 1,2,5,6-tetrahydropyridazin-2-yl, 1,2,3,6-tetrahydropyridazin-1-yl, 3,4,5,6-tetrahydropyrimidin-3-yl, 1,2,3,4-tetrahydropyrazin-1-yl, 1,2,3,4-tetrahydropyrimidin-1-yl, 1,2,3,4-tetrahydropyrimidin-3-yl, 2,3-dihydro-1,4-thiazin-4-yl, 2H-1,2-oxazin-2-yl, 2H-1,2-thiazin-2-yl, 4H-1,4-oxazin-4-yl, 4H-1,4-thiazin-4-yl, 1,4-dihydropyridazin-1-yl, 1,4-dihydropyrazin-1-yl, 1,2-dihydropyrazin-1-yl, 1,4-dihydropyrimidin-1-yl or 3,4-dihydropyrimidin-3-yl; [0097] and also N-bonded cyclic imides such as: [0098] phthalimide, tetrahydrophthalimide, succinimide, maleimide, glutarimide, 5-oxotriazolin-1-yl, 5-oxo-1,3,4-oxadiazolin-4-yl or 2,4-dioxo-(1H,3H)-pyrimidin-3-yl; [0099] where a bicyclic ring system may be formed with a fused-on phenyl ring or with a C.sub.3-C.sub.6-carbocycle or a further 5- to 6-membered heterocycle.

[0100] All phenyl rings, heterocyclyl or N-heterocyclyl radicals and all phenyl components in phenoxy, phenyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl, phenylalkenylcarbonyl, phenoxycarbonyl, phenyloxythiocarbonyl, phenylaminocarbonyl and N--(C.sub.1-C.sub.6-alkyl)-N-phenylaminocarbonyl or heterocyclyl components in heterocyclyloxy, heterocyclyl-C.sub.1-C.sub.6-alkyl, heterocyclylcarbonyl-C.sub.1-C.sub.6-alkyl, heterocyclylcarbonyl, heterocyclyloxythiocarbonyl, heterocyclylalkenylcarbonyl, heterocyclyloxycarbonyl, heterocyclylaminocarbonyl and N--(C.sub.1-C.sub.6-alkyl)-N-heterocyclylaminocarbonyl are, unless stated otherwise, preferably unsubstituted, or they carry one to three halogen atoms and/or one nitro group, one cyano radical and/or one or two methyl, trifluoromethyl, methoxy or trifluoromethoxy substitutents.

[0101] Furthermore, the expression "Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated heterocycle which contains one to three identical or different heteroatoms selected from the following group: oxygen, sulfur and nitrogen" denotes, for example, 5-membered rings having one heteroatom such as:

tetrahydrofurandiyl, tetrahydrothienediyl, tetrahydropyrrolediyl, dihydrofurandiyl, dihydrothienediyl, dihydropyrrolediyl, furandiyl, thienediyl or pyrrolediyl;

or 5-membered rings having two heteroatoms such as:

[0102] tetrahydropyrazolediyl, tetrahydroisoxazolediyl, 1,2-oxathiolanediyl, tetrahydroisothiazolediyl, 1,2-dithiolanediyl, tetrahydroimidazolediyl, tetrahydrooxazolediyl, tetrahydrothiazolediyl, 1,3-dioxolanediyl, 1,3-oxathiolanediyl, dihydropyrazolediyl, dihydroisoxazolediyl, dihydroisothiazolediyl, 1,2-dithiolediyl, dihydroimidazolediyl, dihydrooxazolediyl, dihydrothiazolediyl, dioxolediyl, oxathiolediyl, pyrazolediyl, isoxazolediyl, isothiazolediyl, imidazolediyl, oxazolediyl or thiazolediyl;

or 5-membered rings having three heteroatoms such as:

1,2,3-oxadiazolinediyl, 1,2,3-thiadiazolinediyl, 1,2,3-triazolinediyl, 1,2,3-oxadiazolediyl, 1,2,3-thiadiazolediyl or 1,2,3-triazolediyl;

or 6-membered rings having one heteroatom such as:

tetrahydropyrandiyl, piperidinediyl, tetrahydrothiopyrandiyl, dihydropyrandiyl, dihydrothiopyrandiyl, tetrahydropyridinediyl, pyrandiyl, thiopyrandiyl, dihydropyrinediyl or pyridinediyl;

or 6-membered rings having two heteroatoms such as:

[0103] 1,3-dioxanediyl, 1,4-dioxanediyl, 1,3-dithianediyl, 1,4-dithianediyl, 1,3-oxathianediyl, 1,4-oxathianediyl, 1,2-dithianediyl, hexahydropyrimidinediyl, hexahydropyrazinediyl, hexahydropyridazinediyl, tetrahydro-1,3-oxazinediyl, tetrahydro-1,3-thiazinediyl, tetrahydro-1,4-oxazinediyl, tetrahydro-1,2-oxazinediyl, dihydro-1,2-oxazinediyl, dihydro-1,2-thiazinediyl, tetrahydropyridazinediyl, dihydro-1,3-oxazinediyl, dihydro-1,3-oxazinediyl, dihydro-1,3-thiazinediyl, tetrahydropyrimidinediyl, tetrahydropyrazinediyl, dihydro-1,4-thiazinediyl, dihydro-1,4-oxazinediyl, dihydro-1,4-dioxinediyl, dihydro-1,4-dithiinediyl, 1,2-oxazinediyl, 1,2-thiazinediyl, 1,3-oxazinediyl, 1,3-thiazinediyl, 1,4-oxazinediyl, 1,4-thiazinediyl, dihydropyridazinediyl, dihydropyrazinediyl, dihydropyrimidinediyl, pyridazinediyl, pyrimidinediyl or pyrazinediyl;

or 6-membered rings having 3 heteroatoms such as:

1,2,4-triazinediyl;

where, if appropriate, the sulfur of the abovementioned heterocycles may be oxidized to S.dbd.O or S(.dbd.O).sub.2;

and where the moiety is fused to the skeleton via two adjacent carbon atoms.

[0104] The compounds of the formula I according to the invention where R.sup.9=IIa are referred to as compounds of the formula Ia, and compounds of the formula I where R.sup.9=IIb are referred to as Ib.

[0105] Preference is given to the compounds of the formula I, where [0106] R.sup.11 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, hydroxyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy;

[0107] Preference is likewise given to the compounds of the formula Ia.

[0108] With respect to the use of the compounds of the formula I according to the invention as herbicides, the variables preferably have the following meanings, in each case alone or in combination: [0109] X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7, NR.sup.8 or a bond; [0110] Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated 5- or 6-membered heterocycle which contains one or two identical or different heteroatoms selected from the following group: oxygen, sulfur or nitrogen; [0111] R.sup.1, R.sup.2 are hydrogen or C.sub.1-C.sub.6-alkyl; [0112] R.sup.3 is halogen, C.sub.1-C.sub.6-alkyl or C.sub.1-C.sub.6-alkoxy; [0113] R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl)amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; [0114] in particular nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfonyl or C.sub.1-C.sub.6-haloalkylsulfonyl; [0115] R.sup.5 is hydrogen; [0116] R.sup.6, R.sup.7 are hydrogen or C.sub.1-C.sub.6-alkyl; [0117] R.sup.8 is C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-alkylcarbonyl or C.sub.1-C.sub.6-alkylsulfonyl; [0118] l is 0, 1 or 2; [0119] R.sup.9 is a radical IIa ##STR6## where [0120] R.sup.10 is hydroxyl, mercapto, halogen, OR.sup.13, SR.sup.13, SO.sub.2R.sup.14 or N-bonded heterocyclyl, where the heterocyclyl radical may be partially or fully halogenated and/or may carry one to three of the following radicals: [0121] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; [0122] R.sup.11 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl or C.sub.3-C.sub.6-cycloalkyl; [0123] R.sup.12 is hydrogen, C.sub.1-C.sub.6-alkyl or C.sub.1-C.sub.6-haloalkyl; [0124] R.sup.13 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-alkynyl, C.sub.1-C.sub.6-alkylcarbonyl, C.sub.2-C.sub.6-alkenylcarbonyl, C.sub.3-C.sub.6-cycloalkylcarbonyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.3-C.sub.6-alkenyloxycarbonyl, C.sub.3-C.sub.6-alkynyloxycarbonyl, C.sub.1-C.sub.6-alkylthiocarbonyl, C.sub.1-C.sub.6-alkylaminocarbonyl, C.sub.3-C.sub.6-alkenylaminocarbonyl, C.sub.3-C.sub.6-alkynylaminocarbonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.1-C.sub.6-alkoxy)-N--(C.sub.1-C.sub.6-alkyl) aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl, di(C.sub.1-C.sub.6-alkyl)aminothiocarbonyl, C.sub.1-C.sub.6-alkylcarbonyl-C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-alkoxyimino-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl or N,N-di(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl, where the abovementioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three of the following groups: [0125] cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; [0126] is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl, heterocyclyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl-C.sub.1-C.sub.6-alkyl, heterocyclylcarbonyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl, heterocyclylcarbonyl, phenoxycarbonyl, phenyloxythiocarbonyl, heterocyclyloxycarbonyl, heterocyclyloxythiocarbonyl, phenyl-C.sub.2-C.sub.6-alkenylcarbonyl or heterocyclyl-C.sub.2-C.sub.6-alkenylcarbonyl, where the phenyl and the heterocyclyl radical of the 14 lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: [0127] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-haloalkoxy, heterocyclyl or N-bonded heterocyclyl, where the two lastmentioned substitutents for their part may be partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; [0128] R.sup.14 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-cycloalkyl, C.sub.1-C.sub.6-alkoxy or di(C.sub.1-C.sub.6-haloalkyl)amino, where the abovementioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three of the following groups: [0129] cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; [0130] is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl, heterocyclyl-C.sub.1-C.sub.6-alkyl, phenoxy, heterocyclyloxy, where the phenyl and the heterocyclyl radical of the lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: [0131] nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy.

[0132] Particular preference is given to compounds of the formula I where the variables have the following meanings, either alone or in combination: [0133] X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7 or a bond; [0134] Y together with the two carbons to which it is attached forms the following heterocycles: [0135] (in the embodiments of the heterocycles below, the upper undulating line represents in each case the link to the hydrocarbon which carries the radicals R.sup.1 and R.sup.2, and the lower undulating line represents the link to the meta-carbon of the benzoyl moiety). ##STR7## ##STR8## where the sulfur of the abovementioned heterocycles may be oxidized to S.dbd.O or S(.dbd.O).sub.2; in particular, Y together with the two carbons to which it is attached forms the following heterocycles: ##STR9## ##STR10## [0136] R.sup.1, R.sup.2 are hydrogen; [0137] R.sup.3 is C.sub.1-C.sub.6-alkyl, such as methyl, ethyl or n-propyl; in particular methyl; [0138] R.sup.4 is nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; in particular nitro, halogen, such as fluorine, chlorine or bromine, C.sub.1-C.sub.6-haloalkyl such as trifluoromethyl, C.sub.1-C.sub.6-alkylthio, such as methylthio or ethylthio, or C.sub.1-C.sub.6-alkylsulfonyl, such as methylsulfonyl or ethylsulfonyl; [0139] particularly preferably nitro, chlorine, trifluoromethyl, methylthio or methylsulfonyl; [0140] R.sup.5 is hydrogen; [0141] R.sup.6, R.sup.7 are hydrogen or C.sub.1-C.sub.6-alkyl, such as methyl or ethyl; [0142] in particular hydrogen or methyl; [0143] l is 0, 1 or 2; [0144] in particular 0 or 1; [0145] R.sup.9 is a radical IIa ##STR11## where [0146] R.sup.10 is hydroxyl; [0147] R.sup.11 is C.sub.1-C.sub.6-alkyl, such as methyl, ethyl, n-propyl, 1-methylethyl, n-butyl, 2-methylpropyl or 1,1-dimethylethyl or cyclopropyl; [0148] in particular methyl or ethyl; [0149] likewise particularly preferred cyclopropyl; [0150] R.sup.12 is hydrogen or C.sub.1-C.sub.6-alkyl, such as methyl, ethyl, n-propyl or 1-methylethyl; [0151] in particular hydrogen or methyl.

[0152] Very particular preference is given to the compounds 1a where [0153] X is oxygen, sulfur, S(.dbd.O).sub.2, CH.sub.2 or a bond; [0154] Y together with the two carbons to which it is attached forms the following heterocycles: ##STR12## [0155] R.sup.1, R.sup.2 are hydrogen; [0156] R.sup.3 is C.sub.1-C.sub.4-alkyl; [0157] R.sup.4 is nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; [0158] R.sup.5 is hydrogen or C.sub.1-C.sub.6-alkyl; [0159] l is 0, 1 or 2; [0160] R.sup.9 is a radical IIa; [0161] R.sup.10 is hydroxyl; [0162] R.sup.11 is hydrogen, C.sub.1-C.sub.6-alkyl or cyclopropyl; [0163] in particular C.sub.1-C.sub.6-alkyl; [0164] R.sup.12 is hydrogen, C.sub.1-C.sub.6-alkyl or C.sub.1-C.sub.6-haloalkyl.

[0165] Very particular preference is also given to the compounds Ia where X is oxygen, sulfur or a bond.

[0166] Very particular preference is also given to the compounds 1a where [0167] Y together with the two carbons to which it is attached forms a heterocycle selected from the following group: dihydropyrazolediyl, dihydroisoxazolediyl, pyrazolediyl, isoxazolediyl or pyrimidinediyl.

[0168] Most preferably, Y together with the two carbons to which it is attached forms the following heterocycles: ##STR13##

[0169] Very particular preference is also given to the compounds of the formula I where [0170] R.sup.1, R.sup.2 are hydrogen; [0171] R.sup.3 is C.sub.1-C.sub.6-alkyl; [0172] R.sup.4 is nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; [0173] in particular halogen, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; [0174] R.sup.5 is hydrogen; [0175] l is 0 oder 1.

[0176] Very particular preference is also given to the compounds of the formula I where [0177] R.sup.10 is hydroxyl or phenylcarbonyloxy which may be unsubstituted or partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; [0178] in particular hydroxyl; [0179] R.sup.11 is C.sub.1-C.sub.6-alkyl or C.sub.3-C.sub.6-cycloalkyl; [0180] in particular C.sub.1-C.sub.6-alkyl or [0181] also in particular cyclopropyl; [0182] R.sup.12 is hydrogen or C.sub.1-C.sub.6-alkyl; [0183] in particular hydrogen.

[0184] Very particular preference is also given to the compounds of the formula Ia1 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0, meaning of the heterocycle according to structural formula), most particularly to compounds Ia1.n where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1.

[0185] The radical definitions of R.sup.1 to R.sup.12, X, Y and l given above and the meaning of the fused heterocycle are of particular importance for the compounds according to the invention, not only in combination with one another, but also taken on their own. (For reasons of clarity, in the formulae Ia1, Ia2 . . . , the meaning of the fused heterocycle is in each case as given in the corresponding structural formula.) TABLE-US-00001 TABLE 1 Ia1 ##STR14## n X R.sup.4 R.sup.10 R.sup.11 1 bond F OH CH.sub.3 2 bond Cl OH CH.sub.3 3 bond Br OH CH.sub.3 4 bond NO.sub.2 OH CH.sub.3 5 bond SCH.sub.3 OH CH.sub.3 6 bond SO.sub.2CH.sub.3 OH CH.sub.3 7 bond SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.3 8 bond CH.sub.3 OH CH.sub.3 9 bond CF.sub.3 OH CH.sub.3 10 bond OCHF.sub.2 OH CH.sub.3 11 CH.sub.2 F OH CH.sub.3 12 CH.sub.2 Cl OH CH.sub.3 13 CH.sub.2 Br OH CH.sub.3 14 CH.sub.2 NO.sub.2 OH CH.sub.3 15 CH.sub.2 SCH.sub.3 OH CH.sub.3 16 CH.sub.2 SO.sub.2CH.sub.3 OH CH.sub.3 17 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.3 18 CH.sub.2 CH.sub.3 OH CH.sub.3 19 CH.sub.2 CF.sub.3 OH CH.sub.3 20 CH.sub.2 OCHF.sub.2 OH CH.sub.3 21 O F OH CH.sub.3 22 O Cl OH CH.sub.3 23 O Br OH CH.sub.3 24 O NO.sub.2 OH CH.sub.3 25 O SCH.sub.3 OH CH.sub.3 26 O SO.sub.2CH.sub.3 OH CH.sub.3 27 O SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.3 28 O CH.sub.3 OH CH.sub.3 29 O CF.sub.3 OH CH.sub.3 30 O OCHF.sub.2 OH CH.sub.3 31 S F OH CH.sub.3 32 S Cl OH CH.sub.3 33 S Br OH CH.sub.3 34 S NO.sub.2 OH CH.sub.3 35 S SCH.sub.3 OH CH.sub.3 36 S SO.sub.2CH.sub.3 OH CH.sub.3 37 S SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.3 38 S CH.sub.3 OH CH.sub.3 39 S CF.sub.3 OH CH.sub.3 40 S OCHF.sub.2 OH CH.sub.3 41 SO.sub.2 F OH CH.sub.3 42 SO.sub.2 Cl OH CH.sub.3 43 SO.sub.2 Br OH CH.sub.3 44 SO.sub.2 NO.sub.2 OH CH.sub.3 45 SO.sub.2 SCH.sub.3 OH CH.sub.3 46 SO.sub.2 SO.sub.2CH.sub.3 OH CH.sub.3 47 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.3 48 SO.sub.2 CH.sub.3 OH CH.sub.3 49 SO.sub.2 CF.sub.3 OH CH.sub.3 50 SO.sub.2 OCHF.sub.2 OH CH.sub.3 51 bond F OH CH.sub.2CH.sub.3 52 bond Cl OH CH.sub.2CH.sub.3 53 bond Br OH CH.sub.2CH.sub.3 54 bond NO.sub.2 OH CH.sub.2CH.sub.3 55 bond SCH.sub.3 OH CH.sub.2CH.sub.3 56 bond SO.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 57 bond SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 58 bond CH.sub.3 OH CH.sub.2CH.sub.3 59 bond CF.sub.3 OH CH.sub.2CH.sub.3 60 bond OCHF.sub.2 OH CH.sub.2CH.sub.3 61 CH.sub.2 F OH CH.sub.2CH.sub.3 62 CH.sub.2 Cl OH CH.sub.2CH.sub.3 63 CH.sub.2 Br OH CH.sub.2CH.sub.3 64 CH.sub.2 NO.sub.2 OH CH.sub.2CH.sub.3 65 CH.sub.2 SCH.sub.3 OH CH.sub.2CH.sub.3 66 CH.sub.2 SO.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 67 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 68 CH.sub.2 CH.sub.3 OH CH.sub.2CH.sub.3 69 CH.sub.2 CF.sub.3 OH CH.sub.2CH.sub.3 70 CH.sub.2 OCHF.sub.2 OH CH.sub.2CH.sub.3 71 O F OH CH.sub.2CH.sub.3 72 O Cl OH CH.sub.2CH.sub.3 73 O Br OH CH.sub.2CH.sub.3 74 O NO.sub.2 OH CH.sub.2CH.sub.3 75 O SCH.sub.3 OH CH.sub.2CH.sub.3 76 O SO.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 77 O SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 78 O CH.sub.3 OH CH.sub.2CH.sub.3 79 O CF.sub.3 OH CH.sub.2CH.sub.3 80 O OCHF.sub.2 OH CH.sub.2CH.sub.3 81 S F OH CH.sub.2CH.sub.3 82 S Cl OH CH.sub.2CH.sub.3 83 S Br OH CH.sub.2CH.sub.3 84 S NO.sub.2 OH CH.sub.2CH.sub.3 85 S SCH.sub.3 OH CH.sub.2CH.sub.3 86 S SO.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 87 S SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 88 S CH.sub.3 OH CH.sub.2CH.sub.3 89 S CF.sub.3 OH CH.sub.2CH.sub.3 90 S OCHF.sub.2 OH CH.sub.2CH.sub.3 91 SO.sub.2 F OH CH.sub.2CH.sub.3 92 SO.sub.2 Cl OH CH.sub.2CH.sub.3 93 SO.sub.2 Br OH CH.sub.2CH.sub.3 94 SO.sub.2 NO.sub.2 OH CH.sub.2CH.sub.3 95 SO.sub.2 SCH.sub.3 OH CH.sub.2CH.sub.3 96 SO.sub.2 SO.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 97 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH CH.sub.2CH.sub.3 98 SO.sub.2 CH.sub.3 OH CH.sub.2CH.sub.3 99 SO.sub.2 CF.sub.3 OH CH.sub.2CH.sub.3 100 SO.sub.2 OCHF.sub.2 OH CH.sub.2CH.sub.3 101 bond F OCOC.sub.6H.sub.5 CH.sub.3 102 bond Cl OCOC.sub.6H.sub.5 CH.sub.3 103 bond Br OCOC.sub.6H.sub.5 CH.sub.3 104 bond NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 105 bond SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 106 bond SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 107 bond SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 108 bond CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 109 bond CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 110 bond OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 111 CH.sub.2 F OCOC.sub.6H.sub.5 CH.sub.3 112 CH.sub.2 Cl OCOC.sub.6H.sub.5 CH.sub.3 113 CH.sub.2 Br OCOC.sub.6H.sub.5 CH.sub.3 114 CH.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 115 CH.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 116 CH.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 117 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 118 CH.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 119 CH.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 120 CH.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 121 O F OCOC.sub.6H.sub.5 CH.sub.3 122 O Cl OCOC.sub.6H.sub.5 CH.sub.3 123 O Br OCOC.sub.6H.sub.5 CH.sub.3 124 O NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 125 O SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 126 O SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 127 O SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 128 O CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 129 O CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 130 O OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 131 S F OCOC.sub.6H.sub.5 CH.sub.3 132 S Cl OCOC.sub.6H.sub.5 CH.sub.3 133 S Br OCOC.sub.6H.sub.5 CH.sub.3 134 S NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 135 S SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 136 S SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 137 S SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 138 S CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 139 S CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 140 S OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 141 SO.sub.2 F OCOC.sub.6H.sub.5 CH.sub.3 142 SO.sub.2 Cl OCOC.sub.6H.sub.5 CH.sub.3 143 SO.sub.2 Br OCOC.sub.6H.sub.5 CH.sub.3 144 SO.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 145 SO.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 146 SO.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 147 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 148 SO.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 149 SO.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 150 SO.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.3 151 bond F OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 152 bond Cl OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 153 bond Br OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 154 bond NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 155 bond SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 156 bond SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 157 bond SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 158 bond CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 159 bond CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 160 bond OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 161 CH.sub.2 F OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 162 CH.sub.2 Cl OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 163 CH.sub.2 Br OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 164 CH.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 165 CH.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 166 CH.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 167 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 168 CH.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 169 CH.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 170 CH.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 171 O F OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 172 O Cl OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 173 O Br OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 174 O NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 175 O SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 176 O SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 177 O SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 178 O CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 179 O CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 180 O OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 181 S F OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 182 S Cl OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 183 S Br OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 184 S NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 185 S SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 186 S SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 187 S SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 188 S CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 189 S CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 190 S OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 191 SO.sub.2 F OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 192 SO.sub.2 Cl OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 193 SO.sub.2 Br OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 194 SO.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 195 SO.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 196 SO.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 197 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 198 SO.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 199 SO.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 200 SO.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 CH.sub.2CH.sub.3 201 bond F OCOC(CH.sub.3).sub.3 CH.sub.3 202 bond Cl OCOC(CH.sub.3).sub.3 CH.sub.3 203 bond Br OCOC(CH.sub.3).sub.3 CH.sub.3 204 bond NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 205 bond SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 206 bond SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 207 bond SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 208 bond CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 209 bond CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 210 bond OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 211 CH.sub.2 F OCOC(CH.sub.3).sub.3 CH.sub.3 212 CH.sub.2 Cl OCOC(CH.sub.3).sub.3 CH.sub.3 213 CH.sub.2 Br OCOC(CH.sub.3).sub.3 CH.sub.3 214 CH.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 215 CH.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 216 CH.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 217 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 218 CH.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 219 CH.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 220 CH.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 221 O F OCOC(CH.sub.3).sub.3 CH.sub.3 222 O Cl OCOC(CH.sub.3).sub.3 CH.sub.3 223 O Br OCOC(CH.sub.3).sub.3 CH.sub.3 224 O NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 225 O SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 226 O SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 227 O SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 228 O CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 229 O CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 230 O OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 231 S F OCOC(CH.sub.3).sub.3 CH.sub.3 232 S Cl OCOC(CH.sub.3).sub.3 CH.sub.3 233 S Br OCOC(CH.sub.3).sub.3 CH.sub.3 234 S NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 235 S SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 236 S SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3

237 S SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 238 S CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 239 S CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 240 S OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 241 SO.sub.2 F OCOC(CH.sub.3).sub.3 CH.sub.3 242 SO.sub.2 Cl OCOC(CH.sub.3).sub.3 CH.sub.3 243 SO.sub.2 Br OCOC(CH.sub.3).sub.3 CH.sub.3 244 SO.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 245 SO.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 246 SO.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 247 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 248 SO.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 249 SO.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.3 250 SO.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.3 251 bond F OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 252 bond Cl OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 253 bond Br OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 254 bond NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 255 bond SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 256 bond SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 257 bond SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 258 bond CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 259 bond CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 260 bond OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 261 CH.sub.2 F OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 262 CH.sub.2 Cl OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 263 CH.sub.2 Br OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 264 CH.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 265 CH.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 266 CH.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 267 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 268 CH.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 269 CH.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 270 CH.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 271 O F OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 272 O Cl OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 273 O Br OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 274 O NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 275 O SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 276 O SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 277 O SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 278 O CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 279 O CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 280 O OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 281 S F OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 282 S Cl OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 283 S Br OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 284 S NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 285 S SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 286 S SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 287 S SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 288 S CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 289 S CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 290 S OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 291 SO.sub.2 F OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 292 SO.sub.2 Cl OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 293 SO.sub.2 Br OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 294 SO.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 295 SO.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 296 SO.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 297 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 298 SO.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 299 SO.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 300 SO.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH.sub.2CH.sub.3 301 bond F OCOSCH.sub.3 CH.sub.3 302 bond Cl OCOSCH.sub.3 CH.sub.3 303 bond Br OCOSCH.sub.3 CH.sub.3 304 bond NO.sub.2 OCOSCH.sub.3 CH.sub.3 305 bond SCH.sub.3 OCOSCH.sub.3 CH.sub.3 306 bond SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 307 bond SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 308 bond CH.sub.3 OCOSCH.sub.3 CH.sub.3 309 bond CF.sub.3 OCOSCH.sub.3 CH.sub.3 310 bond OCHF.sub.2 OCOSCH.sub.3 CH.sub.3 311 CH.sub.2 F OCOSCH.sub.3 CH.sub.3 312 CH.sub.2 Cl OCOSCH.sub.3 CH.sub.3 313 CH.sub.2 Br OCOSCH.sub.3 CH.sub.3 314 CH.sub.2 NO.sub.2 OCOSCH.sub.3 CH.sub.3 315 CH.sub.2 SCH.sub.3 OCOSCH.sub.3 CH.sub.3 316 CH.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 317 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 318 CH.sub.2 CH.sub.3 OCOSCH.sub.3 CH.sub.3 319 CH.sub.2 CF.sub.3 OCOSCH.sub.3 CH.sub.3 320 CH.sub.2 OCHF.sub.2 OCOSCH.sub.3 CH.sub.3 321 O F OCOSCH.sub.3 CH.sub.3 322 O Cl OCOSCH.sub.3 CH.sub.3 323 O Br OCOSCH.sub.3 CH.sub.3 324 O NO.sub.2 OCOSCH.sub.3 CH.sub.3 325 O SCH.sub.3 OCOSCH.sub.3 CH.sub.3 326 O SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 327 O SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 328 O CH.sub.3 OCOSCH.sub.3 CH.sub.3 329 O CF.sub.3 OCOSCH.sub.3 CH.sub.3 330 O OCHF.sub.2 OCOSCH.sub.3 CH.sub.3 331 S F OCOSCH.sub.3 CH.sub.3 332 S Cl OCOSCH.sub.3 CH.sub.3 333 S Br OCOSCH.sub.3 CH.sub.3 334 S NO.sub.2 OCOSCH.sub.3 CH.sub.3 335 S SCH.sub.3 OCOSCH.sub.3 CH.sub.3 336 S SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 337 S SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 338 S CH.sub.3 OCOSCH.sub.3 CH.sub.3 339 S CF.sub.3 OCOSCH.sub.3 CH.sub.3 340 S OCHF.sub.2 OCOSCH.sub.3 CH.sub.3 341 SO.sub.2 F OCOSCH.sub.3 CH.sub.3 342 SO.sub.2 Cl OCOSCH.sub.3 CH.sub.3 343 SO.sub.2 Br OCOSCH.sub.3 CH.sub.3 344 SO.sub.2 NO.sub.2 OCOSCH.sub.3 CH.sub.3 345 SO.sub.2 SCH.sub.3 OCOSCH.sub.3 CH.sub.3 346 SO.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 347 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.3 348 SO.sub.2 CH.sub.3 OCOSCH.sub.3 CH.sub.3 349 SO.sub.2 CF.sub.3 OCOSCH.sub.3 CH.sub.3 350 SO.sub.2 OCHF.sub.2 OCOSCH.sub.3 CH.sub.3 351 bond F OCOSCH.sub.3 CH.sub.2CH.sub.3 352 bond Cl OCOSCH.sub.3 CH.sub.2CH.sub.3 353 bond Br OCOSCH.sub.3 CH.sub.2CH.sub.3 354 bond NO.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 355 bond SCH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 356 bond SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 357 bond SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 358 bond CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 359 bond CF.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 360 bond OCHF.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 361 CH.sub.2 F OCOSCH.sub.3 CH.sub.2CH.sub.3 362 CH.sub.2 Cl OCOSCH.sub.3 CH.sub.2CH.sub.3 363 CH.sub.2 Br OCOSCH.sub.3 CH.sub.2CH.sub.3 364 CH.sub.2 NO.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 365 CH.sub.2 SCH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 366 CH.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 367 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 368 CH.sub.2 CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 369 CH.sub.2 CF.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 370 CH.sub.2 OCHF.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 371 O F OCOSCH.sub.3 CH.sub.2CH.sub.3 372 O Cl OCOSCH.sub.3 CH.sub.2CH.sub.3 373 O Br OCOSCH.sub.3 CH.sub.2CH.sub.3 374 O NO.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 375 O SCH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 376 O SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 377 O SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 378 O CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 379 O CF.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 380 O OCHF.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 381 S F OCOSCH.sub.3 CH.sub.2CH.sub.3 382 S Cl OCOSCH.sub.3 CH.sub.2CH.sub.3 383 S Br OCOSCH.sub.3 CH.sub.2CH.sub.3 384 S NO.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 385 S SCH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 386 S SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 387 S SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 388 S CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 389 S CF.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 390 S OCHF.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 391 SO.sub.2 F OCOSCH.sub.3 CH.sub.2CH.sub.3 392 SO.sub.2 Cl OCOSCH.sub.3 CH.sub.2CH.sub.3 393 SO.sub.2 Br OCOSCH.sub.3 CH.sub.2CH.sub.3 394 SO.sub.2 NO.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 395 SO.sub.2 SCH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 396 SO.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 397 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 398 SO.sub.2 CH.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 399 SO.sub.2 CF.sub.3 OCOSCH.sub.3 CH.sub.2CH.sub.3 400 SO.sub.2 OCHF.sub.2 OCOSCH.sub.3 CH.sub.2CH.sub.3 401 bond F OCH.sub.3 CH.sub.3 402 bond Cl OCH.sub.3 CH.sub.3 403 bond Br OCH.sub.3 CH.sub.3 404 bond NO.sub.2 OCH.sub.3 CH.sub.3 405 bond SCH.sub.3 OCH.sub.3 CH.sub.3 406 bond SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 407 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 408 bond CH.sub.3 OCH.sub.3 CH.sub.3 409 bond CF.sub.3 OCH.sub.3 CH.sub.3 410 bond OCHF.sub.2 OCH.sub.3 CH.sub.3 411 CH.sub.2 F OCH.sub.3 CH.sub.3 412 CH.sub.2 Cl OCH.sub.3 CH.sub.3 413 CH.sub.2 Br OCH.sub.3 CH.sub.3 414 CH.sub.2 NO.sub.2 OCH.sub.3 CH.sub.3 415 CH.sub.2 SCH.sub.3 OCH.sub.3 CH.sub.3 416 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 417 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 418 CH.sub.2 CH.sub.3 OCH.sub.3 CH.sub.3 419 CH.sub.2 CF.sub.3 OCH.sub.3 CH.sub.3 420 CH.sub.2 OCHF.sub.2 OCH.sub.3 CH.sub.3 421 O F OCH.sub.3 CH.sub.3 422 O Cl OCH.sub.3 CH.sub.3 423 O Br OCH.sub.3 CH.sub.3 424 O NO.sub.2 OCH.sub.3 CH.sub.3 425 O SCH.sub.3 OCH.sub.3 CH.sub.3 426 O SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 427 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 428 O CH.sub.3 OCH.sub.3 CH.sub.3 429 O CF.sub.3 OCH.sub.3 CH.sub.3 430 O OCHF.sub.2 OCH.sub.3 CH.sub.3 431 S F OCH.sub.3 CH.sub.3 432 S Cl OCH.sub.3 CH.sub.3 433 S Br OCH.sub.3 CH.sub.3 434 S NO.sub.2 OCH.sub.3 CH.sub.3 435 S SCH.sub.3 OCH.sub.3 CH.sub.3 436 S SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 437 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 438 S CH.sub.3 OCH.sub.3 CH.sub.3 439 S CF.sub.3 OCH.sub.3 CH.sub.3 440 S OCHF.sub.2 OCH.sub.3 CH.sub.3 441 SO.sub.2 F OCH.sub.3 CH.sub.3 442 SO.sub.2 Cl OCH.sub.3 CH.sub.3 443 SO.sub.2 Br OCH.sub.3 CH.sub.3 444 SO.sub.2 NO.sub.2 OCH.sub.3 CH.sub.3 445 SO.sub.2 SCH.sub.3 OCH.sub.3 CH.sub.3 446 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 447 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.3 448 SO.sub.2 CH.sub.3 OCH.sub.3 CH.sub.3 449 SO.sub.2 CF.sub.3 OCH.sub.3 CH.sub.3 450 SO.sub.2 OCHF.sub.2 OCH.sub.3 CH.sub.3 451 bond F OCH.sub.3 CH.sub.2CH.sub.3 452 bond Cl OCH.sub.3 CH.sub.2CH.sub.3 453 bond Br OCH.sub.3 CH.sub.2CH.sub.3 454 bond NO.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 455 bond SCH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 456 bond SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 457 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 458 bond CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 459 bond CF.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 460 bond OCHF.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 461 CH.sub.2 F OCH.sub.3 CH.sub.2CH.sub.3 462 CH.sub.2 Cl OCH.sub.3 CH.sub.2CH.sub.3 463 CH.sub.2 Br OCH.sub.3 CH.sub.2CH.sub.3 464 CH.sub.2 NO.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 465 CH.sub.2 SCH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 466 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 467 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 468 CH.sub.2 CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 469 CH.sub.2 CF.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 470 CH.sub.2 OCHF.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 471 O F OCH.sub.3 CH.sub.2CH.sub.3 472 O Cl OCH.sub.3 CH.sub.2CH.sub.3 473 O Br OCH.sub.3 CH.sub.2CH.sub.3 474 O NO.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 475 O SCH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 476 O SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 477 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 478 O CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 479 O CF.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 480 O OCHF.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 481 S F OCH.sub.3 CH.sub.2CH.sub.3 482 S Cl OCH.sub.3 CH.sub.2CH.sub.3 483 S Br OCH.sub.3 CH.sub.2CH.sub.3 484 S NO.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 485 S SCH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3

486 S SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 487 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 488 S CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 489 S CF.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 490 S OCHF.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 491 SO.sub.2 F OCH.sub.3 CH.sub.2CH.sub.3 492 SO.sub.2 Cl OCH.sub.3 CH.sub.2CH.sub.3 493 SO.sub.2 Br OCH.sub.3 CH.sub.2CH.sub.3 494 SO.sub.2 NO.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 495 SO.sub.2 SCH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 496 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 497 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 498 SO.sub.2 CH.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 499 SO.sub.2 CF.sub.3 OCH.sub.3 CH.sub.2CH.sub.3 500 SO.sub.2 OCHF.sub.2 OCH.sub.3 CH.sub.2CH.sub.3 501 bond F OCH(CH.sub.3).sub.2 CH.sub.3 502 bond Cl OCH(CH.sub.3).sub.2 CH.sub.3 503 bond Br OCH(CH.sub.3).sub.2 CH.sub.3 504 bond NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 505 bond SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 506 bond SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 507 bond SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 508 bond CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 509 bond CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 510 bond OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 511 CH.sub.2 F OCH(CH.sub.3).sub.2 CH.sub.3 512 CH.sub.2 Cl OCH(CH.sub.3).sub.2 CH.sub.3 513 CH.sub.2 Br OCH(CH.sub.3).sub.2 CH.sub.3 514 CH.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 515 CH.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 516 CH.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 517 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 518 CH.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 519 CH.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 520 CH.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 521 O F OCH(CH.sub.3).sub.2 CH.sub.3 522 O Cl OCH(CH.sub.3).sub.2 CH.sub.3 523 O Br OCH(CH.sub.3).sub.2 CH.sub.3 524 O NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 525 O SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 526 O SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 527 O SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 528 O CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 529 O CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 530 O OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 531 S F OCH(CH.sub.3).sub.2 CH.sub.3 532 S Cl OCH(CH.sub.3).sub.2 CH.sub.3 533 S Br OCH(CH.sub.3).sub.2 CH.sub.3 534 S NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 535 S SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 536 S SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 537 S SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 538 S CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 539 S CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 540 S OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 541 SO.sub.2 F OCH(CH.sub.3).sub.2 CH.sub.3 542 SO.sub.2 Cl OCH(CH.sub.3).sub.2 CH.sub.3 543 SO.sub.2 Br OCH(CH.sub.3).sub.2 CH.sub.3 544 SO.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 545 SO.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 546 SO.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 547 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 548 SO.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 549 SO.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.3 550 SO.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.3 551 bond F OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 552 bond Cl OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 553 bond Br OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 554 bond NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 555 bond SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 556 bond SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 557 bond SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 558 bond CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 559 bond CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 560 bond OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 561 CH.sub.2 F OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 562 CH.sub.2 Cl OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 563 CH.sub.2 Br OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 564 CH.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 565 CH.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 566 CH.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 567 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 568 CH.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 569 CH.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 570 CH.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 571 O F OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 572 O Cl OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 573 O Br OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 574 O NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 575 O SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 576 O SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 577 O SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 578 O CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 579 O CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 580 O OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 581 S F OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 582 S Cl OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 583 S Br OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 584 S NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 585 S SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 586 S SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 587 S SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 588 S CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 589 S CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 590 S OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 591 SO.sub.2 F OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 592 SO.sub.2 Cl OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 593 SO.sub.2 Br OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 594 SO.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 595 SO.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 596 SO.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 597 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 598 SO.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 599 SO.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 600 SO.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 CH.sub.2CH.sub.3 601 bond F OCH.sub.2C.sub.6H.sub.5 CH.sub.3 602 bond Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.3 603 bond Br OCH.sub.2C.sub.6H.sub.5 CH.sub.3 604 bond NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 605 bond SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 606 bond SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 607 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 608 bond CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 609 bond CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 610 bond OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 611 CH.sub.2 F OCH.sub.2C.sub.6H.sub.5 CH.sub.3 612 CH.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.3 613 CH.sub.2 Br OCH.sub.2C.sub.6H.sub.5 CH.sub.3 614 CH.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 615 CH.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 616 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 617 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 618 CH.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 619 CH.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 620 CH.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 621 O F OCH.sub.2C.sub.6H.sub.5 CH.sub.3 622 O Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.3 623 O Br OCH.sub.2C.sub.6H.sub.5 CH.sub.3 624 O NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 625 O SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 626 O SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 627 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 628 O CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 629 O CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 630 O OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 631 S F OCH.sub.2C.sub.6H.sub.5 CH.sub.3 632 S Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.3 633 S Br OCH.sub.2C.sub.6H.sub.5 CH.sub.3 634 S NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 635 S SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 636 S SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 637 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 638 S CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 639 S CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 640 S OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 641 SO.sub.2 F OCH.sub.2C.sub.6H.sub.5 CH.sub.3 642 SO.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.3 643 SO.sub.2 Br OCH.sub.2C.sub.6H.sub.5 CH.sub.3 644 SO.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 645 SO.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 646 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 647 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 648 SO.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 649 SO.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 650 SO.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.3 651 bond F OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 652 bond Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 653 bond Br OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 654 bond NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 655 bond SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 656 bond SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 657 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 658 bond CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 659 bond CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 660 bond OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 661 CH.sub.2 F OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 662 CH.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 663 CH.sub.2 Br OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 664 CH.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 665 CH.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 666 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 667 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 668 CH.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 669 CH.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 670 CH.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 671 O F OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 672 O Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 673 O Br OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 674 O NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 675 O SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 676 O SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 677 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 678 O CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 679 O CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 680 O OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 681 S F OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 682 S Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 683 S Br OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 684 S NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 685 S SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 686 S SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 687 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 688 S CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 689 S CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 690 S OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 691 SO.sub.2 F OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 692 SO.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 693 SO.sub.2 Br OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 694 SO.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 695 SO.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 696 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 697 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 698 SO.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 699 SO.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 700 SO.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH.sub.2CH.sub.3 701 bond F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 702 bond Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 703 bond Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 704 bond NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 705 bond SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 706 bond SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 707 bond SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 708 bond CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 709 bond CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 710 bond OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 711 CH.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 712 CH.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 713 CH.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 714 CH.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 715 CH.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 716 CH.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 717 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 718 CH.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 719 CH.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 720 CH.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 721 O F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 722 O Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 723 O Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 724 O NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 725 O SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 726 O SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 727 O SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3

728 O CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 729 O CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 730 O OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 731 S F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 732 S Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 733 S Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 734 S NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 735 S SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 736 S SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 737 S SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 738 S CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 739 S CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 740 S OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 741 SO.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 742 SO.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 743 SO.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 744 SO.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 745 SO.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 746 SO.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 747 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 748 SO.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 749 SO.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 750 SO.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.3 751 bond F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 752 bond Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 753 bond Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 754 bond NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 755 bond SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 756 bond SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 757 bond SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 758 bond CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 759 bond CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 760 bond OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 761 CH.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 762 CH.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 763 CH.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 764 CH.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 765 CH.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 766 CH.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 767 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 768 CH.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 769 CH.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 770 CH.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 771 O F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 772 O Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 773 O Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 774 O NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 775 O SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 776 O SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 777 O SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 778 O CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 779 O CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 780 O OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 781 S F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 782 S Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 783 S Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 784 S NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 785 S SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 786 S SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 787 S SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 788 S CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 789 S CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 790 S OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 791 SO.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 792 SO.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 793 SO.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 794 SO.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 795 SO.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 796 SO.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 797 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 798 SO.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 799 SO.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 800 SO.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH.sub.2CH.sub.3 801 bond F SCH.sub.3 CH.sub.3 802 bond Cl SCH.sub.3 CH.sub.3 803 bond Br SCH.sub.3 CH.sub.3 804 bond NO.sub.2 SCH.sub.3 CH.sub.3 805 bond SCH.sub.3 SCH.sub.3 CH.sub.3 806 bond SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 807 bond SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 808 bond CH.sub.3 SCH.sub.3 CH.sub.3 809 bond CF.sub.3 SCH.sub.3 CH.sub.3 810 bond OCHF.sub.2 SCH.sub.3 CH.sub.3 811 CH.sub.2 F SCH.sub.3 CH.sub.3 812 CH.sub.2 Cl SCH.sub.3 CH.sub.3 813 CH.sub.2 Br SCH.sub.3 CH.sub.3 814 CH.sub.2 NO.sub.2 SCH.sub.3 CH.sub.3 815 CH.sub.2 SCH.sub.3 SCH.sub.3 CH.sub.3 816 CH.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 817 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 818 CH.sub.2 CH.sub.3 SCH.sub.3 CH.sub.3 819 CH.sub.2 CF.sub.3 SCH.sub.3 CH.sub.3 820 CH.sub.2 OCHF.sub.2 SCH.sub.3 CH.sub.3 821 O F SCH.sub.3 CH.sub.3 822 O Cl SCH.sub.3 CH.sub.3 823 O Br SCH.sub.3 CH.sub.3 824 O NO.sub.2 SCH.sub.3 CH.sub.3 825 O SCH.sub.3 SCH.sub.3 CH.sub.3 826 O SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 827 O SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 828 O CH.sub.3 SCH.sub.3 CH.sub.3 829 O CF.sub.3 SCH.sub.3 CH.sub.3 830 O OCHF.sub.2 SCH.sub.3 CH.sub.3 831 S F SCH.sub.3 CH.sub.3 832 S Cl SCH.sub.3 CH.sub.3 833 S Br SCH.sub.3 CH.sub.3 834 S NO.sub.2 SCH.sub.3 CH.sub.3 835 S SCH.sub.3 SCH.sub.3 CH.sub.3 836 S SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 837 S SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 838 S CH.sub.3 SCH.sub.3 CH.sub.3 839 S CF.sub.3 SCH.sub.3 CH.sub.3 840 S OCHF.sub.2 SCH.sub.3 CH.sub.3 841 SO.sub.2 F SCH.sub.3 CH.sub.3 842 SO.sub.2 Cl SCH.sub.3 CH.sub.3 843 SO.sub.2 Br SCH.sub.3 CH.sub.3 844 SO.sub.2 NO.sub.2 SCH.sub.3 CH.sub.3 845 SO.sub.2 SCH.sub.3 SCH.sub.3 CH.sub.3 846 SO.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 847 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.3 848 SO.sub.2 CH.sub.3 SCH.sub.3 CH.sub.3 849 SO.sub.2 CF.sub.3 SCH.sub.3 CH.sub.3 850 SO.sub.2 OCHF.sub.2 SCH.sub.3 CH.sub.3 851 bond F SCH.sub.3 CH.sub.2CH.sub.3 852 bond Cl SCH.sub.3 CH.sub.2CH.sub.3 853 bond Br SCH.sub.3 CH.sub.2CH.sub.3 854 bond NO.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 855 bond SCH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 856 bond SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 857 bond SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 858 bond CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 859 bond CF.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 860 bond OCHF.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 861 CH.sub.2 F SCH.sub.3 CH.sub.2CH.sub.3 862 CH.sub.2 Cl SCH.sub.3 CH.sub.2CH.sub.3 863 CH.sub.2 Br SCH.sub.3 CH.sub.2CH.sub.3 864 CH.sub.2 NO.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 865 CH.sub.2 SCH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 866 CH.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 867 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 868 CH.sub.2 CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 869 CH.sub.2 CF.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 870 CH.sub.2 OCHF.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 871 O F SCH.sub.3 CH.sub.2CH.sub.3 872 O Cl SCH.sub.3 CH.sub.2CH.sub.3 873 O Br SCH.sub.3 CH.sub.2CH.sub.3 874 O NO.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 875 O SCH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 876 O SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 877 O SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 878 O CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 879 O CF.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 880 O OCHF.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 881 S F SCH.sub.3 CH.sub.2CH.sub.3 882 S Cl SCH.sub.3 CH.sub.2CH.sub.3 883 S Br SCH.sub.3 CH.sub.2CH.sub.3 884 S NO.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 885 S SCH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 886 S SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 887 S SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 888 S CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 889 S CF.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 890 S OCHF.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 891 SO.sub.2 F SCH.sub.3 CH.sub.2CH.sub.3 892 SO.sub.2 Cl SCH.sub.3 CH.sub.2CH.sub.3 893 SO.sub.2 Br SCH.sub.3 CH.sub.2CH.sub.3 894 SO.sub.2 NO.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 895 SO.sub.2 SCH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 896 SO.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 897 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 898 SO.sub.2 CH.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 899 SO.sub.2 CF.sub.3 SCH.sub.3 CH.sub.2CH.sub.3 900 SO.sub.2 OCHF.sub.2 SCH.sub.3 CH.sub.2CH.sub.3 901 bond F Cl CH.sub.3 902 bond Cl Cl CH.sub.3 903 bond Br Cl CH.sub.3 904 bond NO.sub.2 Cl CH.sub.3 905 bond SCH.sub.3 Cl CH.sub.3 906 bond SO.sub.2CH.sub.3 Cl CH.sub.3 907 bond SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.3 908 bond CH.sub.3 Cl CH.sub.3 909 bond CF.sub.3 Cl CH.sub.3 910 bond OCHF.sub.2 Cl CH.sub.3 911 CH.sub.2 F Cl CH.sub.3 912 CH.sub.2 Cl Cl CH.sub.3 913 CH.sub.2 Br Cl CH.sub.3 914 CH.sub.2 NO.sub.2 Cl CH.sub.3 915 CH.sub.2 SCH.sub.3 Cl CH.sub.3 916 CH.sub.2 SO.sub.2CH.sub.3 Cl CH.sub.3 917 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.3 918 CH.sub.2 CH.sub.3 Cl CH.sub.3 919 CH.sub.2 CF.sub.3 Cl CH.sub.3 920 CH.sub.2 OCHF.sub.2 Cl CH.sub.3 921 O F Cl CH.sub.3 922 O Cl Cl CH.sub.3 923 O Br Cl CH.sub.3 924 O NO.sub.2 Cl CH.sub.3 925 O SCH.sub.3 Cl CH.sub.3 926 O SO.sub.2CH.sub.3 Cl CH.sub.3 927 O SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.3 928 O CH.sub.3 Cl CH.sub.3 929 O CF.sub.3 Cl CH.sub.3 930 O OCHF.sub.2 Cl CH.sub.3 931 S F Cl CH.sub.3 932 S Cl Cl CH.sub.3 933 S Br Cl CH.sub.3 934 S NO.sub.2 Cl CH.sub.3 935 S SCH.sub.3 Cl CH.sub.3 936 S SO.sub.2CH.sub.3 Cl CH.sub.3 937 S SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.3 938 S CH.sub.3 Cl CH.sub.3 939 S CF.sub.3 Cl CH.sub.3 940 S OCHF.sub.2 Cl CH.sub.3 941 SO.sub.2 F Cl CH.sub.3 942 SO.sub.2 Cl Cl CH.sub.3 943 SO.sub.2 Br Cl CH.sub.3 944 SO.sub.2 NO.sub.2 Cl CH.sub.3 945 SO.sub.2 SCH.sub.3 Cl CH.sub.3 946 SO.sub.2 SO.sub.2CH.sub.3 Cl CH.sub.3 947 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.3 948 SO.sub.2 CH.sub.3 Cl CH.sub.3 949 SO.sub.2 CF.sub.3 Cl CH.sub.3 950 SO.sub.2 OCHF.sub.2 Cl CH.sub.3 951 bond F Cl CH.sub.2CH.sub.3 952 bond Cl Cl CH.sub.2CH.sub.3 953 bond Br Cl CH.sub.2CH.sub.3

954 bond NO.sub.2 Cl CH.sub.2CH.sub.3 955 bond SCH.sub.3 Cl CH.sub.2CH.sub.3 956 bond SO.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 957 bond SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 958 bond CH.sub.3 Cl CH.sub.2CH.sub.3 959 bond CF.sub.3 Cl CH.sub.2CH.sub.3 960 bond OCHF.sub.2 Cl CH.sub.2CH.sub.3 961 CH.sub.2 F Cl CH.sub.2CH.sub.3 962 CH.sub.2 Cl Cl CH.sub.2CH.sub.3 963 CH.sub.2 Br Cl CH.sub.2CH.sub.3 964 CH.sub.2 NO.sub.2 Cl CH.sub.2CH.sub.3 965 CH.sub.2 SCH.sub.3 Cl CH.sub.2CH.sub.3 966 CH.sub.2 SO.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 967 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 968 CH.sub.2 CH.sub.3 Cl CH.sub.2CH.sub.3 969 CH.sub.2 CF.sub.3 Cl CH.sub.2CH.sub.3 970 CH.sub.2 OCHF.sub.2 Cl CH.sub.2CH.sub.3 971 O F Cl CH.sub.2CH.sub.3 972 O Cl Cl CH.sub.2CH.sub.3 973 O Br Cl CH.sub.2CH.sub.3 974 O NO.sub.2 Cl CH.sub.2CH.sub.3 975 O SCH.sub.3 Cl CH.sub.2CH.sub.3 976 O SO.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 977 O SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 978 O CH.sub.3 Cl CH.sub.2CH.sub.3 979 O CF.sub.3 Cl CH.sub.2CH.sub.3 980 O OCHF.sub.2 Cl CH.sub.2CH.sub.3 981 S F Cl CH.sub.2CH.sub.3 982 S Cl Cl CH.sub.2CH.sub.3 983 S Br Cl CH.sub.2CH.sub.3 984 S NO.sub.2 Cl CH.sub.2CH.sub.3 985 S SCH.sub.3 Cl CH.sub.2CH.sub.3 986 S SO.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 987 S SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 988 S CH.sub.3 Cl CH.sub.2CH.sub.3 989 S CF.sub.3 Cl CH.sub.2CH.sub.3 990 S OCHF.sub.2 Cl CH.sub.2CH.sub.3 991 SO.sub.2 F Cl CH.sub.2CH.sub.3 992 SO.sub.2 Cl Cl CH.sub.2CH.sub.3 993 SO.sub.2 Br Cl CH.sub.2CH.sub.3 994 SO.sub.2 NO.sub.2 Cl CH.sub.2CH.sub.3 995 SO.sub.2 SCH.sub.3 Cl CH.sub.2CH.sub.3 996 SO.sub.2 SO.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 997 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl CH.sub.2CH.sub.3 998 SO.sub.2 CH.sub.3 Cl CH.sub.2CH.sub.3 999 SO.sub.2 CF.sub.3 Cl CH.sub.2CH.sub.3 1000 SO.sub.2 OCHF.sub.2 Cl CH.sub.2CH.sub.3 1001 bond F OH CH(CH.sub.3).sub.2 1002 bond Cl OH CH(CH.sub.3).sub.2 1003 bond Br OH CH(CH.sub.3).sub.2 1004 bond NO.sub.2 OH CH(CH.sub.3).sub.2 1005 bond SCH.sub.3 OH CH(CH.sub.3).sub.2 1006 bond SO.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1007 bond SO.sub.2CH.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1008 bond CH.sub.3 OH CH(CH.sub.3).sub.2 1009 bond CF.sub.3 OH CH(CH.sub.3).sub.2 1010 bond OCHF.sub.2 OH CH(CH.sub.3).sub.2 1011 CH.sub.2 F OH CH(CH.sub.3).sub.2 1012 CH.sub.2 Cl OH CH(CH.sub.3).sub.2 1013 CH.sub.2 Br OH CH(CH.sub.3).sub.2 1014 CH.sub.2 NO.sub.2 OH CH(CH.sub.3).sub.2 1015 CH.sub.2 SCH.sub.3 OH CH(CH.sub.3).sub.2 1016 CH.sub.2 SO.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1017 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1018 CH.sub.2 CH.sub.3 OH CH(CH.sub.3).sub.2 1019 CH.sub.2 CF.sub.3 OH CH(CH.sub.3).sub.2 1020 CH.sub.2 OCHF.sub.2 OH CH(CH.sub.3).sub.2 1021 O F OH CH(CH.sub.3).sub.2 1022 O Cl OH CH(CH.sub.3).sub.2 1023 O Br OH CH(CH.sub.3).sub.2 1024 O NO.sub.2 OH CH(CH.sub.3).sub.2 1025 O SCH.sub.3 OH CH(CH.sub.3).sub.2 1026 O SO.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1027 O SO.sub.2CH.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1028 O CH.sub.3 OH CH(CH.sub.3).sub.2 1029 O CF.sub.3 OH CH(CH.sub.3).sub.2 1030 O OCHF.sub.2 OH CH(CH.sub.3).sub.2 1031 S F OH CH(CH.sub.3).sub.2 1032 S Cl OH CH(CH.sub.3).sub.2 1033 S Br OH CH(CH.sub.3).sub.2 1034 S NO.sub.2 OH CH(CH.sub.3).sub.2 1035 S SCH.sub.3 OH CH(CH.sub.3).sub.2 1036 S SO.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1037 S SO.sub.2CH.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1038 S CH.sub.3 OH CH(CH.sub.3).sub.2 1039 S CF.sub.3 OH CH(CH.sub.3).sub.2 1040 S OCHF.sub.2 OH CH(CH.sub.3).sub.2 1041 SO.sub.2 F OH CH(CH.sub.3).sub.2 1042 SO.sub.2 Cl OH CH(CH.sub.3).sub.2 1043 SO.sub.2 Br OH CH(CH.sub.3).sub.2 1044 SO.sub.2 NO.sub.2 OH CH(CH.sub.3).sub.2 1045 SO.sub.2 SCH.sub.3 OH CH(CH.sub.3).sub.2 1046 SO.sub.2 SO.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1047 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH CH(CH.sub.3).sub.2 1048 SO.sub.2 CH.sub.3 OH CH(CH.sub.3).sub.2 1049 SO.sub.2 CF.sub.3 OH CH(CH.sub.3).sub.2 1050 SO.sub.2 OCHF.sub.2 OH CH(CH.sub.3).sub.2 1051 bond F OH C(CH.sub.3).sub.3 1052 bond Cl OH C(CH.sub.3).sub.3 1053 bond Br OH C(CH.sub.3).sub.3 1054 bond NO.sub.2 OH C(CH.sub.3).sub.3 1055 bond SCH.sub.3 OH C(CH.sub.3).sub.3 1056 bond SO.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1057 bond SO.sub.2CH.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1058 bond CH.sub.3 OH C(CH.sub.3).sub.3 1059 bond CF.sub.3 OH C(CH.sub.3).sub.3 1060 bond OCHF.sub.2 OH C(CH.sub.3).sub.3 1061 CH.sub.2 F OH C(CH.sub.3).sub.3 1062 CH.sub.2 Cl OH C(CH.sub.3).sub.3 1063 CH.sub.2 Br OH C(CH.sub.3).sub.3 1064 CH.sub.2 NO.sub.2 OH C(CH.sub.3).sub.3 1065 CH.sub.2 SCH.sub.3 OH C(CH.sub.3).sub.3 1066 CH.sub.2 SO.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1067 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1068 CH.sub.2 CH.sub.3 OH C(CH.sub.3).sub.3 1069 CH.sub.2 CF.sub.3 OH C(CH.sub.3).sub.3 1070 CH.sub.2 OCHF.sub.2 OH C(CH.sub.3).sub.3 1071 O F OH C(CH.sub.3).sub.3 1072 O Cl OH C(CH.sub.3).sub.3 1073 O Br OH C(CH.sub.3).sub.3 1074 O NO.sub.2 OH C(CH.sub.3).sub.3 1075 O SCH.sub.3 OH C(CH.sub.3).sub.3 1076 O SO.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1077 O SO.sub.2CH.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1078 O CH.sub.3 OH C(CH.sub.3).sub.3 1079 O CF.sub.3 OH C(CH.sub.3).sub.3 1080 O OCHF.sub.2 OH C(CH.sub.3).sub.3 1081 S F OH C(CH.sub.3).sub.3 1082 S Cl OH C(CH.sub.3).sub.3 1083 S Br OH C(CH.sub.3).sub.3 1084 S NO.sub.2 OH C(CH.sub.3).sub.3 1085 S SCH.sub.3 OH C(CH.sub.3).sub.3 1086 S SO.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1087 S SO.sub.2CH.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1088 S CH.sub.3 OH C(CH.sub.3).sub.3 1089 S CF.sub.3 OH C(CH.sub.3).sub.3 1090 S OCHF.sub.2 OH C(CH.sub.3).sub.3 1091 SO.sub.2 F OH C(CH.sub.3).sub.3 1092 SO.sub.2 Cl OH C(CH.sub.3).sub.3 1093 SO.sub.2 Br OH C(CH.sub.3).sub.3 1094 SO.sub.2 NO.sub.2 OH C(CH.sub.3).sub.3 1095 SO.sub.2 SCH.sub.3 OH C(CH.sub.3).sub.3 1096 SO.sub.2 SO.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1097 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OH C(CH.sub.3).sub.3 1098 SO.sub.2 CH.sub.3 OH C(CH.sub.3).sub.3 1099 SO.sub.2 CF.sub.3 OH C(CH.sub.3).sub.3 1100 SO.sub.2 OCHF.sub.2 OH C(CH.sub.3).sub.3 1101 bond F OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1102 bond Cl OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1103 bond Br OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1104 bond NO.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1105 bond SCH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1106 bond SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1107 bond SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1108 bond CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1109 bond CF.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1110 bond OCHF.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1111 CH.sub.2 F OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1112 CH.sub.2 Cl OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1113 CH.sub.2 Br OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1114 CH.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1115 CH.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1116 CH.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1117 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1118 CH.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1119 CH.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1120 CH.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1121 O F OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1122 O Cl OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1123 O Br OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1124 O NO.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1125 O SCH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1126 O SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1127 O SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1128 O CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1129 O CF.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1130 O OCHF.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1131 S F OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1132 S Cl OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1133 S Br OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1134 S NO.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1135 S SCH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1136 S SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1137 S SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1138 S CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1139 S CF.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1140 S OCHF.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1141 SO.sub.2 F OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1142 SO.sub.2 Cl OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1143 SO.sub.2 Br OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1144 SO.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1145 SO.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1146 SO.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1147 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1148 SO.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1149 SO.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1150 SO.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 CH(CH.sub.3).sub.2 1151 bond F OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1152 bond Cl OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1153 bond Br OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1154 bond NO.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1155 bond SCH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1156 bond SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1157 bond SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1158 bond CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1159 bond CF.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1160 bond OCHF.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1161 CH.sub.2 F OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1162 CH.sub.2 Cl OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1163 CH.sub.2 Br OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1164 CH.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1165 CH.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1166 CH.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1167 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1168 CH.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1169 CH.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1170 CH.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1171 O F OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1172 O Cl OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1173 O Br OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1174 O NO.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1175 O SCH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1176 O SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1177 O SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1178 O CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1179 O CF.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1180 O OCHF.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1181 S F OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1182 S Cl OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1183 S Br OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1184 S NO.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1185 S SCH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1186 S SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1187 S SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1188 S CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1189 S CF.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1190 S OCHF.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1191 SO.sub.2 F OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1192 SO.sub.2 Cl OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1193 SO.sub.2 Br OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1194 SO.sub.2 NO.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1195 SO.sub.2 SCH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1196 SO.sub.2 SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1197 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1198 SO.sub.2 CH.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1199 SO.sub.2 CF.sub.3 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3 1200 SO.sub.2 OCHF.sub.2 OCOC.sub.6H.sub.5 C(CH.sub.3).sub.3

1201 bond F OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1202 bond Cl OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1203 bond Br OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1204 bond NO.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1205 bond SCH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1206 bond SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1207 bond SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1208 bond CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1209 bond CF.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1210 bond OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1211 CH.sub.2 F OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1212 CH.sub.2 Cl OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1213 CH.sub.2 Br OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1214 CH.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1215 CH.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1216 CH.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1217 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1218 CH.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1219 CH.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1220 CH.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1221 O F OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1222 O Cl OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1223 O Br OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1224 O NO.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1225 O SCH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1226 O SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1227 O SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1228 O CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1229 O CF.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1230 O OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1231 S F OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1232 S Cl OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1233 S Br OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1234 S NO.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1235 S SCH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1236 S SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1237 S SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1238 S CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1239 S CF.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1240 S OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1241 SO.sub.2 F OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1242 SO.sub.2 Cl OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1243 SO.sub.2 Br OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1244 SO.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1245 SO.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1246 SO.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1247 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1248 SO.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1249 SO.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1250 SO.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 CH(CH.sub.3).sub.2 1251 bond F OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1252 bond Cl OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1253 bond Br OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1254 bond NO.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1255 bond SCH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1256 bond SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1257 bond SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1258 bond CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1259 bond CF.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1260 bond OCHF.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1261 CH.sub.2 F OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1262 CH.sub.2 Cl OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1263 CH.sub.2 Br OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1264 CH.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1265 CH.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1266 CH.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1267 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1268 CH.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1269 CH.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1270 CH.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1271 O F OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1272 O Cl OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1273 O Br OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1274 O NO.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1275 O SCH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1276 O SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1277 O SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1278 O CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1279 O CF.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1280 O OCHF.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1281 S F OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1282 S Cl OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1283 S Br OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1284 S NO.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1285 S SCH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1286 S SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1287 S SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1288 S CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1289 S CF.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1290 S OCHF.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1291 SO.sub.2 F OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1292 SO.sub.2 Cl OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1293 SO.sub.2 Br OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1294 SO.sub.2 NO.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1295 SO.sub.2 SCH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1296 SO.sub.2 SO.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1297 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1298 SO.sub.2 CH.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1299 SO.sub.2 CF.sub.3 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1300 SO.sub.2 OCHF.sub.2 OCOC(CH.sub.3).sub.3 C(CH.sub.3).sub.3 1301 bond F OCOSCH.sub.3 CH(CH.sub.3).sub.2 1302 bond Cl OCOSCH.sub.3 CH(CH.sub.3).sub.2 1303 bond Br OCOSCH.sub.3 CH(CH.sub.3).sub.2 1304 bond NO.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1305 bond SCH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1306 bond SO.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1307 bond SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1308 bond CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1309 bond CF.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1310 bond OCHF.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1311 CH.sub.2 F OCOSCH.sub.3 CH(CH.sub.3).sub.2 1312 CH.sub.2 Cl OCOSCH.sub.3 CH(CH.sub.3).sub.2 1313 CH.sub.2 Br OCOSCH.sub.3 CH(CH.sub.3).sub.2 1314 CH.sub.2 NO.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1315 CH.sub.2 SCH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1316 CH.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1317 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1318 CH.sub.2 CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1319 CH.sub.2 CF.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1320 CH.sub.2 OCHF.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1321 O F OCOSCH.sub.3 CH(CH.sub.3).sub.2 1322 O Cl OCOSCH.sub.3 CH(CH.sub.3).sub.2 1323 O Br OCOSCH.sub.3 CH(CH.sub.3).sub.2 1324 O NO.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1325 O SCH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1326 O SO.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1327 O SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1328 O CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1329 O CF.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1330 O OCHF.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1331 S F OCOSCH.sub.3 CH(CH.sub.3).sub.2 1332 S Cl OCOSCH.sub.3 CH(CH.sub.3).sub.2 1333 S Br OCOSCH.sub.3 CH(CH.sub.3).sub.2 1334 S NO.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1335 S SCH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1336 S SO.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1337 S SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1338 S CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1339 S CF.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1340 S OCHF.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1341 SO.sub.2 F OCOSCH.sub.3 CH(CH.sub.3).sub.2 1342 SO.sub.2 Cl OCOSCH.sub.3 CH(CH.sub.3).sub.2 1343 SO.sub.2 Br OCOSCH.sub.3 CH(CH.sub.3).sub.2 1344 SO.sub.2 NO.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1345 SO.sub.2 SCH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1346 SO.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1347 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1348 SO.sub.2 CH.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1349 SO.sub.2 CF.sub.3 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1350 SO.sub.2 OCHF.sub.2 OCOSCH.sub.3 CH(CH.sub.3).sub.2 1351 bond F OCOSCH.sub.3 C(CH.sub.3).sub.3 1352 bond Cl OCOSCH.sub.3 C(CH.sub.3).sub.3 1353 bond Br OCOSCH.sub.3 C(CH.sub.3).sub.3 1354 bond NO.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1355 bond SCH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1356 bond SO.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1357 bond SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1358 bond CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1359 bond CF.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1360 bond OCHF.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1361 CH.sub.2 F OCOSCH.sub.3 C(CH.sub.3).sub.3 1362 CH.sub.2 Cl OCOSCH.sub.3 C(CH.sub.3).sub.3 1363 CH.sub.2 Br OCOSCH.sub.3 C(CH.sub.3).sub.3 1364 CH.sub.2 NO.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1365 CH.sub.2 SCH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1366 CH.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1367 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1368 CH.sub.2 CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1369 CH.sub.2 CF.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1370 CH.sub.2 OCHF.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1371 O F OCOSCH.sub.3 C(CH.sub.3).sub.3 1372 O Cl OCOSCH.sub.3 C(CH.sub.3).sub.3 1373 O Br OCOSCH.sub.3 C(CH.sub.3).sub.3 1374 O NO.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1375 O SCH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1376 O SO.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1377 O SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1378 O CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1379 O CF.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1380 O OCHF.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1381 S F OCOSCH.sub.3 C(CH.sub.3).sub.3 1382 S Cl OCOSCH.sub.3 C(CH.sub.3).sub.3 1383 S Br OCOSCH.sub.3 C(CH.sub.3).sub.3 1384 S NO.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1385 S SCH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1386 S SO.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1387 S SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1388 S CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1389 S CF.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1390 S OCHF.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1391 SO.sub.2 F OCOSCH.sub.3 C(CH.sub.3).sub.3 1392 SO.sub.2 Cl OCOSCH.sub.3 C(CH.sub.3).sub.3 1393 SO.sub.2 Br OCOSCH.sub.3 C(CH.sub.3).sub.3 1394 SO.sub.2 NO.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1395 SO.sub.2 SCH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1396 SO.sub.2 SO.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1397 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1398 SO.sub.2 CH.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1399 SO.sub.2 CF.sub.3 OCOSCH.sub.3 C(CH.sub.3).sub.3 1400 SO.sub.2 OCHF.sub.2 OCOSCH.sub.3 C(CH.sub.3).sub.3 1401 bond F OCH.sub.3 CH(CH.sub.3).sub.2 1402 bond Cl OCH.sub.3 CH(CH.sub.3).sub.2 1403 bond Br OCH.sub.3 CH(CH.sub.3).sub.2 1404 bond NO.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1405 bond SCH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1406 bond SO.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1407 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1408 bond CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1409 bond CF.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1410 bond OCHF.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1411 CH.sub.2 F OCH.sub.3 CH(CH.sub.3).sub.2 1412 CH.sub.2 Cl OCH.sub.3 CH(CH.sub.3).sub.2 1413 CH.sub.2 Br OCH.sub.3 CH(CH.sub.3).sub.2 1414 CH.sub.2 NO.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1415 CH.sub.2 SCH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1416 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1417 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1418 CH.sub.2 CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1419 CH.sub.2 CF.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1420 CH.sub.2 OCHF.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1421 O F OCH.sub.3 CH(CH.sub.3).sub.2 1422 O Cl OCH.sub.3 CH(CH.sub.3).sub.2 1423 O Br OCH.sub.3 CH(CH.sub.3).sub.2 1424 O NO.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1425 O SCH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1426 O SO.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1427 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1428 O CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1429 O CF.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1430 O OCHF.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1431 S F OCH.sub.3 CH(CH.sub.3).sub.2 1432 S Cl OCH.sub.3 CH(CH.sub.3).sub.2 1433 S Br OCH.sub.3 CH(CH.sub.3).sub.2 1434 S NO.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1435 S SCH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1436 S SO.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1437 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1438 S CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1439 S CF.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1440 S OCHF.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1441 SO.sub.2 F OCH.sub.3 CH(CH.sub.3).sub.2 1442 SO.sub.2 Cl OCH.sub.3 CH(CH.sub.3).sub.2 1443 SO.sub.2 Br OCH.sub.3 CH(CH.sub.3).sub.2 1444 SO.sub.2 NO.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1445 SO.sub.2 SCH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1446 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2

1447 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1448 SO.sub.2 CH.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1449 SO.sub.2 CF.sub.3 OCH.sub.3 CH(CH.sub.3).sub.2 1450 SO.sub.2 OCHF.sub.2 OCH.sub.3 CH(CH.sub.3).sub.2 1451 bond F OCH.sub.3 C(CH.sub.3).sub.3 1452 bond Cl OCH.sub.3 C(CH.sub.3).sub.3 1453 bond Br OCH.sub.3 C(CH.sub.3).sub.3 1454 bond NO.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1455 bond SCH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1456 bond SO.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1457 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1458 bond CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1459 bond CF.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1460 bond OCHF.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1461 CH.sub.2 F OCH.sub.3 C(CH.sub.3).sub.3 1462 CH.sub.2 Cl OCH.sub.3 C(CH.sub.3).sub.3 1463 CH.sub.2 Br OCH.sub.3 C(CH.sub.3).sub.3 1464 CH.sub.2 NO.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1465 CH.sub.2 SCH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1466 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1467 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1468 CH.sub.2 CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1469 CH.sub.2 CF.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1470 CH.sub.2 OCHF.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1471 O F OCH.sub.3 C(CH.sub.3).sub.3 1472 O Cl OCH.sub.3 C(CH.sub.3).sub.3 1473 O Br OCH.sub.3 C(CH.sub.3).sub.3 1474 O NO.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1475 O SCH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1476 O SO.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1477 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1478 O CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1479 O CF.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1480 O OCHF.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1481 S F OCH.sub.3 C(CH.sub.3).sub.3 1482 S Cl OCH.sub.3 C(CH.sub.3).sub.3 1483 S Br OCH.sub.3 C(CH.sub.3).sub.3 1484 S NO.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1485 S SCH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1486 S SO.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1487 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1488 S CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1489 S CF.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1490 S OCHF.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1491 SO.sub.2 F OCH.sub.3 C(CH.sub.3).sub.3 1492 SO.sub.2 Cl OCH.sub.3 C(CH.sub.3).sub.3 1493 SO.sub.2 Br OCH.sub.3 C(CH.sub.3).sub.3 1494 SO.sub.2 NO.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1495 SO.sub.2 SCH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1496 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1497 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1498 SO.sub.2 CH.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1499 SO.sub.2 CF.sub.3 OCH.sub.3 C(CH.sub.3).sub.3 1500 SO.sub.2 OCHF.sub.2 OCH.sub.3 C(CH.sub.3).sub.3 1501 bond F OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1502 bond Cl OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1503 bond Br OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1504 bond NO.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1505 bond SCH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1506 bond SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1507 bond SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1508 bond CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1509 bond CF.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1510 bond OCHF.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1511 CH.sub.2 F OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1512 CH.sub.2 Cl OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1513 CH.sub.2 Br OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1514 CH.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1515 CH.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1516 CH.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1517 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1518 CH.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1519 CH.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1520 CH.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1521 O F OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1522 O Cl OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1523 O Br OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1524 O NO.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1525 O SCH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1526 O SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1527 O SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1528 O CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1529 O CF.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1530 O OCHF.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1531 S F OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1532 S Cl OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1533 S Br OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1534 S NO.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1535 S SCH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1536 S SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1537 S SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1538 S CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1539 S CF.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1540 S OCHF.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1541 SO.sub.2 F OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1542 SO.sub.2 Cl OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1543 SO.sub.2 Br OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1544 SO.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1545 SO.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1546 SO.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1547 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1548 SO.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1549 SO.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1550 SO.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 CH(CH.sub.3).sub.2 1551 bond F OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1552 bond Cl OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1553 bond Br OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1554 bond NO.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1555 bond SCH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1556 bond SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1557 bond SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1558 bond CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1559 bond CF.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1560 bond OCHF.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1561 CH.sub.2 F OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1562 CH.sub.2 Cl OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1563 CH.sub.2 Br OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1564 CH.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1565 CH.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1566 CH.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1567 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1568 CH.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1569 CH.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1570 CH.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1571 O F OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1572 O Cl OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1573 O Br OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1574 O NO.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1575 O SCH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1576 O SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1577 O SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1578 O CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1579 O CF.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1580 O OCHF.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1581 S F OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1582 S Cl OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1583 S Br OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1584 S NO.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1585 S SCH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1586 S SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1587 S SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1588 S CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1589 S CF.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1590 S OCHF.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1591 SO.sub.2 F OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1592 SO.sub.2 Cl OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1593 SO.sub.2 Br OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1594 SO.sub.2 NO.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1595 SO.sub.2 SCH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1596 SO.sub.2 SO.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1597 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1598 SO.sub.2 CH.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1599 SO.sub.2 CF.sub.3 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1600 SO.sub.2 OCHF.sub.2 OCH(CH.sub.3).sub.2 C(CH.sub.3).sub.3 1601 bond F OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1602 bond Cl OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1603 bond Br OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1604 bond NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1605 bond SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1606 bond SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1607 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1608 bond CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1609 bond CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1610 bond OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1611 CH.sub.2 F OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1612 CH.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1613 CH.sub.2 Br OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1614 CH.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1615 CH.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1616 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1617 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1618 CH.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1619 CH.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1620 CH.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1621 O F OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1622 O Cl OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1623 O Br OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1624 O NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1625 O SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1626 O SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1627 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1628 O CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1629 O CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1630 O OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1631 S F OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1632 S Cl OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1633 S Br OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1634 S NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1635 S SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1636 S SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1637 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1638 S CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1639 S CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1640 S OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1641 SO.sub.2 F OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1642 SO.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1643 SO.sub.2 Br OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1644 SO.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1645 SO.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1646 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1647 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1648 SO.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1649 SO.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1650 SO.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 CH(CH.sub.3).sub.2 1651 bond F OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1652 bond Cl OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1653 bond Br OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1654 bond NO.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1655 bond SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1656 bond SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1657 bond SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1658 bond CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1659 bond CF.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1660 bond OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1661 CH.sub.2 F OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1662 CH.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1663 CH.sub.2 Br OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1664 CH.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1665 CH.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1666 CH.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1667 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1668 CH.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1669 CH.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1670 CH.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1671 O F OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1672 O Cl OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1673 O Br OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1674 O NO.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1675 O SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1676 O SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1677 O SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1678 O CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1679 O CF.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1680 O OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1681 S F OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1682 S Cl OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1683 S Br OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1684 S NO.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1685 S SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1686 S SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3

1687 S SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1688 S CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1689 S CF.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1690 S OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1691 SO.sub.2 F OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1692 SO.sub.2 Cl OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1693 SO.sub.2 Br OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1694 SO.sub.2 NO.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1695 SO.sub.2 SCH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1696 SO.sub.2 SO.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1697 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1698 SO.sub.2 CH.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1699 SO.sub.2 CF.sub.3 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1700 SO.sub.2 OCHF.sub.2 OCH.sub.2C.sub.6H.sub.5 C(CH.sub.3).sub.3 1701 bond F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1702 bond Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1703 bond Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1704 bond NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1705 bond SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1706 bond SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1707 bond SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1708 bond CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1709 bond CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1710 bond OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1711 CH.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1712 CH.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1713 CH.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1714 CH.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1715 CH.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1716 CH.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1717 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1718 CH.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1719 CH.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1720 CH.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1721 O F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1722 O Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1723 O Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1724 O NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1725 O SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1726 O SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1727 O SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1728 O CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1729 O CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1730 O OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1731 S F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1732 S Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1733 S Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1734 S NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1735 S SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1736 S SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1737 S SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1738 S CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1739 S CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1740 S OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1741 SO.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1742 SO.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1743 SO.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1744 SO.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1745 SO.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1746 SO.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1747 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1748 SO.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1749 SO.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1750 SO.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) CH(CH.sub.3).sub.2 1751 bond F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1752 bond Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1753 bond Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1754 bond NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1755 bond SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1756 bond SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1757 bond SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1758 bond CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1759 bond CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1760 bond OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1761 CH.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1762 CH.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1763 CH.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1764 CH.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1765 CH.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1766 CH.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1767 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1768 CH.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1769 CH.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1770 CH.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1771 O F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1772 O Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1773 O Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1774 O NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1775 O SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1776 O SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1777 O SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1778 O CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1779 O CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1780 O OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1781 S F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1782 S Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1783 S Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1784 S NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1785 S SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1786 S SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1787 S SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1788 S CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1789 S CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1790 S OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1791 SO.sub.2 F OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1792 SO.sub.2 Cl OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1793 SO.sub.2 Br OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1794 SO.sub.2 NO.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1795 SO.sub.2 SCH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1796 SO.sub.2 SO.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1797 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1798 SO.sub.2 CH.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1799 SO.sub.2 CF.sub.3 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1800 SO.sub.2 OCHF.sub.2 OSO.sub.2(4-CH.sub.3--C.sub.6H.sub.4) C(CH.sub.3).sub.3 1801 bond F SCH.sub.3 CH(CH.sub.3).sub.2 1802 bond Cl SCH.sub.3 CH(CH.sub.3).sub.2 1803 bond Br SCH.sub.3 CH(CH.sub.3).sub.2 1804 bond NO.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1805 bond SCH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1806 bond SO.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1807 bond SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1808 bond CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1809 bond CF.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1810 bond OCHF.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1811 CH.sub.2 F SCH.sub.3 CH(CH.sub.3).sub.2 1812 CH.sub.2 Cl SCH.sub.3 CH(CH.sub.3).sub.2 1813 CH.sub.2 Br SCH.sub.3 CH(CH.sub.3).sub.2 1814 CH.sub.2 NO.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1815 CH.sub.2 SCH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1816 CH.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1817 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1818 CH.sub.2 CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1819 CH.sub.2 CF.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1820 CH.sub.2 OCHF.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1821 O F SCH.sub.3 CH(CH.sub.3).sub.2 1822 O Cl SCH.sub.3 CH(CH.sub.3).sub.2 1823 O Br SCH.sub.3 CH(CH.sub.3).sub.2 1824 O NO.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1825 O SCH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1826 O SO.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1827 O SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1828 O CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1829 O CF.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1830 O OCHF.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1831 S F SCH.sub.3 CH(CH.sub.3).sub.2 1832 S Cl SCH.sub.3 CH(CH.sub.3).sub.2 1833 S Br SCH.sub.3 CH(CH.sub.3).sub.2 1834 S NO.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1835 S SCH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1836 S SO.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1837 S SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1838 S CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1839 S CF.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1840 S OCHF.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1841 SO.sub.2 F SCH.sub.3 CH(CH.sub.3).sub.2 1842 SO.sub.2 Cl SCH.sub.3 CH(CH.sub.3).sub.2 1843 SO.sub.2 Br SCH.sub.3 CH(CH.sub.3).sub.2 1844 SO.sub.2 NO.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1845 SO.sub.2 SCH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1846 SO.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1847 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1848 SO.sub.2 CH.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1849 SO.sub.2 CF.sub.3 SCH.sub.3 CH(CH.sub.3).sub.2 1850 SO.sub.2 OCHF.sub.2 SCH.sub.3 CH(CH.sub.3).sub.2 1851 bond F SCH.sub.3 C(CH.sub.3).sub.3 1852 bond Cl SCH.sub.3 C(CH.sub.3).sub.3 1853 bond Br SCH.sub.3 C(CH.sub.3).sub.3 1854 bond NO.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1855 bond SCH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1856 bond SO.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1857 bond SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1858 bond CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1859 bond CF.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1860 bond OCHF.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1861 CH.sub.2 F SCH.sub.3 C(CH.sub.3).sub.3 1862 CH.sub.2 Cl SCH.sub.3 C(CH.sub.3).sub.3 1863 CH.sub.2 Br SCH.sub.3 C(CH.sub.3).sub.3 1864 CH.sub.2 NO.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1865 CH.sub.2 SCH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1866 CH.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1867 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1868 CH.sub.2 CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1869 CH.sub.2 CF.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1870 CH.sub.2 OCHF.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1871 O F SCH.sub.3 C(CH.sub.3).sub.3 1872 O Cl SCH.sub.3 C(CH.sub.3).sub.3 1873 O Br SCH.sub.3 C(CH.sub.3).sub.3 1874 O NO.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1875 O SCH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1876 O SO.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1877 O SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1878 O CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1879 O CF.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1880 O OCHF.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1881 S F SCH.sub.3 C(CH.sub.3).sub.3 1882 S Cl SCH.sub.3 C(CH.sub.3).sub.3 1883 S Br SCH.sub.3 C(CH.sub.3).sub.3 1884 S NO.sub.2 SCH.sub.3 C(CH.sub.3).sub.3

1885 S SCH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1886 S SO.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1887 S SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1888 S CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1889 S CF.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1890 S OCHF.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1891 SO.sub.2 F SCH.sub.3 C(CH.sub.3).sub.3 1892 SO.sub.2 Cl SCH.sub.3 C(CH.sub.3).sub.3 1893 SO.sub.2 Br SCH.sub.3 C(CH.sub.3).sub.3 1894 SO.sub.2 NO.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1895 SO.sub.2 SCH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1896 SO.sub.2 SO.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1897 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1898 SO.sub.2 CH.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1899 SO.sub.2 CF.sub.3 SCH.sub.3 C(CH.sub.3).sub.3 1900 SO.sub.2 OCHF.sub.2 SCH.sub.3 C(CH.sub.3).sub.3 1901 bond F Cl CH(CH.sub.3).sub.2 1902 bond Cl Cl CH(CH.sub.3).sub.2 1903 bond Br Cl CH(CH.sub.3).sub.2 1904 bond NO.sub.2 Cl CH(CH.sub.3).sub.2 1905 bond SCH.sub.3 Cl CH(CH.sub.3).sub.2 1906 bond SO.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1907 bond SO.sub.2CH.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1908 bond CH.sub.3 Cl CH(CH.sub.3).sub.2 1909 bond CF.sub.3 Cl CH(CH.sub.3).sub.2 1910 bond OCHF.sub.2 Cl CH(CH.sub.3).sub.2 1911 CH.sub.2 F Cl CH(CH.sub.3).sub.2 1912 CH.sub.2 Cl Cl CH(CH.sub.3).sub.2 1913 CH.sub.2 Br Cl CH(CH.sub.3).sub.2 1914 CH.sub.2 NO.sub.2 Cl CH(CH.sub.3).sub.2 1915 CH.sub.2 SCH.sub.3 Cl CH(CH.sub.3).sub.2 1916 CH.sub.2 SO.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1917 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1918 CH.sub.2 CH.sub.3 Cl CH(CH.sub.3).sub.2 1919 CH.sub.2 CF.sub.3 Cl CH(CH.sub.3).sub.2 1920 CH.sub.2 OCHF.sub.2 Cl CH(CH.sub.3).sub.2 1921 O F Cl CH(CH.sub.3).sub.2 1922 O Cl Cl CH(CH.sub.3).sub.2 1923 O Br Cl CH(CH.sub.3).sub.2 1924 O NO.sub.2 Cl CH(CH.sub.3).sub.2 1925 O SCH.sub.3 Cl CH(CH.sub.3).sub.2 1926 O SO.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1927 O SO.sub.2CH.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1928 O CH.sub.3 Cl CH(CH.sub.3).sub.2 1929 O CF.sub.3 Cl CH(CH.sub.3).sub.2 1930 O OCHF.sub.2 Cl CH(CH.sub.3).sub.2 1931 S F Cl CH(CH.sub.3).sub.2 1932 S Cl Cl CH(CH.sub.3).sub.2 1933 S Br Cl CH(CH.sub.3).sub.2 1934 S NO.sub.2 Cl CH(CH.sub.3).sub.2 1935 S SCH.sub.3 Cl CH(CH.sub.3).sub.2 1936 S SO.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1937 S SO.sub.2CH.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1938 S CH.sub.3 Cl CH(CH.sub.3).sub.2 1939 S CF.sub.3 Cl CH(CH.sub.3).sub.2 1940 S OCHF.sub.2 Cl CH(CH.sub.3).sub.2 1941 SO.sub.2 F Cl CH(CH.sub.3).sub.2 1942 SO.sub.2 Cl Cl CH(CH.sub.3).sub.2 1943 SO.sub.2 Br Cl CH(CH.sub.3).sub.2 1944 SO.sub.2 NO.sub.2 Cl CH(CH.sub.3).sub.2 1945 SO.sub.2 SCH.sub.3 Cl CH(CH.sub.3).sub.2 1946 SO.sub.2 SO.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1947 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl CH(CH.sub.3).sub.2 1948 SO.sub.2 CH.sub.3 Cl CH(CH.sub.3).sub.2 1949 SO.sub.2 CF.sub.3 Cl CH(CH.sub.3).sub.2 1950 SO.sub.2 OCHF.sub.2 Cl CH(CH.sub.3).sub.2 1951 bond F Cl C(CH.sub.3).sub.3 1952 bond Cl Cl C(CH.sub.3).sub.3 1953 bond Br Cl C(CH.sub.3).sub.3 1954 bond NO.sub.2 Cl C(CH.sub.3).sub.3 1955 bond SCH.sub.3 Cl C(CH.sub.3).sub.3 1956 bond SO.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1957 bond SO.sub.2CH.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1958 bond CH.sub.3 Cl C(CH.sub.3).sub.3 1959 bond CF.sub.3 Cl C(CH.sub.3).sub.3 1960 bond OCHF.sub.2 Cl C(CH.sub.3).sub.3 1961 CH.sub.2 F Cl C(CH.sub.3).sub.3 1962 CH.sub.2 Cl Cl C(CH.sub.3).sub.3 1963 CH.sub.2 Br Cl C(CH.sub.3).sub.3 1964 CH.sub.2 NO.sub.2 Cl C(CH.sub.3).sub.3 1965 CH.sub.2 SCH.sub.3 Cl C(CH.sub.3).sub.3 1966 CH.sub.2 SO.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1967 CH.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1968 CH.sub.2 CH.sub.3 Cl C(CH.sub.3).sub.3 1969 CH.sub.2 CF.sub.3 Cl C(CH.sub.3).sub.3 1970 CH.sub.2 OCHF.sub.2 Cl C(CH.sub.3).sub.3 1971 O F Cl C(CH.sub.3).sub.3 1972 O Cl Cl C(CH.sub.3).sub.3 1973 O Br Cl C(CH.sub.3).sub.3 1974 O NO.sub.2 Cl C(CH.sub.3).sub.3 1975 O SCH.sub.3 Cl C(CH.sub.3).sub.3 1976 O SO.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1977 O SO.sub.2CH.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1978 O CH.sub.3 Cl C(CH.sub.3).sub.3 1979 O CF.sub.3 Cl C(CH.sub.3).sub.3 1980 O OCHF.sub.2 Cl C(CH.sub.3).sub.3 1981 S F Cl C(CH.sub.3).sub.3 1982 S Cl Cl C(CH.sub.3).sub.3 1983 S Br Cl C(CH.sub.3).sub.3 1984 S NO.sub.2 Cl C(CH.sub.3).sub.3 1985 S SCH.sub.3 Cl C(CH.sub.3).sub.3 1986 S SO.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1987 S SO.sub.2CH.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1988 S CH.sub.3 Cl C(CH.sub.3).sub.3 1989 S CF.sub.3 Cl C(CH.sub.3).sub.3 1990 S OCHF.sub.2 Cl C(CH.sub.3).sub.3 1991 SO.sub.2 F Cl C(CH.sub.3).sub.3 1992 SO.sub.2 Cl Cl C(CH.sub.3).sub.3 1993 SO.sub.2 Br Cl C(CH.sub.3).sub.3 1994 SO.sub.2 NO.sub.2 Cl C(CH.sub.3).sub.3 1995 SO.sub.2 SCH.sub.3 Cl C(CH.sub.3).sub.3 1996 SO.sub.2 SO.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1997 SO.sub.2 SO.sub.2CH.sub.2CH.sub.3 Cl C(CH.sub.3).sub.3 1998 SO.sub.2 CH.sub.3 Cl C(CH.sub.3).sub.3 1999 SO.sub.2 CF.sub.3 Cl C(CH.sub.3).sub.3 2000 SO.sub.2 OCHF.sub.2 Cl C(CH.sub.3).sub.3

[0186] Very particular preference is also given to the compounds of the formula Ia2 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sub.3, l=1), in particular to the compounds Ia2.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR15##

[0187] Very particular preference is also given to the compounds of the formula Ia3 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3.dbd.CH.sub.3, l=1), in particular to the compounds Ia3.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR16##

[0188] Very particular preference is also given to the compounds of the formula Ia4 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sub.3, l=2), in particular to the compounds Ia4.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR17##

[0189] Very particular preference is also given to the compounds of the formula Ia5 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sub.3, l=1), in particular to the compounds Ia5.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR18##

[0190] Very particular preference is also given to the compounds of the formula Ia6 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sub.3, l=2), in particular to the compounds Ia6.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR19##

[0191] Very particular preference is also given to the compounds of the formula Ia7 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia7.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR20##

[0192] Very particular preference is also given to the compounds of the formula Ia8 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sup.3, l=1), in particular to the compounds Ia8.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR21##

[0193] Very particular preference is also given to the compounds of the formula Ia9 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia9.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR22##

[0194] Very particular preference is also given to the compounds of the formula Ia10 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia10.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR23##

[0195] Very particular preference is also given to the compounds of the formula Ia11 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia11.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR24##

[0196] Very particular preference is also given to the compounds of the formula Ia12 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia12.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR25##

[0197] Very particular preference is also given to the compounds of the formula Ia13 (=Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia13.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR26##

[0198] Very particular preference is also given to the compounds of the formula Ia14 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sub.3, l=1), in particular to the compounds Ia14.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR27##

[0199] Very particular preference is also given to the compounds of the formula Ia15 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sub.3, l=1), in particular to the compounds Ia15.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR28##

[0200] Very particular preference is also given to the compounds of the formula Ia16 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia16.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR29##

[0201] Very particular preference is also given to the compounds of the formula Ia17 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia17.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR30##

[0202] Very particular preference is also given to the compounds of the formula Ia18 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.13=CH.sub.3, l=1), in particular to the compounds Ia18.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR31##

[0203] Very particular preference is also given to the compounds of the formula Ia19 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia19.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR32##

[0204] Very particular preference is also given to the compounds of the formula Ia20 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia20.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR33##

[0205] Very particular preference is also given to the compounds of the formula Ia21 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, l=0), in particular to the compounds Ia21.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR34##

[0206] Very particular preference is also given to the compounds of the formula Ia22 (.ident.Ia where R.sup.1, R.sup.2, R.sup.5 and R.sup.12=H, R.sup.3=CH.sub.3, l=1), in particular to the compounds Ia22.n, where the variables X, R.sup.4, R.sup.10 and R.sup.11 are as defined in Table 1. ##STR35##

[0207] The tricyclic benzoylpyrazole derivatives of the formula I can be obtained by various routes, for example by one of the following processes: [0208] A. Preparation of compounds of the formula I where R.sup.10=halogen by reacting a tricyclic benzoylpyrazole derivative of the formula I.alpha. (.ident.I where R.sup.10=hydroxyl) with a halogenating agent: ##STR36## [0209] Suitable halogenating agents are, for example, phosgene, diphosgene, triphosgene, thionyl chloride, oxalyl chloride, phosphorus oxychloride, phosphorus pentachloride, mesyl chloride, chloromethylene-N,N-dimethylammonium chloride, oxalyl bromide, phosphorus oxybromide, etc. [0210] The starting materials are generally employed in equimolar amounts. However, it may also be advantageous to employ an excess of one or the other component. [0211] Suitable solvents are, for example, chlorinated hydrocarbons, such as methylene chloride or 1,2-dichloroethane, aromatic hydrocarbons, for example toluene, xylene or chlorobenzene, polar aprotic solvents, such as acetonitrile, dimethylformamide or dimethyl sulfoxide, or mixtures of these. However, it is also possible to carry out the reaction in the absence of solvent. [0212] The reaction temperature is generally in the range from 0.degree. C. to the boiling point of the reaction mixture. [0213] Work-up can be carried out in a manner known per se to afford the product. [0214] B. Preparation of compounds of the formula I where R.sup.10=OR.sup.13, by reacting a tricyclic benzoylpyrazole derivative of the formula I.alpha. (.ident.I where R.sup.10=hydroxyl) with an alkylating agent III. ##STR37## [0215] L.sup.1 is a nucleophilically replaceable leaving group, such as halogen, for example chlorine or bromine, hetaryl, for example imidazolyl, carboxylate, for example acetate, or sulfonate, for example mesylate or triflate, etc. [0216] The compounds of the formula III can be employed directly, such as, for example, in the case of the carbonyl halides, or be generated in situ, for example activated carboxylic acids (using carboxylic acid and dicyclohexylcarbodiimide etc.). [0217] The starting materials are generally employed in equimolar amounts. However, it may also be advantageous to employ an excess of one or the other component. [0218] If appropriate, it may also be advantageous to carry out the reaction in the presence of a base. Here, the reactants and the base are advantageously employed in equimolar amounts. In certain cases, an excess of base, for example from 1.5 to 3 molar equivalents, may be advantageous. [0219] Suitable bases are tertiary alkylamines, such as triethylamine, aromatic amines, such as pyridine, alkali metal carbonates, for example sodium carbonate or potassium carbonate, alkali metal bicarbonates, for example sodium bicarbonate and potassium bicarbonate, alkali metal alkoxides, such as sodium methoxide, sodium ethoxide, potassium tert-butoxide, or alkali metal hydrides, for example sodium hydride. Preference is given to using triethylamine or pyridine. [0220] Suitable solvents are, for example, chlorinated hydrocarbons, such as methylene chloride or 1,2-dichloroethane, aromatic hydrocarbons, for example toluene, xylene or chlorobenzene, ethers, such as diethyl ether, methyl tert-butyl ether, tetrahydrofuran or dioxane, polar aprotic solvents, such as acetonitrile, dimethylformamide or dimethyl sulfoxide, or esters, such as ethyl acetate, or mixtures of these. [0221] The reaction temperature is generally in the range from 0.degree. C. to the boiling point of the reaction mixture. [0222] Work-up can be carried out in a manner known per se to afford the product. [0223] C. Preparation of compounds of the formula I where R.sup.10=OR.sup.13, SR.sup.13, NR.sup.15R.sup.16 or N-bonded heterocyclyl by reacting compounds of the formula I.beta. (.ident.I where R.sup.10=halogen) with a compound of the formula IV.alpha., IV.beta., IV.gamma. or IV.delta., if appropriate in the presence of a base or with prior formation of salt. ##STR38## [0224] The starting materials are generally employed in equimolar amounts. However, it may also be advantageous to employ an excess of one or the other component. [0225] If appropriate, it may also be advantageous to carry out the reaction in the presence of a base. Here, the reactants and the base are advantageously employed in equimolar amounts. An excess of base, for example from 1.5 to 3 molar equivalents, based on I.beta. (where R.sup.10=halogen), may be advantageous in certain cases. [0226] Suitable bases are tertiary alkylamines, such as triethylamine, aromatic amines, such as pyridine, alkali metal carbonates, for example sodium carbonate or potassium carbonate, alkali metal bicarbonates, for example sodium bicarbonate and potassium bicarbonate, alkali metal alkoxides, such as sodium methoxide, sodium ethoxide, potassium tert-butoxide, or alkali metal hydrides, for example sodium hydride. Preference is given to using sodium hydride or potassium tert-butoxide. [0227] Suitable solvents are, for example, chlorinated hydrocarbons, such as methylene chloride or 1,2-dichloroethane, aromatic hydrocarbons, for example toluene, xylene or chlorobenzene, ethers, such as diethyl ether, methyl tert-butyl ether, tetrahydrofuran or dioxane, polar aprotic solvents, such as acetonitrile, dimethylformamide or dimethyl sulfoxide, or mixtures of these. [0228] The reaction temperature is generally in the range from 0.degree. C. to the boiling point of the reaction mixture. [0229] Work-up can be carried out in a manner known per se to afford the product. [0230] D. Preparation of compounds of the formula I where R.sup.10=SO.sub.2R.sup.14 by reacting compounds of the formula I where R.sup.10=SR.sup.10 (I.gamma.) with an oxidizing agent. ##STR39## [0231] Suitable oxidizing agents are, for example, m-chloroperbenzoic acid, peroxyacetic acid, trifluoroperoxyacetic acid, hydrogen peroxide, if appropriate in the presence of a catalyst, such as tungstate. [0232] The starting materials are generally employed in equimolar amounts. However, it may also be advantageous to employ an excess of one or the other component. [0233] Suitable solvents are, for example, chlorinated hydrocarbons, such as methylene chloride or 1,2-dichloroethane, aromatic hydrocarbons, for example, toluene, xylene or chlorobenzene, ethers, such as diethyl ether, methyltert-butyl ether, tetrahydrofuran or dioxane, polar aprotic solvents, such as acetonitrile or dimethylformamide, or esters, such as ethyl acetate, or mixtures of these. [0234] The reaction temperature is generally in the range from 0.degree. C. to the boiling point of the reaction mixture. [0235] Work-up can be carried out in a manner known per se to afford the product. [0236] E. Preparation of compounds of the formula I where R.sup.9=IIa (where R.sup.10+ hydroxyl or mercapto) by reacting a metalated pyrazole derivative of the formula V with a tricyclic benzoic acid derivative of the formula VI.alpha.: ##STR40## [0237] Here, M is a metal, in particular an alkali metal, such as lithium or sodium, an alkaline earth metal, such as, for example, magnesium, or a transition metal, such as palladium, nickel, etc. and L.sup.2 is a nucleophilically replaceable leaving group, such as halogen, for example chlorine or bromine, alkylsulfonate, such as mesylate, haloalkylsulfonate, such as triflate, or cyanide. [0238] The reaction is generally carried out at temperatures of from -100.degree. C. to the reflux temperature of the reaction mixture. Suitable solvents are inert aprotic solvents, such as ethers, for example diethyl ether, tetrahydrofuran. The compounds of the formula VI.alpha. are generally employed in excess, but it may also be advantageous to employ them in equimolar amounts or in substoichiometric amounts. Work-up is carried out to afford the product. [0239] The metalated pyrazole derivatives of the formula V can be formed in a manner known per se by reacting pyrazoles which are halogenated in the 4-position with metals, such as lithium, sodium, magnesium, etc., or with organometallic compounds, such as, for example, butyllithium. However, it is also possible to metalate pyrazoles which are linked in the 4 position to hydrogen directly, for example with the abovementioned metals or organometallic compounds. The reactions are generally carried out in an inert aprotic solvent, preferably in ether, such as diethyl ether, tetrahydrofuran, etc. The reaction temperature is in the range from -100.degree. C. to the boiling point of the reaction mixture. The compounds of the formula V are generally directly reacted further or generated in situ. [0240] F. Preparation of compounds of the formula I.alpha. (.ident.I where R.sup.10=hydroxyl) by reacting an activated tricyclic benzoic acid of the formula VI.beta. or a tricyclic benzoic acid VI.gamma., preferably activated in situ, with a pyrazole of the formula VII to give the acylation product, followed by rearrangement. ##STR41##

[0241] L.sup.3 is a nucleophilically replaceable leaving group, such as halogen, for example bromine or chlorine, hetaryl, for example imidazolyl or pyridyl, carboxylate, for example acetate or trifluoroacetate, etc.

[0242] The activated tricyclic benzoic acid VI.beta. can be employed directly, such as in the case of the tricyclic benzoyl halides, or be generated in situ, for example using dicyclohexylcarbodiimide, triphenylphosphine/azodicarboxylic ester, 2-pyridine disulfide/triphenylphosphine, carbonyldiimidazole, etc.

[0243] If appropriate, it may be advantageous to carry out the acylation reaction in the presence of a base. Here, the reactants and the auxiliary base are advantageously employed in equimolar amounts. A slight excess of auxiliary base, for example from 1.2 to 1.5 molar equivalents, based on VI, may be advantageous in certain cases.

[0244] Suitable auxiliary bases are tertiary alkylamines, pyridine, or alkali metal carbonates. Suitable solvents are, for example, chlorinated hydrocarbons, such as methylene chloride or 1,2-dichloroethane, aromatic hydrocarbons, such as toluene, xylene or chlorobenzene, ethers, such as diethyl ether, methyl tert-butyl ether, tetrahydrofuran or dioxane, polar aprotic solvents, such as acetonitrile, dimethylformamide or dimethyl sulfoxide, or esters, such as ethyl acetate, or mixtures of these.

[0245] If tricyclic benzoyl halides are employed as activated carboxylic acid components, it may be advantageous to cool the reaction mixture to 0-10.degree. C. when adding this reaction partner. The mixture is subsequently stirred at 20-100.degree. C., preferably at 25-50.degree. C., until the reaction has gone to completion. Work-up is carried out in a customary manner, for example by pouring the reaction mixture into water and extracting the product of value. Solvents which are suitable for this purpose are, in particular, methylene chloride, diethyl ether and ethyl acetate. The organic phase is dried and the solvent removed, and the crude ester can then be employed for the rearrangement without further purification.

[0246] The rearrangement of the esters VIII to give the compounds of the formula I.alpha. is advantageously carried out at from 20 to 100.degree. C. in a solvent and in the presence of a base and, if appropriate, using a cyano compound as catalyst.

[0247] Solvents which may be used are, for example, acetonitrile, methylene chloride, 1,2-dichloroethane, dioxane, ethyl acetate, toluene or mixtures of these. Preferred solvents are acetonitrile and dioxane.

[0248] Suitable bases are tertiary amines, such as triethylamine, aromatic amines, such as pyridine, or alkali metal carbonates, such as sodium carbonate or potassium carbonate, which are preferably employed in equimolar amounts or in an up to four-fold excess, based on the ester. Preference is given to using triethylamine or alkali metal carbonate, preferably in double the equimolar ratio, based on the ester.

[0249] Suitable cyano compounds are inorganic cyanides, such as sodium cyanide or potassium cyanide, and organic cyano compounds, such as acetone cyanohydrin or trimethylsilyl cyanide. They are employed in an amount of from 1 to 50 mol percent, based on the ester. Preference is given to using acetone cyanohydrin or trimethylsilyl cyanide, for example in an amount of from 5 to 15, preferably 10, mol percent, based on the ester.

[0250] Work-up may be carried out in a manner known per se. The reaction mixture is, for example, acidified using dilute mineral acid, such as 5% strength hydrochloric acid or sulfuric acid, and extracted with an organic solvent, for example methylene chloride or ethyl acetate. The organic extract can be extracted with 5-10% strength alkali metal carbonate solution, for example sodium carbonate or potassium carbonate solution. The aqueous phase is acidified and the resulting precipitate is filtered off with suction and/or extracted with methylene chloride or ethyl acetate, the extract being dried and concentrated.

[0251] However, it is also possible to generate the ester VIII in situ by reacting a pyrazole of the formula VII, or an alkali metal salt thereof, with a tricyclic benzene derivative of the formula IX in the presence of carbon monoxide, a catalyst and a base. ##STR42##

[0252] L.sup.4 is a leaving group, such as halogen, for example chlorine, bromine or iodine, or sulfonate such as mesylate or triflate; preference is given to bromine or triflate.

[0253] If appropriate, the ester VIII reacts directly to give the tricyclic benzoylpyrazole derivative of the formula I.alpha..

[0254] Suitable catalysts are palladium ligand complexes in which the palladium is present in oxidation state 0, metallic palladium, if appropriate applied to a support, and preferably palladium(II) salts. The reaction with palladium(II) salts and metallic palladium is preferably carried out in the presence of complex ligands.

[0255] A suitable palladium(0) ligand complex is, for example, tetrakis(triphenylphosphane)palladium.

[0256] Metallic palladium is preferably applied to an inert carrier, such as, for example, activated carbon, silica, alumina, barium sulfate or calcium carbonate. The reaction is preferably carried out in the presence of complex ligands, such as, for example, triphenylphosphane.

[0257] Suitable palladium(II) salts are, for example, palladium acetate and palladium chloride. Preference is given to carrying out the reaction in the presence of complex ligands such as, for example, triphenylphosphane.

[0258] Suitable complex ligands for the palladium ligand complexes, or complex ligands in whose presence the reaction with metallic palladium or palladium(II) salts is preferably carried out are tertiary phosphanes whose structure is represented by the following formulae: ##STR43## where n is a number from 1 to 4 and the radicals R.sup.a to R.sup.g are C.sub.1-C.sub.6-alkyl, aryl-C.sub.1-C.sub.2-alkyl or preferably aryl. Aryl is, for example, naphthyl and unsubstituted or substituted phenyl such as, for example, 2-tolyl and in particular unsubstituted phenyl.

[0259] The complex palladium salts can be prepared in a manner known per se starting from commercially available palladium salts, such as palladium chloride or palladium acetate, and the corresponding phosphanes, such as, for example, triphenylphosphane or 1,2-bis(diphenylphosphano)ethane. A large number of complexed palladium salts is also commercially available. Preferred palladium salts are [(R)-(+)-2,2'-bis(diphenylphosphano)-1,1'-binaphthyl]palladium(II) chloride, bis(triphenylphosphane)palladium(II) acetate and in particular bis(triphenylphosphane)palladium(II) chloride.

[0260] The palladium catalyst is generally employed in a concentration of from 0.05 to 5 mol %, and preferably of 1-3 mol %.

[0261] Suitable bases are tertiary amines, such as, for example, N-methylpiperidine, ethyldiisopropylamine, 1,8-bisdimethylaminonaphthalene and in particular triethylamine. Also suitable are alkali metal carbonates, such as sodium carbonate or potassium carbonate. However, mixtures of potassium carbonate and triethylamine are also suitable.

[0262] In general, from 2 to 4 molar equivalents, in particular 2 molar equivalents, of the alkali metal carbonate, and from 1 to 4 molar equivalents, in particular 2 molar equivalents, of the tertiary amine are employed, based on the tricyclic benzene derivative of the formula IX.

[0263] Suitable solvents are nitrites, such as benzonitrile and acetonitrile, amides, such as dimethylformamide, dimethylacetamide, tetra-C.sub.1-C.sub.4-alkylureas or N-methylpyrrolidone, and preferably ethers, such as tetrahydrofuran, methyl tert-butyl ether. Particular preference is given to using, as solvents, ethers such as 1,4-dioxane and dimethoxyethane.

[0264] The tricyclic benzoyl halides of the formula VI.beta. where L.sup.3=Cl, Br can be prepared in a manner known per se by reacting the tricyclic benzoic acids of the formula VI.gamma. (.ident.VIb) with halogenating agents such as thionyl chloride, thionyl bromide, phosgene, diphosgene, triphosgene, oxalyl chloride and oxalyl bromide.

[0265] In a known manner, the tricyclic benzoic acids of the formula VI.gamma. (.ident.VIb) can be prepared by acidic or basic hydrolysis from the corresponding esters VIc.

[0266] Tricyclic benzoic acid derivatives of the formula VI ##STR44## where: [0267] X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7, NR.sup.8 or a bond; [0268] Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated 5- or 6-membered heterocycle which contains one to three identical or different heteroatoms selected from the following group: oxygen, sulfur or nitrogen; [0269] R.sup.1, R.sup.2, R.sup.6, R.sup.7 are hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0270] R.sup.3 is halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0271] R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)-aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl) amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; [0272] R.sup.5 is hydrogen, C.sub.1-C.sub.6-alkyl or halogen; [0273] R.sup.8 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkylcarbonyl, formyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.1-C.sub.6-haloalkoxycarbonyl, C.sub.1-C.sub.6-alkylsulfonyl or C.sub.1-C.sub.6-haloalkylsulfonyl; [0274] l is 0, 1 or 2; [0275] R.sup.17 is hydroxyl or a radical which can be removed by hydrolysis; are novel.

[0276] Examples of radicals which can be removed by hydrolysis are alkoxy, phenoxy, alkylthio and phenylthio radicals which can be unsubstituted or substituted, halides, heteroaryl radicals which are attached via nitrogen, amino and imino radicals which may be unsubstituted or substituted, etc.

[0277] Preference is given to tricyclic benzoyl halides VIa (VI where R.sup.17=halogen) ##STR45## where the variables X, Y, R.sup.1 to R.sup.5 and l are as defined under formula VI and [0278] Hal is halogen, in particular chloride or bromide.

[0279] Preference is also given to tricyclic benzoic acids of the formula VIb (VI where R.sup.17=hydroxyl; .ident.VI.gamma.), ##STR46## where the variables X, Y, R.sup.1 to R.sup.5 and l are as defined under formula VI.

[0280] Preference is also given to tricyclic benzoic esters of the formula VIc (VI where R.sup.17=T=C.sub.1-C.sub.6-alkoxy), ##STR47## where the variables X, Y, R.sup.1 to R.sup.5 and l are as defined under formula VI and [0281] T is C.sub.1-C.sub.6-alkoxy.

[0282] With respect to the variables X, Y, R.sup.1 to R.sup.5 and l, the particularly preferred embodiments of the tricyclic benzoic acid derivatives of the formulae VI, VIa, VIb and VIc correspond to those of the tricyclic benzoylpyrazole derivatives of the formula I.

[0283] Particular preference is given to the compounds VI, VIa, VIb and VIc where Y together with the two carbons to which it is attached forms the following heterocycles: ##STR48##

[0284] Here, extraordinary preference is given to the compounds VI, VIa, VIb and VIc where [0285] R.sup.4 is nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; in particular C.sub.1-C.sub.6-alkylsulfonyl.

[0286] The tricyclic benzoic esters VIc can be obtained in different ways.

[0287] For example, benzoic esters of the formula X, which are prepared in a manner known per se (cf., for example, Chem. Pharm. Bull. 1985, 33 (8), 3336; Helv. Chim. Acta 1987, 70, 1326; J. Chem. Soc. Perkin Trans. 1972, 2019; J. Chem. Soc. Perkin Trans. 1991, 2763; Tetrahydron Asymmetry 1998, 9, 1137), can be cyclized to cyclic ketones of the formula XI (cf., for example, Chem. Ber. 1923, 56, 1819; J. Chem. Soc. Perkin 11991, 2763; J. Med. Chem. 1988, 31, 230; Tetrahedron 1987, 43, 4549; Synlett 1991, 6, 443; Chem. Pharm. Bull. 1985, 33 (8), 3336). Analogously to known processes (cf., for example, J. Heterocyclic Chem. 1976, 13, 545; J. Heterocyclic Chem. 1972, 9, 1341; J. Org. Chem. 1978, 43, 3015; J. Chem. Soc. Perkin Trans. I 1978, 86; J. Org. Chem. 1986, 51, 2021), these can be converted into the tricyclic benzoic esters of the formula VIc. ##STR49##

[0288] Furthermore, it may be suitable to cyclize the cyclic ketone of the formula XI in a manner known per se (XII), for example using an anhydride or acid anhydride, if appropriate in the presence of catalytic amounts of a Lewis acid, such as boron trifluoride (cf., for example, Can. J. Chem. 1979, 57, 3292; J. Am. Chem. Soc. 1953, 75, 626), followed by reaction with a hydrazine (cf. A. R. Katritzky et al., Comprehensive Heterocyclic Chemistry, Vol. 5, p. 121, 277-280 (1984), Pergamon Press; J. Org. Chem. 1961, 26, 451; Org. Synth. 1949, 29, 54), where the resulting pyrazole radical can be modified further by customary processes.

[0289] Furthermore, the diketone XII can be reacted with hydroxylamine or equivalents thereof (cf. A. R. Katritzky et al., Comprehensive Heterocyclic Chemistry, Vol. 6, p. 61-64, 118 (1984), Pergamon Press; Chem. Ber. 1967, 100, 3326). This gives the corresponding isoxazole derivatives which can be modified further by customary processes.

[0290] It is also possible to react the diketone XII with amidines (cf., for example, A. R. Katritzky et al., Comprehensive Heterocyclic Chemistry, Vol. 3, p. 112-114 (1924), Pergamon Press; J. Chem. Soc. C 1967, 1922; Org. Synth. 1963, IV, 182). If required, the resulting pyrimidine derivatives can be modified further by customary processes. ##STR50##

[0291] In the reactA123ions mentioned above, it is also possible to employ, instead of the diketone XII, equivalents thereof, such as enol ethers or enamines, which can be prepared analogously to known processes.

[0292] It may also be possible to react the cyclic ketone of the formula XI analogously to known processes with an aldehyde or ketone to give (XIII) (cf., for example, Tetrahedron Lett. 1978, 2111; Tetrahedron Lett. 1981, 5251; Chem. Ber. 1960, 2294; J. Chem. Soc. Perkin Trans. 1, 1991, 1467; Tetrahedron Lett. 1992, 8091). The resulting unsaturated cyclic ketone of the formula XIII can be reacted with a hydrazine in a manner known per se (cf., for example, A. R. Katritzky et al. Comprehensive Heterocyclic Chemistry, Vol. 2, 6 (1984), Pergamon Press; J. Heterocyclic Chem. 1969, 533; J. Heterocyclic Chem. 1968, 853), where the resulting pyrazoline can be modified further by customary processes.

[0293] It is furthermore possible to react the unsaturated cyclic ketone of the formula XIII with hydroxylamine or equivalents thereof (Z. Chem. 1980, 20, 19). This gives the corresponding isoxazoline derivatives, which can be modified further by customary processes. ##STR51##

[0294] Furthermore, it is possible to convert aldehydes of the formula XIV, which can be prepared in a manner known per se, analogously to processes known from the literature by reaction with a hydrazine or hydroxylamine (or equivalents of these) into the corresponding hydrazones or oximes (cf., for example, Synth. Commun. 1990, 20, 1373; J. Org. Chem. 1980, 45, 3756). These in turn can be converted in a manner known per se into the corresponding 1,3-dipoles, which then react in a [3+2]-cycloaddition to give the compounds VIc (cf., for example, Synth. Commun. 1990, 20, 1373; EP-A 386 892; J. Org. Chem. 1980, 45, 3756; Tetrahedron Lett. 1981, 22, 1333.)

[0295] The resulting pyrazoles or pyrazolines and isoxazoles or isoxazolines can be modified further by customary processes. ##STR52##

[0296] It is also possible to react the cyclic ketone of the formula XI with a dithiol or a "mixed alcohol" analogously to processes known from the literature (cf., for example, T. W. Greene et al., Protective Groups in Organic Synthesis, John Wiley & Sons, 133-140), and to subject it subsequently to a rearrangement in the presence of bromine or a suitable Lewis acid, such as, for example, tellurium tetrachloride (cf. Tetrahedron 1991, 47, 4187; Synthesis 1991, 223; J. Chem. Soc. Chem. Commun. 1985, 1645). ##STR53##

[0297] The resulting heterocycles can, if desired, be modified further by processes known per se.

[0298] The abovementioned substitutents R.sup.3a are hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, hydroxyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; furthermore, the abovementioned radicals R.sup.3b are hydrogen, C.sub.1-C.sub.6-alkyl or C.sub.1-C.sub.6-haloalkyl.

[0299] The tricyclic benzoic esters of the formula VIc or the tricyclic benzoic acids of the formula VIb can be obtained by reacting a tricyclic benzene derivative of the formula IX with a C.sub.1-C.sub.6-alcohol or water in the presence of carbon monoxide, a catalyst and a base. In general, the conditions mentioned under process F apply. ##STR54##

[0300] L.sup.4 is a leaving group, such as halogen, for example chlorine, bromine or iodine, or sulfate, such as mesylate or triflate; preference is given to bromine or triflate.

[0301] Furthermore, the tricyclic benzoic acids of the formula VIb can be obtained by converting a tricyclic benzene derivative of the formula IX where L.sup.4 is halogen, such as chlorine or bromine, in particular bromine, by reaction with, for example, n-butyllithium or magnesium into the metalated derivative, followed by quenching with carbon dioxide (cf., for example, J. Org. Chem. 1990, 55, 773; Angew. Chem. Int. Ed. 1969, 8, 68). ##STR55##

[0302] It is also possible to obtain the tricyclic benzoic acids VIb by hydrolyzing the corresponding nitrites, analogously to processes known from the literature. The nitriles for their part can be obtained by halogen/nitrile exchange or by Sandmeyer reaction from the corresponding anilines XV. ##STR56##

[0303] The compounds of the formula IX,

where:

[0304] X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7, NR.sup.8 or a bond; [0305] Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated 5- or 6-membered heterocycle which contains one to three identical or different heteroatoms selected from the following group: oxygen, sulfur or nitrogen; [0306] R.sup.1, R.sup.2, R.sup.6, R.sup.7 are hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0307] R.sup.3 is halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0308] R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl)amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl) amino; [0309] R.sup.5 is hydrogen, C.sub.1-C.sub.6-alkyl or halogen; [0310] R.sup.8 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkylcarbonyl, formyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.1-C.sub.6-haloalkoxycarbonyl, C.sub.1-C.sub.6-alkylsulfonyl or C.sub.1-C.sub.6-haloalkylsulfonyl; [0311] l is 0, 1 or 2; [0312] L.sup.4 is halogen, C.sub.1-C.sub.6-alkylsulfonyloxy, C.sub.1-C.sub.6-haloalkylsulfonyloxy or phenylsulfonyloxy, where the phenyl ring of the lastmentioned radical may be unsubstituted or partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; are novel.

[0313] Preference is given to compounds of the formula IX where L.sup.4 is halogen, in particular bromine.

[0314] The particularly preferred embodiments of the compounds of the formula IX with respect to the variables X, Y, R.sup.1 to R.sup.5 and l correspond to those of the tricyclic benzoylpyrazole derivatives of the formula I.

[0315] Particular preference is given to the compounds of the formula IX where [0316] Y together with the two carbons to which it is attached forms the following heterocycles: ##STR57##

[0317] Here, extraordinary preference is given to the compounds IX where [0318] R.sup.4 is nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; in particular C.sub.1-C.sub.6-alkylsulfonyl.

[0319] The compounds of the formula IX can be obtained in different ways, the fused system, for example, can be constructed analogously to the processes described for the compounds of the formula VIc.

[0320] However, it is also possible to construct the fused system from a suitable parent compound (analogously to the processes described for compounds of the formula VIc) and to introduce L.sup.4=halogen subsequently by customary halogenating reactions.

[0321] The anilines of the formula XV and the nitriles of the formula XVI ##STR58## where: [0322] X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7, NR.sup.8 or a bond; [0323] Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated 5- or 6-membered heterocycle which contains one to three identical or different heteroatoms selected from the following group: oxygen, sulfur or nitrogen; [0324] R.sup.1, R.sup.2, R.sup.6, R.sup.7 are hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0325] R.sup.3 is halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; [0326] R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl) amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; [0327] R.sup.5 is hydrogen, C.sub.1-C.sub.6-alkyl or halogen; [0328] R.sup.8 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkylcarbonyl, formyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.1-C.sub.6-haloalkoxycarbonyl, C.sub.1-C.sub.6-alkylsulfonyl or C.sub.1-C.sub.6-haloalkylsulfonyl; [0329] l is 0, 1 or 2; are also novel.

[0330] The particularly preferred embodiments of the compounds of the formulae XV and XVI with respect to the variables X, Y, R.sup.1 to R.sup.5 and l correspond to those of the tricyclic benzoylpyrazole derivatives of the formula I.

[0331] Particular preference is given to the compounds of the formula XV or XVI where [0332] Y together with the two carbons to which it is attached forms the following heterocycles: ##STR59##

[0333] Here, extraordinary preference is given to the compounds XV or XVI where [0334] R.sup.4 is nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; in particular C.sub.1-C.sub.6-alkylsulfonyl.

[0335] The compounds of the formula XV can be obtained in different ways; for example, the fused system can be constructed analogously to the processes described for the compounds of the formula VIc.

[0336] However, it is also possible to construct the fused system from a suitable parent compound (analogously to the processes described for the compounds of the formula VIc) and to introduce a nitro group subsequently by nitration para to R.sup.4, analogously to processes known from the literature, and to convert this group in a manner known per se by reduction into the amino group.

[0337] If appropriate, it may be advantageous in the synthesis variants described above to introduce protective groups for certain functionalities if the functionalities are not compatible with the reaction conditions required.

[0338] The selection of the protective groups depends both on the reaction conditions and on the structure of the molecule. The protective groups, their introduction and their removal are generally known from the literature (cf., for example, T. W. Greene et al., "Protective Groups in Organic Synthesis", 2.sup.nd edition, Wiley, New York, 1991), and they can be employed analogously to processes known from the literature.

[0339] Furthermore, it may be necessary to carry out a combination of the synthesis variants described above.

[0340] It is also possible to introduce further substitutents or to modify the substitutents present by electrophilic, nucleophilic, free-radical or organometallic reactions and by oxidation or reduction reactions.

PREPARATION EXAMPLES

1. (5-Phenylcarbonyloxy-1-methyl-1H-pyrazol-4-yl)-(8-methyl-sulfonyl-3a,4-- dihydro-3H-indeno[1,2-c]isoxazol-5-yl)methanone (compound 2.2)

2-Allyl-6-chlorobenzaldehyde

[0341] Under an atmosphere of protective gas, a solution of 10.89 g (0.107 mol) of trimethylethylenediamine in 50 ml of anhydrous tetrahydrofuran was cooled to -10.degree. C. and admixed dropwise with 66.6 ml of a 1.6 molar solution of n-butyllithium in hexane (0.107 mol). After 10 minutes, 15 g (0.107 mol) of 6-chlorobenzaldehyde in 70 ml of tetrahydrofuran were added dropwise, and the mixture was admixed with a further 0.214 mol of n-butyllithium in hexane (146.8 ml) and stirred at 0.degree. C. for 2.5 hours. The mixture was cooled to -20.degree. C., 12.42 g (0.139 mol) of copper(I) cyanide were added, the mixture was stirred at -10.degree. C. for 30 minutes, and 28.42 g of allyl bromide in 100 ml of tetrahydrofuran were then added dropwise. The mixture was stirred at 0.degree. C. for another 2.5 hours, and 230 ml of saturated ammonium chloride solution were then added dropwise. The resulting solid was separated off and the aqueous phase was extracted with diethyl ether. The combined organic phases were then washed with saturated ammonium chloride solution and dried, and the solvent was removed under reduced pressure. This gave 17.0 g of 2-allyl-6-chlorobenzaldehyde (89%) in the form of a dark oil.

[0342] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.73 (d, 2H); 5.05 (dd, 2H); 5.96 (m, 1H); 7.05-7.48 (m, 3H); 10.58 (s, 1H).

2-Allyl-6-chlorobenzaldehyde oxime

[0343] 5.58 g of sodium bicarbonate were added to a solution of 4.62 g of hydroxylamine hydrochloride in 50 ml of water, and the mixture was cooled to 0.degree. C. A solution of 9.7 g (44.32 mmol) of 2-allyl-6-chlorobenzaldehyde in 50 ml of methanol was then added dropwise, and the mixture was stirred at room temperature overnight. The methanol was subsequently removed under reduced pressure and the residue was stirred into 300 ml of water. The aqueous phase was extracted with diethyl ether and the combined organic phases were washed with saturated ammonium chloride solution and dried, and the solvent was removed. This gave 8.7 g (quantitative) of 2-allyl-6-chlorobenzaldehyde oxime in the form of a viscous oil.

[0344] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.58 (d, 2H); 5.02 (2d, 2H); 5.95 (m, 1H); 7.08-7.36 (m, 3H); 8.49 (s, 1H).

8-Chloro-3a,4-dihydro-3H-indeno[1,2-c]isoxazole

[0345] At room temperature, 37.0 ml of a sodium hypochlorite solution (12.5% of active chlorine) were added dropwise to a solution of 8.4 g (42.9 mmol) of 2-allyl-6-chlorobenzaldehyde oxime in 100 ml of methylene chloride, and a spatula tip of sodium acetate was added. The mixture was stirred at room temperature for 2 hours, the organic phase was separated off, the aqueous phase was extracted with methylene chloride and the combined organic phases were washed with saturated ammonium chloride solution. The organic phase was dried and the solvent was removed. This gave 7.0 g (94%) of 8-chloro-3a,4-dihydro-3H-indeno-[1,2-c]isoxazole in the form of a viscous oil.

[0346] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 2.81 (dd, 1H); 3.24 (dd, 1H); 3.78-4.03 (s, 2H); 4.78 (t, 1H); 7.23-7.41 (m, 3H).

8-Methylthio-3a,4-dihydro-3H-indeno[1,2c]isoxazole

[0347] At room temperature, 3.6 g (52.0 mmol) of sodium thiomethoxide were added to a solution of 5.0 g (25.8 mmol) of 8-chloro-3a,4-dihydro-3H-indeno-[1,2-c]isoxazole in 60 ml of N-methylpyrrolidone, and the mixture was stirred overnight. The mixture was subsequently stirred into 800 ml of water, the aqueous phase was extracted with diethyl ether, the combined organic phases were washed with saturated ammonium chloride solution and dried, and the solvent was removed. This gave 4.6 g (87%) of 8-methylthio-3a,4-dihydro-3H-indeno[1,2-c]isoxazole in the form of a dark brown solid.

[0348] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 2.54 (s, 3H); 2.78 (dd, 1H); 3.21 (dd, 1H); 3.72-3.93 (s, 2H); 4.64 (t, 1H); 7.09-7.38 (m, 3H).

5-Bromo-8-methylthio-3a,4-dihydro-3H-indeno[1,2-c]isoxazole

[0349] 120 ml of sulfuric acid (98 percent strength) were cooled to 0.degree. C., and 11.2 g (54.8 mmol) of 8-methylthio-3a,4-dihydro-3H-indeno[1,2-c]isoxazole were added a little at a time. 9.2 g (57.5 mmol) of bromine were then added dropwise, and stirring was continued at 0.degree. C. for another 2 hours. The resulting solution was poured into 2 l of a mixture of water and ice, this mixture was stirred for 1.5 hours and the precipitated solid was filtered off with suction and then washed and dried. This gave 11.4 g (73%) of 5-bromo-8-methylthio-3a,4-dihydro-3H-indeno[1,2-c]isoxazole of a brown solid having a m.p. of 127-135.degree. C.

[0350] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 2.53 (s, 3H); 2.71 (dd, 1H); 3.24 (dd, 1H); 3.81-4.02 (s, 2H); 4.71 (t, 1H); 7.01 (d, 1H); 7.47 (d, 1H).

5-Bromo-8-methylsulfonyl-3a,4-dihydro-3H-indeno[1,2-c]-isoxazole

[0351] A solution of 11.2 g (39.4 mmol) of 5-bromo-8-methylthio-3a,4-dihydro-3H-indeno[1,2-c]isoxazole and 1.55 g of sodium tungstate in 250 ml of toluene and 50 ml of glacial acetic acid was heated to 70.degree. C. and mixed dropwise with 10.73 g (39 percent strength, 86.8 mmol) of hydrogen peroxide. Stirring was continued at 70.degree. C. for another 3 hours, and a solid precipitated out. The mixture was allowed to cool to room temperature and stirred into 1 l of water, and the white solid was filtered off with suction. The organic phase of the filtrate was separated off and the aqueous phase was extracted with ethyl acetate. The combined organic phases were washed with water and dried, and the solvent was removed. This gave a viscous brown oil which was stirred with hexane/ethyl acetate (4:1). The resulting precipitate was filtered off with suction and combined with the solid obtained above. This gave 7.3 g (59%) of 5-bromo-8-methylsulfonyl-3a,4-dihydro-3H-indeno[1,2-c]-isoxazole.

[0352] .sup.1H-NMR (d.sup.6-DMSO, .delta. in ppm): 2.93 (dd, 1H); 3.23 (dd, 1H); 3.41 (s, 3H); 3.94 (dd, 1H); 4.16 (m, 1H); 4.81 (t, 1H); 7.82 (d, 1H); 8.03 (d, 1H).

(5-Hydroxy-1-methyl-1H-pyrazol-4-yl)-(8-methylsulfonyl-3a,4-dihydro-3H-ind- eno[1,2-c]isoxazol-5-yl)methanone (compound 2.1)

[0353] 0.62 g (6.33 mmol) of 5-hydroxy-1-methylpyrazole, 1.75 g (12.66 mmol) of dry potassium carbonate, 1.28 g (12.67 mmol) of triethylamine and 0.22 g (0.30 mmol) of bis-(triphenylphosphane)palladium dichloride were added to a suspension of 2.0 g (6.33 mmol) of 5-bromo-8-methylsulfonyl-3a,4-dihydro-3H-indeno[1,2-c]-isoxazole in 100 ml of dioxane. In a miniautoclave, a carbon monoxide pressure of 20 bar was applied, the mixture was stirred for 5 minutes and the autoclave was vented. This procedure was repeated 3 times. The autoclave was subsequently heated to 130.degree. C., a carbon monoxide pressure of 20 bar was applied once more and the mixture was stirred for 24 hours. After cooling and venting, the solvent was removed, and the residue was taken up in water, adjusted to pH 11 and washed with methylene chloride. The mixture was subsequently acidified to pH 4 using 10 percent strength hydrochloric acid and extracted with methylene chloride. The combined organic phases were washed with saturated ammonium chloride solution and dried, and the solvent was removed. This gave 0.58 g (25%) of (5-hydroxy-1-methyl-1H-pyrazol-4-yl)-(8-methylsulfonyl-3a,4-dihydro-3H-in- deno[1,2-c]isoxazole)-methanone in the form of a dark oil.

[0354] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.03 (dd, 1H); 3.42 (s, 3H); 3.40 (m, 1H); 3.51 (s, 3H); 4.05 (m, 2H); 4.85 (t, 1H); 7.57 (s, 1H); 7.92 (d, 1H); 8.22 (d, 1H).

(5-Phenylcarbonyloxy-1-methyl-1H-pyrazol-4-yl)-(8-methylsulfonyl-3a,4-dihy- dro-3H-indeno[1,2-c]isoxazol-5-yl)methanone (compound 2.2)

[0355] Under an atmosphere of protective gas, 0.18 g of triethylamine and 0.26 g (1.82 mmol) of benzoyl chloride in 10 ml of tetrahydrofuran were added at 0.degree. C. to a suspension of 0.55 g (1.52 mmol) of (5-hydroxy-1-methyl-1H-pyrazol-4-yl)-(8-methylsulfonyl-3a,4-dihydro-3H-in- deno[1,2-c]-isoxazol-5-yl)methanone in 10 ml of tetrahydrofuran. The mixture was stirred overnight at room temperature, the solvent was removed, the residue was taken up in ethyl acetate, washed with water and dried, and the solvent was removed. The crude product was purified by silica gel chromatography (mobile phase: ethyl acetate:hexane=1:1). This gave 0.22 g (31%) of (5-phenylcarbonyloxy-1-methyl-1H-pyrazol-4-yl)-(8-methylsulfonyl-3a,4-dih- ydro-3H-indeno[1,2-c]isoxazol-5-yl)methanone in the form of a yellow solid having a m.p. of 86-93.degree. C.

[0356] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.22 (s, 3H); 3.34 (m, 2H); 3.81 (s, 3H); 3.98 (m, 2H); 4.81 (t, 1H); 7.20-8.21 (m, 8H).

2. 4-(2-Methyl-9-chloro-[1]-thiochromano[4,3-c]pyrazol-6-yl)carbonyl-5-hyd- roxy-1-methyl-1H-pyrazole (compound 3.1)

Methyl 2-chlorosulfonyl-4-chlorobenzoate

[0357] At from 0 to 5.degree. C., a solution of 60.9 g (0.88 mol) of sodium nitrite in 100 ml of water was added dropwise to a solution of 139 g (0.75 mol) of methyl 2-amino-4-chlorobenzoate in 400 ml of concentrated hydrochloric acid and the mixture was stirred at 0.degree. C. for another hour.

[0358] In a second apparatus, 3 g of copper(II) chloride, 3 g of benzyltriethylammonium chloride, 10 ml of water and 400 ml of 1,2-dichloroethane were combined and 64 g (1 mol) of sulfur dioxide were introduced.

[0359] The diazonium salt described above was subsequently added at from 10 to 15.degree. C., and the mixture was slowly heated to 50.degree. C. A further 54 g (0.84 mol) of sulfur dioxide were then introduced, and stirring was continued at 50.degree. C. for another 30 minutes. After cooling, 7.4 g (0.1 mol) of chlorine gas were then introduced at room temperature, stirring was continued for 15 minutes and the phases which had formed were then separated. The organic phase was dried and the solvent was removed. This gave 207 g of methyl 2-chlorosulfonyl-4-chlorobenzoate.

[0360] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 4.00 (s, 3H); 7.75 (m, 2H); 8.18 (m, 1H)

Methyl 2-mercapto-4-chlorobenzoate

[0361] Over a period of 1.5 hours, 243.5 g (3.7 mol) of zinc powder were added a little at a time to a suspension of 205 g (0.75 mol) of methyl 2-chlorosulfonyl-4-chlorobenzoate in 1 l of concentrated hydrochloric acid and 375 g of ice. The mixture was stirred for another 3 hours and slowly heated to 70.degree. C. After 2 hours at this temperature, the mixture was cooled. The reaction mixture was allowed to stand at room temperature for 12 hours and then extracted with ethyl acetate, the combined organic phases were dried and the solvent was removed. This gave 125.4 g (83%) of methyl 2-mercapto-4-chlorobenzoate.

[0362] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.95 (s, 3H); 4.88 (s, 1H); 7.10 (m, 1H); 7.30 (m, 1H); 7.96 (d, 1H).

Methyl 2-(2-hydroxycarbonyleth-1-yl)thio-4-chlorobenzoate

[0363] 179.5 g (1.3 mol) of potassium carbonate and, a little at a time, 94.5 g (0.62 mol) of 3-bromopropionic acid were added to a solution of 125.4 g (0.62 mol) of methyl 2-mercapto-4-chlorobenzoate in 1.5 l of acetone, and the reaction mixture was stirred at room temperature for 12 hours. The solvent was distilled off, the residue was taken up in water and the mixture was extracted with diethyl ether. The aqueous phase was then made acidic using concentrated hydrochloric acid, and the resulting precipitate was filtered off with suction and dried. This gave 150 g (88%) of methyl 2-(2-hydroxycarbonyleth-1-yl)thio-4-chlorobenzoate.

[0364] M.p.: 133 to 136.degree. C.

Methyl 5-chloro-4-oxothiochromane-8-carboxylate

[0365] At 70.degree. C., 50 g (0.18 mol) of methyl 2-(2-hydroxycarbonyleth-1-yl)thio-4-chlorobenzoate were added to 500 g of polyphosphoric acid, and the mixture was stirred for a further 30 minutes. The reaction mixture was then stirred into water and the resulting precipitate was filtered off with suction and dried. This gave 41.1 g (88%) of methyl 5-chloro-4-oxothiochromane-8-carboxylate.

[0366] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.08 (m, 4H); 3.96 (s, 3H); 7.14 (d, 1H); 7.95 (d, 1H).

Methyl 5-chloro-3-(N,N-dimethylaminomethylidene)-4-oxothiochromane-8-carbo- xylate

[0367] 30 g (0.078 mol) of methyl 5-chloro-4-oxothiochromane-8-carboxylate in 300 ml of N,N-dimethylformamide dimethyl acetal were refluxed for 6 hours. Volatile components were then distilled off, the residue was taken up in methylene chloride and the organic phase washed with water. Drying and removal of the solvent gave 35.3 g (97%) of methyl 5-chloro-3-(N,N-dimethylaminomethylidene)-4-oxothiochromane-8-carboxylate- .

[0368] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.18 (s, 6H); 3.80 (s, 2H); 3.95 (s, 3H); 7.24 (d, 1H); 7.64 (s, 1H); 7.82 (d, 1H).

2-Methyl-6-methoxycarbonyl-9-chloro-[1]-thiochromano[4,3-c]-pyrazole

[0369] 1.3 g (29.2 mmol) of methylhydrazine were added dropwise to a solution of 7.0 g (22.5 mmol) of methyl 5-chloro-3-(N,N-dimethylaminomethylidene)-4-oxothiochromane-8-carboxylate in 700 ml of ethanol, and the mixture was refluxed for 2 hours. The solvent was removed and the residue was chromatographed over silica gel using ethyl acetate/cyclohexane (2:3) as mobile phase. This gave 4.0 g (60%) of 2-methyl-6-methoxycarbonyl-9-chloro-[1]-thiochromano[4,3-c]pyraz- ole.

[0370] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.76 (s, 2H); 3.95 (s, 3H); 4.00 (s, 3H); 7.24 (s, 1H); 7.36 (d, 1H); 7.70 (d, 1H).

2-Methyl-6-hydroxycarbonyl-9-chloro-[1]-thiochromano[4,3-c]pyrazole

[0371] 4.0 g (13.6 mmol) of 2-methyl-6-methoxycarbonyl-9-chloro-[1]-thiochromano[4,3-c]pyrazole in 100 ml of methanol/water (1:1) were refluxed with 0.8 g (20 mmol) of sodium hydroxide for 1 hour. The organic solvent was removed under reduced pressure and the residue was extracted with ethyl acetate. The aqueous phase was acidified using concentrated hydrochloric acid and the resulting precipitate was filtered off with suction and dried. This gave 3.5 g (92%) of 2-methyl-6-hydroxycarbonyl-9-chloro-[1]-thiochromano[4,3-c]-pyrazole

[0372] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.80 (s, 2H); 3.96 (s, 3H); 7.40 (d, 1H); 7.65 (m, 2H).

4-(2-Methyl-9-chloro-[1]-thiochromano[4,3-c]pyrazol-6-yl)-carbonyl-5-hydro- xy-1-methyl-1H-pyrazole (compound 3.1)

[0373] A mixture of 0.60 g (2.1 mmol) of 2-methyl-6-hydroxycarbonyl-9-chloro-[1]-thiochromano[4,3-c]-pyrazole and 0.21 g (2.1 mmol) of N,N-dicyclohexylcarbodiimide in 20 ml of acetonitrile was stirred at room temperature overnight. The mixture was admixed with in each case 500 ml of ethyl acetate and 2% strength sodium carbonate solution, the resulting precipitate was filtered off, the organic phase was dried and the solvent was removed. The residue was then refluxed with 0.59 g (4.3 mmol) of potassium carbonate in 5 ml of 1,4-dioxane for 3 hours. After cooling, the mixture was extracted with diethyl ether and the aqueous phase was acidified to pH 3. The resulting precipitate was filtered off with suction and dried. This gave 0.14 g of 4-(2-methyl-9-chloro-[1]-thiochromano[4,3-c]pyrazol-6-yl)-carbonyl-5-hydr- oxy-1-methyl-1H-pyrazole.

[0374] M.p.: 168-171.degree. C.

3. (5-Hydroxy-1-methyl-1H-pyrazol-4-yl)-(6-methoxy-3a,4-dihydro-3H-chromen- o[4,3-c]isoxazolin-9-yl)methanone (compound 2.3)

Methyl 2-hydroxy-3-formyl-4-methoxybenzoate

[0375] At from 0 to 5.degree. C., a solution of 209.0 g (1.1 mol) of titanium tetrachloride in 150 ml of methylene chloride was added dropwise to a solution of 50.1 g (0.275 mol) of methyl 2-hydroxy-4-methoxybenzoate and 88 g (0.725 mol) of dichloromethoxymethane in 400 ml of methylene chloride, and the mixture was stirred at room temperature overnight. The mixture was then stirred into ice-water and extracted with methylene chloride. The combined organic phases were washed with sodium bicarbonate solution, water and sodium chloride solution and dried, and the solvent was then removed. Silica gel chromatography using cyclohexane/ethyl acetate=1:1 gave 24.5 g (42%) of methyl 2-hydroxy-3-formyl-4-methoxybenzoate in the form of a colorless solid of m.p.: 123-124.degree. C.

[0376] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.92 (s, 3H); 3.98 (s, 3H); 6.49 (d, 1H); 8.19 (d, 1H); 10.39 (s, 1H).

Methyl 2-allyloxy-3-formyl-4-methoxybenzoate

[0377] At room temperature, 23.2 g (0.192 mol) of allyl bromide were added dropwise to a mixture of 21.0 g (0.375 mol) of potassium hydroxide and 20.2 g (0.096 mol) of methyl 2-hydroxy-3-formyl-4-methoxybenzoate in 500 ml of dimethyl sulfoxide, and the mixture was stirred at room temperature for 4 hours. The mixture was subsequently stirred into 1.5 l of 3% strength aqueous hydrochloric acid and extracted with ethyl acetate. The combined organic phases were washed with water and dried, and the solvent was removed. Silica gel chromatography using cyclohexane/ethyl acetate=1:2 gave 7.7 g (36%) of methyl 2-allyloxy-3-formyl-4-methoxybenzoate in the form of a yellowish oil.

[0378] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.86 (s, 3H); 3.93 (s, 3H); 4.58 (d, 2H); 5.32 (d, 1H); 5.39 (d, 1H); 6.15 (m, 1H); 6.79 (d, 1H); 8.04 (d, 1H); 10.41 (s, 1H).

6-Methoxy-9-methoxycarbonyl-3a,4-dihydro-3H-chromeno[4,3-c]isoxazoline

[0379] Step a)

[0380] At room temperature, 4.6 g (18.4 mmol) of methyl 2-allyloxy-3-formyl-4-methoxybenzoate in 70 ml of methanol were added dropwise to a solution of 2.25 g (32.3 mmol) of hydroxylammonium chloride and 2.7 g of pyridine in 70 ml of water. The mixture was stirred at room temperature overnight, 150 ml of water were added, the mixture was extracted with methylene chloride, the combined organic phases were washed with 3% strength aqueous hydrochloric acid and dried, and the solvent was removed. The resulting oxime has a melting point of 126-129.degree. C.

[0381] Step b)

[0382] This oxime was reacted further without any further purification by dissolving it in 40 ml of methylene chloride, followed by dropwise addition of 15.0 ml (25.0 mmol) of sodium hypochlorite solution (12.5% of active chlorine). A spatula tip of sodium acetate was added and the mixture was stirred at room temperature for 12 hours. The organic phase was separated off, the aqueous phase was extracted with methylene chloride, the combined organic phases were washed with water and dried, and the solvent was removed. Silica gel chromatography using cyclohexane/ethyl acetate=1:1 gave 2.2 g (49%) of 6-methoxy-9-methoxycarbonyl-3a,4-dihydro-3H-chromeno[4,3-c]-isoxazoline in the form of a colorless solid of m.p: 199-203.degree. C.

[0383] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.84 (s, 3H); 3.98 (s, 3H); 3.8-4.0 (m, 2H); 4.16 (dt, 1H); 4.63 (t, 1H); 4.84 (dd, 1H); 6.61 (d, 1H); 7.93 (d, 1H).

6-Methoxy-9-hydroxycarbonyl-3a,4-dihydro-3H-chromeno[4,3-c]isoxazoline

[0384] At room temperature, a solution of 0.8 g (20.0 mmol) of sodium hydroxide in 7 ml of water was added dropwise to a solution of 2.1 g (8.0 mmol) of 6-methoxy-9-methoxycarbonyl-3a,4-dihydro-3H-chromeno[4,3-c]isoxa- zoline in 40 ml of methanol, and the mixture was refluxed for 6 hours. After cooling, the solvent was removed and the residue was taken up in about 50 ml of water and washed with methylene chloride. The aqueous phase was subsequently acidified using 10% strength hydrochloric acid (pH=1-2), and the precipitate was filtered off with suction, washed with water and dried at 60.degree. C. This gave 1.7 g (86%) of 6-methoxy-9-hydroxycarbonyl-3a,4-dihydro-3H-chromeno[4,3-c]-isoxazoline in the form of colorless crystals.

[0385] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.73 (dd, 1H); 3.89 (s, 3H); 3.84-3.95 (m, 1H); 4.11 (dd, 1H); 4.54 (dd, 1H); 4.79 (dd, 1H); 6.61 (d, 1H); 7.81 (d, 1H).

(5-Hydroxy-1-methyl-1H-pyrazol-4-yl)-(6-methoxy-3a,4-dihydro-3H-chromeno[4- ,3-c]isoxazolin-9-yl)methanone (compound 2.3)

[0386] Step a)

[0387] At room temperature, 0.26 g (2.2 mmol) of thionyl chloride and a drop of dimethylformamide were added to a solution of 0.50 g (2.0 mmol) of 6-methoxy-9-hydroxycarbonyl-3a,4-dihydro-3H-chromeno[(4,3-c)]isoxazoli- ne in 30 ml of carbon tetrachloride, and the mixture was stirred at 40-50.degree. C. for 3 hours. The solvent was subsequently removed under reduced pressure. This gave, in quantitative yield, 6-methoxy-9-chloroformyl-3a,4-dihydro-3H-chromeno[4,3-c]isoxazoline (0.54 g) as a brownish oil.

[0388] Step b)

[0389] 0.54 g (2 mmol) of 6-methoxy-9-chloroformyl-3a,4-dihydro-3H-chromeno[4,3-c]isoxazoline was dissolved in 30 ml of acetonitrile and, at 0.degree. C., added dropwise to a solution of 0.2 g (2.0 mmol) of 1-methyl-5-hydroxypyrazole and 0.6 g (6.0 mmol) of triethylamine in 20 ml of acetonitrile. The mixture was stirred at room temperature overnight, the solvent was removed, and the residue was taken up in methylene chloride and washed with water. The solution was dried and the solvent was distilled off. The residue was dissolved in 30 ml of dioxane and admixed with 0.42 g (3.0 mmol) of potassium carbonate, and the mixture was refluxed for 7 hours. After cooling, the solvent was distilled off under reduced pressure, the residue was taken up in water and the solution was adjusted to pH=1 using 10% strength hydrochloric acid. The solution was extracted with methylene chloride, the combined organic phases were dried and the solvent was subsequently removed. This gave 0.45 g (68%) of (5-hydroxy-1-methyl-1H-pyrazol-4-yl)-(6-methoxy-3a,4-dihydro-3H-chromeno[- 4,3-c]isoxazolin-9-yl)methanone of m.p. 236-238.degree. C.

[0390] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 3.66 (s, 3H); 3.84-4.2 (m, 2H); 4.02 (s, 3H); 4.12 (dd, 1H); 4.63-4.77 (m, 2H); 6.68 (d, 1H); 7.24 (s, 1H); 7.61 (d, 1H).

4. [5-Hydroxy-1-(1,1-dimethyleth-1-yl)-1H-pyrazol-4-yl]-[6-methoxy-3a,4-di- hydro-3H-chromeno[4,3-c]isoxazolin-9-yl]methanone (compound 2.4)

[0391] 0.54 g (2 mmol) of 6-methoxy-9-chloroformyl-3a,4-dihydro-3H-chromeno[4,3-c]-isoxazoline was dissolved in 30 ml of acetonitrile and, at 0.degree. C., added dropwise to a solution of 0.28 g (2.0 mmol) of 1-(1,1-dimethyleth-1-yl)-5-hydroxy-1H-pyrazole and 0.6 g (6.0 mmol) of triethylamine in 20 ml of acetonitrile. The mixture was stirred at room temperature overnight, the solvent was removed, and the residue was taken up in methylene chloride and washed with water. The solution was dried, and the solvent was distilled off. The residue was dissolved in 30 ml of dioxane and admixed with 0.42 g (3.0 mmol) of potassium carbonate, and the mixture was refluxed for 7 hours. After cooling, the solvent was distilled off under reduced pressure, the residue was taken up in water and the solution was adjusted to pH=1 using 10% strength hydrochloric acid. The solution was extracted with methylene chloride, the combined organic phases were dried, and the solvent was subsequently removed. This gave 0.3 g (40%) of [5-hydroxy-1-(1,1-dimethyleth-1-yl)-1H-pyrazol-4-yl]-[6-methoxy-3a,4-dihy- dro-3H-chromeno[4,3-c]isoxazolin-9-yl]methanone having a melting point of 223.degree. C.-225.degree. C.

[0392] .sup.1H NMR (CDCl.sub.3, .delta. in ppm): 1.64 (s, 9H); 3.8-4.2 (m, 6H); 4.6-4.8 (m, 2H); 6.68 (d, 1H); 7.44 (s, 1H); 7.62 (d, 1H).

[0393] In addition to the compounds above, other tricyclic benzoylpyrazole derivatives of the formula I which were prepared or are preparable in a similar manner are listed in Tables 2 to 5: TABLE-US-00002 TABLE 2 ##STR60## physical data (m.p. [.degree. C.]; No. X R.sup.4 R.sup.10 R.sup.11 R.sup.12 .sup.1H NMR [ppm]) 2.1 Bond SO.sub.2CH.sub.3 OH CH.sub.3 H 3.03 (dd, 1H); 3.42 (s, 3H); 3.51 (s, 3H); 4.05 (m, 2H); 4.85 (t, 1H); 7.57 (s, 1H); 7.92 (d, 1H); 8.22 (d, 1H) 2.2 Bond SO.sub.2CH.sub.3 OCOC.sub.6H.sub.5 CH.sub.3 H 3.22 (s, 3H); 3.34 (m, 2H); 3.81 (s, 3H); 3.98 (m, 2H); 4.81 (t, 1H); 7.20-8.21 (m, 8H); 2.3 O OCH.sub.3 OH CH.sub.3 H 236-238 2.4 O OCH.sub.3 OH C(CH.sub.3).sub.3 H 223-225 2.5 O OCH.sub.3 OCO (3-F--C.sub.6H.sub.4) CH.sub.3 H oil

[0394] TABLE-US-00003 TABLE 3 ##STR61## No. X R.sup.4 R.sup.10 R.sup.11 R.sup.12 physical data (m.p.[.degree. C]) 3.1 S Cl OH CH.sub.3 H 168-171 3.2 S Cl OH CH.sub.2CH.sub.3 H 115 3.3 S SCH.sub.3 OH CH.sub.3 H 245 3.4 S SCH.sub.3 OH CH.sub.2CH.sub.3 H 222

[0395] TABLE-US-00004 TABLE 4 ##STR62## physical data (m.p. [.degree. C.]; No. X R.sup.4 R.sup.10 R.sup.11 R.sup.12 .sup.1H NMR [ppm]) 4.1 S Cl OH CH.sub.3 H 180.degree. C. 4.2 S Cl OH CH.sub.2CH.sub.3 H 112.degree. C.

[0396] TABLE-US-00005 TABLE 5 ##STR63## physical data (m.p. [.degree. C.]; Nr. X R.sup.4 R.sup.10 R.sup.11 R.sup.12 .sup.1H NMR [ppm]) 5.1 O SCH.sub.3 OH CH.sub.3 H 201

[0397] The compounds of the formula I and their agriculturally useful salts are suitable, both in the form of isomer mixtures and in the form of the pure isomers, as herbicides. The herbicidal compositions comprising compounds of the formula I control vegetation on non-crop areas very efficiently, especially at high rates of application. They act against broad-leaved weeds and grass weeds in crops such as wheat, rice, maize, soya and cotton without causing any significant damage to the crop plants. This effect is mainly observed at low rates of application.

[0398] Depending on the application method in question, the compounds of the formula I, or herbicidal compositions comprising them, can additionally be employed in a further number of crop plants for eliminating undesirable plants. Examples of suitable crops are the following:

[0399] Allium cepa, Ananas comosus, Arachis hypogaea, Asparagus officinalis, Beta vulgaris spec. altissima, Beta vulgaris spec. rapa, Brassica napus var. napus, Brassica napus var. napobrassica, Brassica rapa var. silvestris, Camellia sinensis, Carthamus tinctorius, Carya illinoinensis, Citrus limon, Citrus sinensis, Coffea arabica (Coffea canephora, Coffea liberica), Cucumis sativus, Cynodon dactylon, Daucus carota, Elaeis guineensis, Fragaria vesca, Glycine max, Gossypium hirsutum, (Gossypium arboreum, Gossypium herbaceum, Gossypium vitifolium), Helianthus annuus, Hevea brasiliensis, Hordeum vulgare, Humulus lupulus, Ipomoea batatas, Juglans regia, Lens culinaris, Linum usitatissimum, Lycopersicon lycopersicum, Malus spec., Manihot esculenta, Medicago sativa, Musa spec., Nicotiana tabacum (N. rustica), Olea europaea, Oryza sativa, Phaseolus lunatus, Phaseolus vulgaris, Picea abies, Pinus spec., Pisum sativum, Prunus avium, Prunus persica, Pyrus communis, Ribes sylvestre, Ricinus communis, Saccharum officinarum, Secale cereale, Solanum tuberosum, Sorghum bicolor (s. vulgare), Theobroma cacao, Trifolium pratense, Triticum aestivum, Triticum durum, Vicia faba, Vitis vinifera and Zea mays.

[0400] In addition, the compounds of the formula I may also be used in crops which tolerate the action of herbicides owing to breeding, including genetic engineering methods.

[0401] The compounds of the formula I, or the herbicidal compositions comprising them, can be used for example in the form of ready-to-spray aqueous solutions, powders, suspensions, also highly-concentrated aqueous, oily or other suspensions or dispersions, emulsions, oil dispersions, pastes, dusts, materials for broadcasting, or granules, by means of spraying, atomizing, dusting, spreading or watering. The use forms depend on the intended purpose; in any case, they should guarantee the finest possible distribution of the active compounds according to the invention.

[0402] The herbicidal compositions comprise a herbicidally effective amount of at least one compound of the formula I or an agriculturally useful salt of I and auxiliaries which are customarily used for formulating crop protection agents.

[0403] Suitable for use as inert auxiliaries are essentially the following:

[0404] mineral oil fractions of medium to high boiling point, such as kerosene and diesel oil, furthermore coal-tar oils and oils of vegetable or animal origin, aliphatic, cyclic and aromatic hydrocarbons, for example paraffin, tetrahydronaphthalene, alkylated naphthalenes and their derivatives, alkylated benzenes or their derivatives, alcohols such as methanol, ethanol, propanol, butanol and cyclohexanol, ketones such as cyclohexanone, strongly polar solvents, for example amines such as N-methylpyrrolidone, and water.

[0405] Aqueous use forms can be prepared from emulsion concentrates, suspensions, pastes, wettable powders or water-dispersible granules by adding water. To prepare emulsions, pastes or oil dispersions, the tricyclic benzoylpyrazole derivatives of the formula I, either as such or dissolved in an oil or solvent, can be homogenized in water by means of a wetting agent, tackifier, dispersant or emulsifier. Alternatively, it is possible to prepare concentrates comprising active compound, wetting agent, tackifier, dispersant or emulsifier and, if desired, solvent or oil, which are suitable for dilution with water.

[0406] Suitable surfactants are the alkali metal salts, alkaline earth metal salts and ammonium salts of aromatic sulfonic acids, e.g. ligno-, phenol-, naphthalene- and dibutylnaphthalenesulfonic acid, and of fatty acids, alkyl- and alkylarylsulfonates, alkyl sulfates, lauryl ether sulfates and fatty alcohol sulfates, and salts of sulfated hexa-, hepta- and octadecanols, and also of fatty alcohol glycol ethers, condensates of sulfonated naphthalene and its derivatives with formaldehyde, condensates of naphthalene or of the naphthalenesulfonic acids with phenol and formaldehyde, polyoxyethylene octylphenol ether, ethoxylated isooctyl-, octyl- or nonylphenol, alkylphenyl or tributylphenyl polyglycol ether, alkylaryl polyether alcohols, isotridecyl alcohol, fatty alcohol/ethylene oxide condensates, ethoxylated castor oil, polyoxyethylene alkyl ethers or polyoxypropylene alkyl ethers, lauryl alcohol polyglycol ether acetate, sorbitol esters, lignin-sulfite waste liquors or methylcellulose.

[0407] Powders, materials for broadcasting and dusts can be prepared by mixing or grinding the active compounds together with a solid carrier.

[0408] Granules, e.g. coated granules, impregnated granules and homogeneous granules, can be prepared by binding the active compounds to solid carriers. Solid carriers are mineral earths such as silicas, silica gels, silicates, talc, kaolin, limestone, lime, chalk, bole, loess, clay, dolomite, diatomaceous earth, calcium sulfate, magnesium sulfate and magnesium oxide, ground synthetic materials, fertilizers such as ammonium sulfate, ammonium phosphate, ammonium nitrate and ureas, and products of vegetable origin, such as cereal meal, tree bark meal, wood meal and nutshell meal, cellulose powders, or other solid carriers.

[0409] The concentrations of the compounds of the formula I in the ready-to-use preparations can be varied within wide ranges. In general, the formulations comprise approximately from 0.001 to 98% by weight, preferably 0.01 to 95% by weight, of at least one active compound. The active compounds are employed in a purity of from 90% to 100%, preferably 95% to 100% (according to NMR spectrum).

[0410] The following formulation examples illustrate the preparation of such formulations: [0411] I. 20 parts by weight of the compound No. 2.2 are dissolved in a mixture composed of 80 parts by weight of alkylated benzene, parts by weight of the adduct of from 8 to 10 mol of ethylene oxide to 1 mol of oleic acid N-monoethanolamide, 5 parts by weight of calcium salt of dodecylbenzenesulfonic acid and 5 parts by weight of the adduct of 40 mol of ethylene oxide to 1 mol of castor oil. Pouring the solution into 100,000 parts by weight of water and finely distributing it therein gives an aqueous dispersion which comprises 0.02% by weight of the active compound. [0412] II. 20 parts by weight of the compound No. 3.1 are dissolved in a mixture composed of 40 parts by weight of cyclohexanone, 30 parts by weight of isobutanol, 20 parts by weight of the adduct of 7 mol of ethylene oxide to 1 mol of isooctylphenol and 10 parts by weight of the adduct of 40 mol of ethylene oxide to 1 mol of castor oil. Pouring the solution into 100,000 parts by weight of water and finely distributing it therein gives an aqueous dispersion which comprises 0.02% by weight of the active compound. [0413] III. 20 parts by weight of the compound No. 2.3 are dissolved in a mixture composed of 25 parts by weight of cyclohexanone, 65 parts by weight of a mineral oil fraction of boiling point 210 to 280.degree. C. and 10 parts by weight of the adduct of 40 mol of ethylene oxide to 1 mol of castor oil. Pouring the solution into 100,000 parts by weight of water and finely distributing it therein gives an aqueous dispersion which comprises 0.02% by weight of the active compound. [0414] IV. 20 parts by weight of the compound No. 2.4 are mixed thoroughly with 3 parts by weight of the sodium salt of diisobutylnaphthalenesulfonic acid, 17 parts by weight of the sodium salt of a lignosulfonic acid from a sulfite waste liquor and 60 parts by weight of pulverulent silica gel, and the mixture is ground in a hammer mill. Finely distributing the mixture in 20,000 parts by weight of water gives a spray mixture which comprises 0.1% by weight of the active compound. [0415] V. 3 parts by weight of the compound No. 2.3 are mixed with 97 parts by weight of finely divided kaolin. This gives a dust which comprises 3% by weight of the active compound. [0416] VI. 20 parts by weight of the compound No. 2.4 are mixed intimately with 2 parts by weight of calcium salt of dodecylbenzenesulfonic acid, 8 parts by weight of fatty alcohol polyglycol ether, 2 parts by weight of sodium salt of a phenol/urea/formaldehyde condensate and 68 parts by weight of a paraffinic mineral oil. This gives a stable oily dispersion. [0417] VII. 1 part by weight of the compound No. 2.2 is dissolved in a mixture composed of 70 parts by weight of cyclohexanone, 20 parts by weight of ethoxylated isooctylphenol and 10 parts by weight of ethoxylated castor oil. This gives a stable emulsion concentrate. [0418] VIII. 1 part by weight of the compound No. 3.1 is dissolved in a mixture composed of 80 parts by weight of cyclohexanone and 20 parts by weight of Wettol.RTM. EM 31 (=nonionic emulsifier based on ethoxylated castor oil). This gives a stable emulsion concentrate.

[0419] The compounds of the formula I or the herbicidal compositions can be applied pre- or post-emergence. If the active compounds are less well tolerated by certain crop plants, application techniques may be used in which the herbicidal compositions are sprayed, with the aid of the spraying equipment, in such a way that as far as possible they do not come into contact with the leaves of the sensitive crop plants, while the active compounds reach the leaves of undesirable plants growing underneath, or the bare soil surface (post-directed, lay-by).

[0420] The rates of application of the compound of the formula I are from 0.001 to 3.0, preferably 0.01 to 1.0, kg/ha of active substance (a.s.), depending on the control target, the season, the target plants and the growth stage.

[0421] To widen the spectrum of action and to achieve synergistic effects, the tricyclic benzylpyrazole derivatives of the formula I may be mixed with a large number of representatives of other herbicidal or growth-regulating active compound groups and applied concomitantly. Suitable components for mixtures are, for example, 1,2,4-thiadiazoles, 1,3,4-thiadiazoles, amides, aminophosphoric acid and its derivatives, aminotriazoles, anilides, aryloxy-/heteroaryloxyalkanoic acids and their derivatives, benzoic acid and its derivatives, benzothiadiazinones, 2-aroyl-1,3-cyclohexanediones, heteroaryl aryl ketones, benzylisoxazolidinones, meta-CF.sub.3-phenyl derivatives, carbamates, quinoline carboxylic acid and its derivatives, chloroacetanilides, cyclohexenone oxime ether derivatives, diazines, dichloropropionic acid and its derivatives, dihydrobenzofurans, dihydrofuran-3-ones, dinitroanilines, dinitrophenols, diphenyl ethers, dipyridyls, halocarboxylic acids and their derivatives, ureas, 3-phenyluracils, imidazoles, imidazolinones, N-phenyl-3,4,5,6-tetrahydrophthalimides, oxadiazoles, oxiranes, phenols, aryloxy- and hetaryloxyphenoxypropionic esters, phenylactic acid and its derivatives, 2-phenylpropionic acid and its derivatives, pyrazoles, phenylpyrazoles, pyridazines, pyridinecarboxylic acid and its derivatives, pyrimidyl ethers, sulfonamides, sulfonylureas, triazines, triazinones, triazolinones, triazolecarboxamides and uracils.

[0422] It may furthermore be advantageous to apply the compounds of the formula I, alone or in combination with other herbicides, in the form of a mixture with other crop protection agents, for example together with agents for controlling pests or phytopathogenic fungi or bacteria. Also of interest is the miscibility with mineral salt solutions, which are employed for treating nutritional and trace element deficiencies. Non-phytotoxic oils and oil concentrates may also be added.

USE EXAMPLES

[0423] The herbicidal activity of the tricyclic benzylpyrazole derivatives of the formula I was demonstrated by the following greenhouse experiments:

[0424] The culture containers used were plastic pots containing loamy sand with approximately 3.0% of humus as the substrate. The seeds of the test plants were sown separately for each species.

[0425] For the pre-emergence treatment, the active compounds, which had been suspended or emulsified in water, were applied directly after sowing by means of finely distributing nozzles. The containers were irrigated gently to promote germination and growth and subsequently covered with transparent plastic hoods until the plants had rooted. This cover causes uniform germination of the test plants, unless this was adversely affected by the active compounds.

[0426] For post-emergence treatment, the test plants were first grown to a plant height of from 3 to 15 cm, depending on the plant habit, and only then treated with the active compounds which had been suspended or emulsified in water. For this purpose, the test plants were either sown directly and grown in the same containers, or they were first grown separately as seedlings and transplanted into the test containers a few days prior to the treatment. The application rate for the post-emergence treatment was 0.5 or 0.25 kg of a.s./ha.

[0427] Depending on the species, the plants were kept at 10-25.degree. C. or 20-35.degree. C. The test period extended over 2 to 4 weeks. During this time, the plants were tended, and their response to the individual treatments was evaluated.

[0428] Evaluation was carried out using a scale from 0 to 100. 100 means no emergence of the plants, or complete destruction of at least the above-ground parts, and 0 means no damage, or normal course of growth.

[0429] The plants used in the greenhouse trials were of the following species: TABLE-US-00006 Scientific Name Common Name Chenopodium album lambsquarters (goosefoot) Echinochloa crusgalli barnyardgrass Setaria viridis green foxtail Solanum nigrum black nightshade Veronica ssp. speadwell

[0430] At application rates of 0.5 or 0.25 kg/ha, the compound 2.2 shows very good activity against the abovementioned undesired broad-leaved weeds and weed grasses when applied by the post-emergence method.

Claims

1.-20. (canceled)

21. A tricyclic benzoylpyrazole compound of formula I ##STR64## where: X is oxygen, sulfur, S.dbd.O, S(.dbd.O).sub.2, CR.sup.6R.sup.7, or NR.sup.8; Y together with the two carbons to which it is attached forms a saturated, partially saturated or unsaturated 5- or 6-membered heterocycle which contains one to three identical or different heteroatoms selected from the following group: oxygen, sulfur and nitrogen; R.sup.1, R.sup.2, R.sup.6, R.sup.7 are hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; R.sup.3 is halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; R.sup.4 is hydrogen, nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl)amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; R.sup.5 is hydrogen, C.sub.1-C.sub.6-alkyl or halogen; R.sup.8 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkylcarbonyl, formyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.1-C.sub.6-haloalkoxycarbonyl, C.sub.1-C.sub.6-alkylsulfonyl or C.sub.1-C.sub.6-haloalkylsulfonyl; l is 0, 1 or 2; R.sup.9 is a radical IIa or IIb ##STR65## where R.sup.10 is hydroxyl, mercapto, halogen, OR.sup.13, SR.sup.13, SO.sub.2R.sup.14, NR.sup.15R.sup.16 or N-bonded heterocyclyl, where the heterocyclyl radical may be partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; R.sup.11 is hydrogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.3-C.sub.6-cycloalkyl, hydroxyl, C.sub.1-C.sub.6-alkoxy or C.sub.1-C.sub.6-haloalkoxy; R.sup.12 is hydrogen, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, hydroxyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-haloalkylthio; R.sup.13 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-alkynyl, C.sub.3-C.sub.6-haloalkynyl, C.sub.3-C.sub.6-cycloalkyl, C.sub.1-C.sub.20-alkylcarbonyl, C.sub.2-C.sub.20-alkenylcarbonyl, C.sub.2-C.sub.6-alkynylcarbonyl, C.sub.3-C.sub.6-cycloalkylcarbonyl, C.sub.1-C.sub.6-alkoxycarbonyl, C.sub.3-C.sub.6-alkenyloxycarbonyl, C.sub.3-C.sub.6-alkynyloxycarbonyl, C.sub.1-C.sub.6-alkylthiocarbonyl, C.sub.1-C.sub.6-alkylaminocarbonyl, C.sub.3-C.sub.6-alkenylaminocarbonyl, C.sub.3-C.sub.6-alkynylaminocarbonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.1-C.sub.6-alkoxy)-N--(C.sub.1-C.sub.6-alkyl)aminocarbonyl, N--(C.sub.3-C.sub.6-alkenyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl, N--(C.sub.3-C.sub.6-alkynyl)-N--(C.sub.1-C.sub.6-alkoxy)aminocarbonyl, di(C.sub.1-C.sub.6-alkyl)aminothiocarbonyl, C.sub.1-C.sub.6-alkylcarbonyl-C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-alkoxyimino-C.sub.1-C.sub.6-alkyl, N--(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl or N,N-di(C.sub.1-C.sub.6-alkylamino)imino-C.sub.1-C.sub.6-alkyl, where the abovementioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three of the following groups: cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, di(C.sub.1-C.sub.4-alkyl)amino, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxycarbonyl, di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, C.sub.1-C.sub.4-alkylaminocarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl, heterocyclyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl-C.sub.1-C.sub.6-alkyl, heterocyclylcarbonyl-C.sub.1-C.sub.6-alkyl, phenylcarbonyl, heterocyclylcarbonyl, phenoxycarbonyl, phenyloxythiocarbonyl, heterocyclyloxycarbonyl, heterocyclyloxythiocarbonyl, phenylaminocarbonyl, N--(C.sub.1-C.sub.6-alkyl)-N-(phenyl)aminocarbonyl, heterocyclylaminocarbonyl, N--(C.sub.1-C.sub.6-alkyl)-N-(heterocyclyl)aminocarbonyl, phenyl-C.sub.2-C.sub.6-alkenylcarbonyl or heterocyclyl-C.sub.2-C.sub.6-alkenylcarbonyl, where the phenyl and the heterocyclyl radical of the 18 lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-haloalkoxy, heterocyclyl or N-bonded heterocyclyl, where the two lastmentioned substitutents for their part may be partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; R.sup.14 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-alkynyl, C.sub.3-C.sub.6-haloalkynyl, C.sub.3-C.sub.6-cycloalkyl, C.sub.1-C.sub.6-alkoxy, di(C.sub.1-C.sub.6-alkyl)amino or di(C.sub.1-C.sub.6-haloalkyl)amino, where the abovementioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three of the following groups: cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, di(C.sub.1-C.sub.4-alkyl)amino, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxycarbonyl, di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, C.sub.1-C.sub.4-alkylaminocarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl, heterocyclyl-C.sub.1-C.sub.6-alkyl, phenoxy, heterocyclyloxy, where the phenyl and the heterocyclyl radical of the lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; R.sup.15 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-haloalkenyl, C.sub.3-C.sub.6-alkynyl, C.sub.3-C.sub.6-haloalkynyl, C.sub.3-C.sub.6-cycloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.3-C.sub.6-alkenyloxy, C.sub.3-C.sub.6-alkynyloxy, di(C.sub.1-C.sub.6-alkyl)amino or C.sub.1-C.sub.6-alkylcarbonylamino, where the abovementioned alkyl, cycloalkyl and alkoxy radicals may be partially or fully halogenated and/or may carry one to three radicals of the following group: cyano, C.sub.1-C.sub.4-alkoxy, C.sub.1-C.sub.4-alkylthio, di(C.sub.1-C.sub.4-alkyl)amino, C.sub.1-C.sub.4-alkylcarbonyl, C.sub.1-C.sub.4-alkoxycarbonyl, C.sub.1-C.sub.4-alkoxy-C.sub.1-C.sub.4-alkoxycarbonyl, di(C.sub.1-C.sub.4-alkyl)amino-C.sub.1-C.sub.4-alkoxycarbonyl, hydroxycarbonyl, C.sub.1-C.sub.4-alkylaminocarbonyl, di(C.sub.1-C.sub.4-alkyl)aminocarbonyl, aminocarbonyl, C.sub.1-C.sub.4-alkylcarbonyloxy or C.sub.3-C.sub.6-cycloalkyl; is phenyl, heterocyclyl, phenyl-C.sub.1-C.sub.6-alkyl or heterocyclyl-C.sub.1-C.sub.6-alkyl, where the phenyl or heterocyclyl radical of the four lastmentioned substitutents may be partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy; R.sup.16 is C.sub.1-C.sub.6-alkyl, C.sub.3-C.sub.6-alkenyl, C.sub.3-C.sub.6-alkynyl or C.sub.1-C.sub.6-alkylcarbonyl; or an agriculturally useful salt thereof.

22. The tricyclic benzoylpyrazole compound of formula I defined in claim 21 where R.sup.9 is IIa.

23. The tricyclic benzoylpyrazole compound of formula I defined in claim 21 where X is oxygen, sulfur or CR.sup.6R.sup.7.

24. The tricyclic benzoylpyrazole compound of formula I defined in claim 21 where Y together with the two carbons to which it is attached forms a heterocycle selected from the following group: dihydroisoxazolediyl, isoxazolediyl or tetrahydroisoxazolediyl.

25. The tricyclic benzoylpyrazole compound of formula I defined in claim 21 where R.sup.1, R.sup.2 are hydrogen; R.sup.3 is C.sub.1-C.sub.6-alkyl; R.sup.4 is nitro, halogen, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-alkylthio or C.sub.1-C.sub.6-alkylsulfonyl; R.sup.5 is hydrogen; l is 0 oder 1.

26. The tricyclic benzoylpyrazole compound of formula I defined in claim 21 where R.sup.10 is hydroxyl; R.sup.11 is C.sub.1-C.sub.6-alkyl or C.sub.3-C.sub.6-cycloalkyl; R.sup.12 is hydrogen or C.sub.1-C.sub.6-alkyl.

27. A process for preparing the compound of formula I where R.sup.10=halogen as claimed in claim 21, which comprises reacting a tricyclic benzoylpyrazole compound of formula I.alpha. (=I where R.sup.10=hydroxyl), ##STR66## where the variables R.sup.1 to R.sup.5, R.sup.11 and R.sup.12, X, Y and l are as defined in claim 21, with a halogenating agent.

28. A process for preparing the compound of formula I where R.sup.10=OR.sup.13 as claimed in claim 21, which comprises reacting a tricyclic benzoylpyrazole compound of formula I.alpha. (=I where R.sup.10=hydroxyl), ##STR67## where the variables R.sup.1 to R.sup.5, R.sup.11 and R.sup.12, X, Y and l are as defined in claim 21, with a compound of formula III L.sup.1R.sup.13 III where the variable R.sup.13 is as defined in claim 21 and L.sup.1 is a nucleophilically replaceable leaving group.

29. A process for preparing the compound of formula I where R.sup.10=OR.sup.13, SR.sup.13, NR.sup.15R.sup.16 or N-bonded heterocyclyl as claimed in claim 21, which comprises reacting a compound of formula I.beta. (.ident.I where R.sup.10=halogen), ##STR68## where the variables R.sup.1 to R.sup.5, R.sup.11 and R.sup.12, X, Y and l are as defined in claim 21, with a compound of formula IV.alpha., IV.beta., IV.gamma. or IV.delta. ##STR69## HOR.sup.13HSR.sup.13NHR.sup.15R.sup.16H(N-bonded heterocyclyl) Ivo. IVp ivy IV8 where the variables R.sup.13 to R.sup.16 are as defined in claim 21, optionally in the presence of a base.

30. A process for preparing the compound of formula I where R.sup.10=SO.sub.2R.sup.14 as claimed in claim 21, which comprises reacting a compound of formula I.gamma. (.ident.I where R.sup.10=SR.sup.14), ##STR70## where the variables R.sup.1 to R.sup.5, R.sup.11 and R.sup.12, X, Y and l are as defined in claim 21, with an oxidizing agent.

31. A process for preparing the compound of formula I where R.sup.9=IIa as claimed in claim 21, which comprises reacting a metalated pyrazole compound of formula V where M is a metal and R.sup.10 to R.sup.12 are as defined in claim 21, except for R.sup.10=hydroxyl and mercapto, with a tricyclic benzoic acid compound of formula VI.alpha. where R.sup.1 to R.sup.5, X, Y and l are as defined in claim 21 and L.sup.2 is a nucleophilically replaceable leaving group. ##STR71##

32. A process for preparing the compound of formula I.alpha. (=I where R.sup.10=hydroxyl) as claimed in claim 21, which comprises acylating a pyrazole of formula VII in which the variables R.sup.11 and R.sup.12 are as defined in claim 21 ##STR72## with an activated tricyclic benzoic acid of formula VI.beta. or with a tricyclic benzoic acid of formula VI.gamma., ##STR73## where the variables R.sup.1 to R.sup.5, X, Y and l are as defined in claim 21 and L.sup.3 is a nucleophilically replaceable leaving group, and rearranging the acylation product, optionally in the presence of a catalyst.

33. A process for preparing the compound of formula I.alpha. (.ident.I where R.sup.10=hydroxyl) as claimed in claim 21, which comprises reacting a pyrazole of formula VII in which the variables R.sup.11 and R.sup.12 are as defined in claim 21, or an alkali metal salt thereof, ##STR74## with a tricyclic benzene compound of formula IX where L.sup.4 is a leaving group and the variables X, Y, R.sup.1 to R.sup.5 and l are as defined in claim 21 ##STR75## in the presence of carbon monoxide, a catalyst and a base.

34. A composition, comprising a herbicidally effective amount of at least one compound of formula I or an agriculturally useful salt thereof as claimed in claim 21 and auxiliaries which are customary for formulating crop protection agents.

35. A process for preparing the composition defined in claim 34, which comprises mixing a herbicidally effective amount of at least one compound of formula I or an agriculturally useful salt thereof and auxiliaries which are customary for formulating crop protection agents.

36. A method for controlling undesirable vegetation, which comprises allowing a herbicidally effective amount of at least one compound of formula I or an agriculturally useful salt thereof as claimed in claim 21 to act on plants, their habitat or on seed.

37. A tricyclic benzoic acid compound of formula VI ##STR76## in which the variables X, Y, R.sup.1 to R.sup.3 and R.sup.5 and l are as defined in claim 21 and R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl)amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; R.sup.17 is hydroxyl or a radical which can be removed by hydrolysis.

38. A tricyclic benzene compound of formula IX ##STR77## in which the variables X, Y, R.sup.1 to R.sup.3 and R.sup.5 and l are as defined in claim 21 and R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-alkyl, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl)amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; R.sup.5 is hydrogen or C.sub.1-C.sub.6-alkyl; L.sup.4 is halogen, C.sub.1-C.sub.6-alkylsulfonyloxy, C.sub.1-C.sub.6-haloalkylsulfonyloxy or phenylsulfonyloxy, where the phenyl ring of the lastmentioned radical may be unsubstituted or partially or fully halogenated and/or may carry one to three of the following radicals: nitro, cyano, C.sub.1-C.sub.4-alkyl, C.sub.1-C.sub.4-haloalkyl, C.sub.1-C.sub.4-alkoxy or C.sub.1-C.sub.4-haloalkoxy.

39. An aniline compound of formula XV ##STR78## in which the variables X, Y, R.sup.1 to R.sup.3 and R.sup.5 and 1 are in each case as defined in claim 21 and R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkoxy, C.sub.1-C.sub.6-haloalkoxy, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl)amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino.

40. A nitrile compound of formula XVI ##STR79## in which the variables X, Y, R.sup.1 to R.sup.3 and l are in each case as defined in claim 21 and R.sup.4 is nitro, halogen, cyano, C.sub.1-C.sub.6-haloalkyl, C.sub.1-C.sub.6-alkylthio, C.sub.1-C.sub.6-haloalkylthio, C.sub.1-C.sub.6-alkylsulfinyl, C.sub.1-C.sub.6-haloalkinylsulfinyl, C.sub.1-C.sub.6-alkylsulfonyl, C.sub.1-C.sub.6-haloalkylsulfonyl, aminosulfonyl, N--(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N,N-di-(C.sub.1-C.sub.6-alkyl)aminosulfonyl, N--(C.sub.1-C.sub.6-alkylsulfonyl)amino, N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino, N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-alkylsulfonyl)amino or N--(C.sub.1-C.sub.6-alkyl)-N--(C.sub.1-C.sub.6-haloalkylsulfonyl)amino; R.sup.5 is hydrogen or C.sub.1-C.sub.6-alkyl.

41. The compound of formula I defined in claim 21, wherein X is O or S; Y together with the two carbons to which it is attached forms an isoxazole ring which is saturated, partially saturated or unsaturated; and R.sup.9 is a radical IIa.

42. The compound of formula I defined in claim 41, wherein R.sup.10 is hydroxyl, mercapto, halogen, OR.sup.13, SR.sup.13, SO.sub.2R.sup.14 or NR.sup.15R.sup.16.